Al-modified environmental barrier coatings for protection against water vapor corrosion
High-temperature water vapor corrosion is a great challenge for long lifetime of Si/mullite/Yb2SiO5 Environmental Barrier Coatings. In this work, the Yb3Al5O12 modified layer was in-situ synthesized on the surface of Yb2SiO5 layer to improve the steam resistance. The reaction mechanism of the Al-mod...
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Published in | Corrosion science Vol. 217; p. 111123 |
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Main Authors | , , , , , , , |
Format | Journal Article |
Language | English |
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Elsevier Ltd
01.06.2023
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Abstract | High-temperature water vapor corrosion is a great challenge for long lifetime of Si/mullite/Yb2SiO5 Environmental Barrier Coatings. In this work, the Yb3Al5O12 modified layer was in-situ synthesized on the surface of Yb2SiO5 layer to improve the steam resistance. The reaction mechanism of the Al-modified layer was explored. The steam corrosion experimental results indicated that the defects in Yb2SiO5 layer healed, and the oxidation rate of Si-bonded coating was slowed down under the protection of modified layer. Additionally, the calculation results of first-principle molecular dynamics confirmed that Yb3Al5O12 has excellent steam corrosion resistance.
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•A protective layer was prepared on the surface of the Yb2SiO5 coating through the Al-modification method.•The reaction of Yb3Al5O12 with water vapor needs to break through a higher energy barrier than that of Yb2O3 and Yb2SiO5 at 1400 ℃.•The Al-modified EBCs exhibited excellent water vapor corrosion resistance due to the formation of a new Yb3Al5O12 phase as well as the healing of voids and microcracks in the Yb2SiO5 coating. |
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AbstractList | High-temperature water vapor corrosion is a great challenge for long lifetime of Si/mullite/Yb2SiO5 Environmental Barrier Coatings. In this work, the Yb3Al5O12 modified layer was in-situ synthesized on the surface of Yb2SiO5 layer to improve the steam resistance. The reaction mechanism of the Al-modified layer was explored. The steam corrosion experimental results indicated that the defects in Yb2SiO5 layer healed, and the oxidation rate of Si-bonded coating was slowed down under the protection of modified layer. Additionally, the calculation results of first-principle molecular dynamics confirmed that Yb3Al5O12 has excellent steam corrosion resistance.
[Display omitted]
•A protective layer was prepared on the surface of the Yb2SiO5 coating through the Al-modification method.•The reaction of Yb3Al5O12 with water vapor needs to break through a higher energy barrier than that of Yb2O3 and Yb2SiO5 at 1400 ℃.•The Al-modified EBCs exhibited excellent water vapor corrosion resistance due to the formation of a new Yb3Al5O12 phase as well as the healing of voids and microcracks in the Yb2SiO5 coating. |
ArticleNumber | 111123 |
Author | Fan, Zhengjie Wang, Chao Wu, Jian Zhuo, Xueshi Zhang, Xiaofeng Cui, Jianlei Mei, Xuesong Wang, Meng |
Author_xml | – sequence: 1 givenname: Xueshi surname: Zhuo fullname: Zhuo, Xueshi organization: State Key Laboratory for Manufacturing Systems Engineering, Xi'an Jiaotong University, Xi'an 710054, China – sequence: 2 givenname: Chao surname: Wang fullname: Wang, Chao organization: National Engineering Laboratory for Modern Materials Surface Engineering Technology & The Key Lab of Guangdong for Modern Surface Engineering Technology, Guangdong, China – sequence: 3 givenname: Meng surname: Wang fullname: Wang, Meng organization: School of Materials Science and Engineering, Research Center for Materials Genome Engineering, Wuhan University of Technology, Wuhan 430070, China – sequence: 4 givenname: Jian surname: Wu fullname: Wu, Jian organization: National Engineering Laboratory for Modern Materials Surface Engineering Technology & The Key Lab of Guangdong for Modern Surface Engineering Technology, Guangdong, China – sequence: 5 givenname: Xiaofeng surname: Zhang fullname: Zhang, Xiaofeng email: zxf200808@126.com organization: National Engineering Laboratory for Modern Materials Surface Engineering Technology & The Key Lab of Guangdong for Modern Surface Engineering Technology, Guangdong, China – sequence: 6 givenname: Jianlei surname: Cui fullname: Cui, Jianlei organization: State Key Laboratory for Manufacturing Systems Engineering, Xi'an Jiaotong University, Xi'an 710054, China – sequence: 7 givenname: Xuesong surname: Mei fullname: Mei, Xuesong organization: State Key Laboratory for Manufacturing Systems Engineering, Xi'an Jiaotong University, Xi'an 710054, China – sequence: 8 givenname: Zhengjie orcidid: 0000-0002-7106-8470 surname: Fan fullname: Fan, Zhengjie email: fanzhengjie@xjtu.edu.cn organization: State Key Laboratory for Manufacturing Systems Engineering, Xi'an Jiaotong University, Xi'an 710054, China |
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CitedBy_id | crossref_primary_10_1016_j_jeurceramsoc_2023_09_063 crossref_primary_10_1016_j_surfcoat_2024_130600 crossref_primary_10_1016_j_jmrt_2024_01_170 crossref_primary_10_1016_j_surfcoat_2024_130433 crossref_primary_10_1016_j_corsci_2024_112255 crossref_primary_10_1016_j_corsci_2024_111962 crossref_primary_10_1007_s44251_024_00039_4 crossref_primary_10_1016_j_surfcoat_2023_130317 |
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Keywords | Environmental barrier coatings Yb3Al5O12 Water vapor corrosion Oxidation Al-modified layer |
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Snippet | High-temperature water vapor corrosion is a great challenge for long lifetime of Si/mullite/Yb2SiO5 Environmental Barrier Coatings. In this work, the Yb3Al5O12... |
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SubjectTerms | Al-modified layer Environmental barrier coatings Oxidation Water vapor corrosion Yb3Al5O12 |
Title | Al-modified environmental barrier coatings for protection against water vapor corrosion |
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