Enhanced optoelectronic performances of FePS3/ReS2 Van der Waals heterostructures with type-II band alignment

FePS3, as a typical represent of newly emerged transition metal chalcogenophosphates (TMCPs) with antiferromagnetic properties, has been considered as a splendid candidate for ultraviolet (UV) photodetectors. However, the limited response spectra band and photoresponsivity has seriously restricted i...

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Published inMaterials today communications Vol. 35; p. 105959
Main Authors Gao, Honglei, Du, Changhui, Sun, Jie, Zhang, Jing, Leng, Jiancai, Li, Jianfei, Wang, Wenjia, Li, Kuilong
Format Journal Article
LanguageEnglish
Published Elsevier Ltd 01.06.2023
Subjects
FePS3/ReS2
Optical anisotropy
Photodetector
Photoresponsivity
Response speed
FePS3/ReS2
Photoresponsivity
Photodetector
Optical anisotropy
Response speed
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Abstract FePS3, as a typical represent of newly emerged transition metal chalcogenophosphates (TMCPs) with antiferromagnetic properties, has been considered as a splendid candidate for ultraviolet (UV) photodetectors. However, the limited response spectra band and photoresponsivity has seriously restricted its applications. As a typical representative of transition metal Re-based chalcogenides, ReS2 has an adjustable absorption band gap in the visible light band and extremely weak interlayer coupling force, which makes the material have higher absorbance and exciton transition probability, thereby greatly enhancing PL. Herein, we construct a high performance photodetector based on FePS3/ReS2 van der Waals (vdWs) heterostructure with excellent optical and optoelectronic properties. The in-plane optical anisotropic ratio of ReS2 nanoflake is significantly enhanced owing to the strong vdWs interlayer couplings, which is confirmed by the linear-polarized photoluminescence (PL) spectra. The photodetector exhibits broadband response spectrum ranging from UV to near-infrared (NIR) region, high photoresponsivity upto 102.5 A/W at 305 nm and 41.8 A/W at 638 nm, and fast response speed with rising/decaying times about 0.22/1.22 ms, which displays excellent superiority over other FePS3-based photodetectors. The high performances of FePS3/ReS2 are primarily attributed to the high electron mobility, strong light-matter interactions and built-in electric field at the heterointerface with type-II band alignment. The eminent and novel optoelectronic properties of the heterostructure pave promising platforms for the further development and applications of TMCPs in high-performance photodetections. [Display omitted] •High performance photodetectors based on FePS3/ReS2 heterostructures were fabricated.•The in-plane optical anisotropic ratio of ReS2 nanoflake is significantly enhanced.•The photodetector displays broadband photoresponse and high photoresponsivity.•The photodetector shows a fast response speed.
AbstractList FePS3, as a typical represent of newly emerged transition metal chalcogenophosphates (TMCPs) with antiferromagnetic properties, has been considered as a splendid candidate for ultraviolet (UV) photodetectors. However, the limited response spectra band and photoresponsivity has seriously restricted its applications. As a typical representative of transition metal Re-based chalcogenides, ReS2 has an adjustable absorption band gap in the visible light band and extremely weak interlayer coupling force, which makes the material have higher absorbance and exciton transition probability, thereby greatly enhancing PL. Herein, we construct a high performance photodetector based on FePS3/ReS2 van der Waals (vdWs) heterostructure with excellent optical and optoelectronic properties. The in-plane optical anisotropic ratio of ReS2 nanoflake is significantly enhanced owing to the strong vdWs interlayer couplings, which is confirmed by the linear-polarized photoluminescence (PL) spectra. The photodetector exhibits broadband response spectrum ranging from UV to near-infrared (NIR) region, high photoresponsivity upto 102.5 A/W at 305 nm and 41.8 A/W at 638 nm, and fast response speed with rising/decaying times about 0.22/1.22 ms, which displays excellent superiority over other FePS3-based photodetectors. The high performances of FePS3/ReS2 are primarily attributed to the high electron mobility, strong light-matter interactions and built-in electric field at the heterointerface with type-II band alignment. The eminent and novel optoelectronic properties of the heterostructure pave promising platforms for the further development and applications of TMCPs in high-performance photodetections. [Display omitted] •High performance photodetectors based on FePS3/ReS2 heterostructures were fabricated.•The in-plane optical anisotropic ratio of ReS2 nanoflake is significantly enhanced.•The photodetector displays broadband photoresponse and high photoresponsivity.•The photodetector shows a fast response speed.
ArticleNumber 105959
Author Gao, Honglei
Zhang, Jing
Du, Changhui
Leng, Jiancai
Wang, Wenjia
Li, Kuilong
Li, Jianfei
Sun, Jie
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  givenname: Jianfei
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  givenname: Wenjia
  surname: Wang
  fullname: Wang, Wenjia
  email: wangwenjia@qlu.edu.cn
  organization: International School For Optoelectronic Engineering, Qilu University of Technology (Shandong Academy of Sciences), Jinan 250353, China
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  givenname: Kuilong
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  fullname: Li, Kuilong
  email: kuilongli@qlu.edu.cn
  organization: International School For Optoelectronic Engineering, Qilu University of Technology (Shandong Academy of Sciences), Jinan 250353, China
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Keywords FePS3/ReS2
Photoresponsivity
Photodetector
Optical anisotropy
Response speed
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Snippet FePS3, as a typical represent of newly emerged transition metal chalcogenophosphates (TMCPs) with antiferromagnetic properties, has been considered as a...
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StartPage 105959
SubjectTerms FePS3/ReS2
Optical anisotropy
Photodetector
Photoresponsivity
Response speed
Title Enhanced optoelectronic performances of FePS3/ReS2 Van der Waals heterostructures with type-II band alignment
URI https://dx.doi.org/10.1016/j.mtcomm.2023.105959
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