Velocity map ion imaging of H atoms from the dissociation of HCO ( A ∼ 2 A ″ ) using Doppler-free multi-photon ionization
Velocity map ion imaging using Doppler-free 2+1 multi-photon ionization at λ = 243.1 nm has been applied to monitor the nascent H atoms from the predissociation of HCO ( A ∼ 2 A ″ ) in the (0, 0, 10 1) vibrational state. Employing two balanced, counterpropagating circularly (σ + and σ −) polarized p...
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Published in | Chemical physics letters Vol. 414; no. 4; pp. 473 - 478 |
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Main Authors | , , , , |
Format | Journal Article |
Language | English |
Published |
Elsevier B.V
14.10.2005
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Abstract | Velocity map ion imaging using Doppler-free 2+1 multi-photon ionization at
λ
=
243.1
nm has been applied to monitor the nascent H atoms from the predissociation of HCO (
A
∼
2
A
″
) in the (0,
0,
10
1) vibrational state. Employing two balanced, counterpropagating circularly (σ
+ and σ
−) polarized probe beams, complete velocity map images were accumulated with every laser shot without having to scan the probe wavelength over the strongly Doppler-broadened line profile. The H–CO bond dissociation energy, CO internal energy distribution, and anisotropy parameter are presented and compared with literature data. |
---|---|
AbstractList | Velocity map ion imaging using Doppler-free 2+1 multi-photon ionization at
λ
=
243.1
nm has been applied to monitor the nascent H atoms from the predissociation of HCO (
A
∼
2
A
″
) in the (0,
0,
10
1) vibrational state. Employing two balanced, counterpropagating circularly (σ
+ and σ
−) polarized probe beams, complete velocity map images were accumulated with every laser shot without having to scan the probe wavelength over the strongly Doppler-broadened line profile. The H–CO bond dissociation energy, CO internal energy distribution, and anisotropy parameter are presented and compared with literature data. |
Author | Riedel, J. Dziarzhytski, S. Temps, F. Renth, F. Kuczmann, A. |
Author_xml | – sequence: 1 givenname: J. surname: Riedel fullname: Riedel, J. – sequence: 2 givenname: S. surname: Dziarzhytski fullname: Dziarzhytski, S. – sequence: 3 givenname: A. surname: Kuczmann fullname: Kuczmann, A. – sequence: 4 givenname: F. surname: Renth fullname: Renth, F. – sequence: 5 givenname: F. surname: Temps fullname: Temps, F. email: temps@phc.uni-kiel.de |
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Title | Velocity map ion imaging of H atoms from the dissociation of HCO ( A ∼ 2 A ″ ) using Doppler-free multi-photon ionization |
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