New insights into “dead lithium” during stripping in lithium metal batteries
The formation of dead Lithium during stripping process is investigated in the whole course from the electron transfer, the conversion of Li0 to Li+ and the diffusion of Li+. [Display omitted] Lithium (Li) metal attributes to the promising anode but endures the low Columbic efficiency (CE) and safety...
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| Published in | Journal of energy chemistry Vol. 62; pp. 289 - 294 |
|---|---|
| Main Authors | , , , , |
| Format | Journal Article |
| Language | English |
| Published |
Elsevier B.V
01.11.2021
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| Subjects | |
| Online Access | Get full text |
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| Abstract | The formation of dead Lithium during stripping process is investigated in the whole course from the electron transfer, the conversion of Li0 to Li+ and the diffusion of Li+.
[Display omitted]
Lithium (Li) metal attributes to the promising anode but endures the low Columbic efficiency (CE) and safety issues from the inactive Li accumulation. The metallic Li which is isolated from the lithium anode (named dead Li0) consists the major component of the inactive Li. We systematically and meticulously investigated the formation and evaluation of dead Li0 during stripping process from electron transfer, the oxidation of Li0 to Li+ and the diffusion of Li+ through solid electrolyte interphase (SEI). The above-mentioned processes were regulated by adjusting the contact sites of electron channels, the dynamic rate of conversion from Li0 to Li+, and the structure as well as components of SEI. The design principles for achieving less dead Li0 and higher CE are proposed as a proof of concept in lithium metal batteries. This new insight sheds a comprehensive light on dead Li0 formation and guides the next-generation safe batteries for future application. |
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| AbstractList | The formation of dead Lithium during stripping process is investigated in the whole course from the electron transfer, the conversion of Li0 to Li+ and the diffusion of Li+.
[Display omitted]
Lithium (Li) metal attributes to the promising anode but endures the low Columbic efficiency (CE) and safety issues from the inactive Li accumulation. The metallic Li which is isolated from the lithium anode (named dead Li0) consists the major component of the inactive Li. We systematically and meticulously investigated the formation and evaluation of dead Li0 during stripping process from electron transfer, the oxidation of Li0 to Li+ and the diffusion of Li+ through solid electrolyte interphase (SEI). The above-mentioned processes were regulated by adjusting the contact sites of electron channels, the dynamic rate of conversion from Li0 to Li+, and the structure as well as components of SEI. The design principles for achieving less dead Li0 and higher CE are proposed as a proof of concept in lithium metal batteries. This new insight sheds a comprehensive light on dead Li0 formation and guides the next-generation safe batteries for future application. |
| Author | Ding, Jun-Fan Chen, Xiao-Ru Peng, Hong-Jie Zhang, Qiang Yan, Chong |
| Author_xml | – sequence: 1 givenname: Xiao-Ru surname: Chen fullname: Chen, Xiao-Ru organization: Beijing Key Laboratory of Green Chemical Reaction Engineering and Technology, Department of Chemical Engineering, Tsinghua University, Beijing 100084, China – sequence: 2 givenname: Chong surname: Yan fullname: Yan, Chong organization: Beijing Key Laboratory of Green Chemical Reaction Engineering and Technology, Department of Chemical Engineering, Tsinghua University, Beijing 100084, China – sequence: 3 givenname: Jun-Fan surname: Ding fullname: Ding, Jun-Fan organization: Advanced Research Institute of Multidisciplinary Science, School of Materials Science and Engineering, Beijing Institute of Technology, Beijing 100081, China – sequence: 4 givenname: Hong-Jie surname: Peng fullname: Peng, Hong-Jie organization: Department of Chemical Engineering, Stanford University, Stanford, CA 94305, USA – sequence: 5 givenname: Qiang orcidid: 0000-0002-3929-1541 surname: Zhang fullname: Zhang, Qiang email: zhang-qiang@mails.tsinghua.edu.cn organization: Beijing Key Laboratory of Green Chemical Reaction Engineering and Technology, Department of Chemical Engineering, Tsinghua University, Beijing 100084, China |
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| Keywords | Lithium metal batteries Lithium dendrite growth Dead lithium Charge transfer Lithium stripping |
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| Snippet | The formation of dead Lithium during stripping process is investigated in the whole course from the electron transfer, the conversion of Li0 to Li+ and the... |
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| SubjectTerms | Charge transfer Dead lithium Lithium dendrite growth Lithium metal batteries Lithium stripping |
| Title | New insights into “dead lithium” during stripping in lithium metal batteries |
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