Effective photocurrent generation in supramolecular porphyrin-fullerene conjugates assembled by crown ether-alkyl ammonium cation interactions
In this paper, a new approach for fabricating donor-acceptor (D-A) arrays, (Si-TCP)n-PhC60NH3+, 5,10,15,20-Tetrakis(benzo-15-crown-5)porphyrin (TCP), 2-Phenyl-5-(n-butylammonium)-3,4-fulleropyrrolidine (PhC60NH3+), on indium-tin oxide (ITO) electrode is demonstrated. Electronic absorption spectra, a...
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Published in | Dyes and pigments Vol. 151; pp. 385 - 390 |
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Language | English |
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Abstract | In this paper, a new approach for fabricating donor-acceptor (D-A) arrays, (Si-TCP)n-PhC60NH3+, 5,10,15,20-Tetrakis(benzo-15-crown-5)porphyrin (TCP), 2-Phenyl-5-(n-butylammonium)-3,4-fulleropyrrolidine (PhC60NH3+), on indium-tin oxide (ITO) electrode is demonstrated. Electronic absorption spectra, atomic force microscopy, infrared spectroscopy, electrochemical impedance spectroscopy, and X-ray diffraction analysis were used as powerful tools to characterize (Si-TCP)n arrays and (Si-TCP)n-PhC60NH3+ arrays on the ITO electrode. The (Si-TCP)n-PhC60NH3+ arrays was immobilized on the electrode avoided the traditional fussy operations for immobilizing both porphyrin materials and fullerene, which led to a significantly reduction of background signal and an enhancement of initial photocurrent signal. These results would provide fundamental clues for the molecular design of high-performance organic photovoltaics.
A new approach for fabrication porphyrin-fullerene arrays immobilized on the ITO electrode was demonstrated, which led to an enhancement of photocurrent. [Display omitted]
•A new approach for fabrication porphyrin-fullerene arrays immobilized on the ITO electrode was demonstrated.•The porphyrin-fullerene arrays with precise controlling were obtained.•The porphyrin-fullerene arrays led to an enhancement of photocurrent. |
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AbstractList | In this paper, a new approach for fabricating donor-acceptor (D-A) arrays, (Si-TCP)n-PhC60NH3+, 5,10,15,20-Tetrakis(benzo-15-crown-5)porphyrin (TCP), 2-Phenyl-5-(n-butylammonium)-3,4-fulleropyrrolidine (PhC60NH3+), on indium-tin oxide (ITO) electrode is demonstrated. Electronic absorption spectra, atomic force microscopy, infrared spectroscopy, electrochemical impedance spectroscopy, and X-ray diffraction analysis were used as powerful tools to characterize (Si-TCP)n arrays and (Si-TCP)n-PhC60NH3+ arrays on the ITO electrode. The (Si-TCP)n-PhC60NH3+ arrays was immobilized on the electrode avoided the traditional fussy operations for immobilizing both porphyrin materials and fullerene, which led to a significantly reduction of background signal and an enhancement of initial photocurrent signal. These results would provide fundamental clues for the molecular design of high-performance organic photovoltaics.
A new approach for fabrication porphyrin-fullerene arrays immobilized on the ITO electrode was demonstrated, which led to an enhancement of photocurrent. [Display omitted]
•A new approach for fabrication porphyrin-fullerene arrays immobilized on the ITO electrode was demonstrated.•The porphyrin-fullerene arrays with precise controlling were obtained.•The porphyrin-fullerene arrays led to an enhancement of photocurrent. |
Author | Wang, Yucheng Song, Feifei Zhu, Peihua Ma, Pan Li, Shanshan |
Author_xml | – sequence: 1 givenname: Peihua surname: Zhu fullname: Zhu, Peihua email: chm_zhuph@ujn.edu.cn organization: School of Chemistry and Chemical Engineering, University of Jinan, Jinan, 250022, China – sequence: 2 givenname: Feifei surname: Song fullname: Song, Feifei organization: School of Chemistry and Chemical Engineering, University of Jinan, Jinan, 250022, China – sequence: 3 givenname: Pan surname: Ma fullname: Ma, Pan organization: Jinan Academy of Agricultural Sciences, Jinan, 250316, China – sequence: 4 givenname: Shanshan surname: Li fullname: Li, Shanshan organization: School of Chemistry and Chemical Engineering, University of Jinan, Jinan, 250022, China – sequence: 5 givenname: Yucheng surname: Wang fullname: Wang, Yucheng organization: School of Chemistry and Chemical Engineering, University of Jinan, Jinan, 250022, China |
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CitedBy_id | crossref_primary_10_1016_j_synthmet_2020_116635 crossref_primary_10_1016_j_dyepig_2020_108918 crossref_primary_10_1134_S0036024422040240 crossref_primary_10_1021_acs_jpcc_9b11661 |
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Keywords | Fullerene Photoelectrochemistry Crown ether Porphyrin D-A arrays |
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Snippet | In this paper, a new approach for fabricating donor-acceptor (D-A) arrays, (Si-TCP)n-PhC60NH3+, 5,10,15,20-Tetrakis(benzo-15-crown-5)porphyrin (TCP),... |
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SubjectTerms | Crown ether D-A arrays Fullerene Photoelectrochemistry Porphyrin |
Title | Effective photocurrent generation in supramolecular porphyrin-fullerene conjugates assembled by crown ether-alkyl ammonium cation interactions |
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