Enhanced stretchability of porous PDMS/CIP composites via weak interfacial bonding and their electromagnetic noise suppression properties

[Display omitted] •Polydimethylsiloxane sponge was fabricated using an eco-friendly sacrificial template method.•The stretchability of the PDMS composite was achieved to be 1.2–1.6 times higher by using modified-CIP.•Porous CIP/PDMS composite exhibits improved EM wave absorption compared to non-poro...

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Published inApplied surface science Vol. 664; p. 160200
Main Authors Hong, Seungwoo, Qaiser, Nadeem, Ha, Heebo, Hwang, Byungil
Format Journal Article
LanguageEnglish
Published Elsevier B.V 15.08.2024
Subjects
Carbonyl iron powder
Mechanical properties
Polymer matrix composites
Porous
Stretchable
Mechanical properties
Stretchable
Polymer matrix composites
Carbonyl iron powder
Porous
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Abstract [Display omitted] •Polydimethylsiloxane sponge was fabricated using an eco-friendly sacrificial template method.•The stretchability of the PDMS composite was achieved to be 1.2–1.6 times higher by using modified-CIP.•Porous CIP/PDMS composite exhibits improved EM wave absorption compared to non-porous CIP/PDMS composite. The development of wearable devices operated through massive data communication necessitates the use of lightweight, highly efficient stretchable composites to suppress electromagnetic (EM) noise. In this study, highly stretchable porous polydimethylsiloxane (PDMS)/carbonyl iron powder (CIP) composite-based EM noise suppressors were explored. The porous structure reduced the volume fraction of PDMS in the composites, leading to a reduction in the total weight of the composites. The introduction of CIP to porous PDMS initially degraded stretchability owing to stress concentration at the strongly bonded interfaces between the CIP surface and PDMS. However, reducing the interfacial bonding strength by removing the SiO2 layer on the CIP surface significantly enhanced stretchability, causing the resulting composite to display 1.2–1.6 times higher rupture strain values at the same CIP loading contents than those with high interfacial bonding strength. The EM absorption properties of the porous and nonporous PDMS/CIP composites were characterized, and the porous PDMS/CIP composites exhibited ∼1.5 times higher EM noise suppression performance than the nonporous composites. This improvement is attributed to the vacant space within the porous framework filled with air, which enhances impedance matching and extends the transmission route of EM waves.
AbstractList [Display omitted] •Polydimethylsiloxane sponge was fabricated using an eco-friendly sacrificial template method.•The stretchability of the PDMS composite was achieved to be 1.2–1.6 times higher by using modified-CIP.•Porous CIP/PDMS composite exhibits improved EM wave absorption compared to non-porous CIP/PDMS composite. The development of wearable devices operated through massive data communication necessitates the use of lightweight, highly efficient stretchable composites to suppress electromagnetic (EM) noise. In this study, highly stretchable porous polydimethylsiloxane (PDMS)/carbonyl iron powder (CIP) composite-based EM noise suppressors were explored. The porous structure reduced the volume fraction of PDMS in the composites, leading to a reduction in the total weight of the composites. The introduction of CIP to porous PDMS initially degraded stretchability owing to stress concentration at the strongly bonded interfaces between the CIP surface and PDMS. However, reducing the interfacial bonding strength by removing the SiO2 layer on the CIP surface significantly enhanced stretchability, causing the resulting composite to display 1.2–1.6 times higher rupture strain values at the same CIP loading contents than those with high interfacial bonding strength. The EM absorption properties of the porous and nonporous PDMS/CIP composites were characterized, and the porous PDMS/CIP composites exhibited ∼1.5 times higher EM noise suppression performance than the nonporous composites. This improvement is attributed to the vacant space within the porous framework filled with air, which enhances impedance matching and extends the transmission route of EM waves.
ArticleNumber 160200
Author Hong, Seungwoo
Ha, Heebo
Qaiser, Nadeem
Hwang, Byungil
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  surname: Hong
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Stretchable
Polymer matrix composites
Carbonyl iron powder
Porous
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Snippet [Display omitted] •Polydimethylsiloxane sponge was fabricated using an eco-friendly sacrificial template method.•The stretchability of the PDMS composite was...
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SubjectTerms Carbonyl iron powder
Mechanical properties
Polymer matrix composites
Porous
Stretchable
Title Enhanced stretchability of porous PDMS/CIP composites via weak interfacial bonding and their electromagnetic noise suppression properties
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