Thermal safety of dendritic lithium against non-aqueous electrolyte in pouch-type lithium metal batteries
With the rise of the specific surface areas of Li deposits, the initial exothermic temperature between Li metal and electrolyte reduces gradually. The heat release of per gram Li increases firstly and then reduces in a working battery. [Display omitted] A quantitative relationship between safety iss...
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| Published in | Journal of energy chemistry Vol. 72; pp. 158 - 165 |
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| Main Authors | , , , , , , , , , |
| Format | Journal Article |
| Language | English |
| Published |
Elsevier B.V
01.09.2022
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| Subjects | |
| Online Access | Get full text |
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| Abstract | With the rise of the specific surface areas of Li deposits, the initial exothermic temperature between Li metal and electrolyte reduces gradually. The heat release of per gram Li increases firstly and then reduces in a working battery.
[Display omitted]
A quantitative relationship between safety issues and dendritic lithium (Li) has been rarely investigated yet. Herein the thermal stability of Li deposits with distinct surface area against non-aqueous electrolyte in pouch-type Li metal batteries is probed. The thermal runaway temperatures of Li metal batteries obtained by accelerating rate calorimeter are reduced from 211 °C for Li foil to 111 °C for cycled Li. The initial exothermic temperature is reduced from 194 °C for routine Li foil to 142 °C for 49.5 m2 g−1 dendrite. Li with different specific surface areas can regulate the reaction routes during the temperature range from 50 to 300 °C. The mass percent of Li foil and highly dendritic Li reacting with ethylene carbonate is higher than that of moderately dendritic Li. This contribution can strengthen the understanding of the thermal runaway mechanism and shed fresh light on the rational design of safe Li metal batteries. |
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| AbstractList | With the rise of the specific surface areas of Li deposits, the initial exothermic temperature between Li metal and electrolyte reduces gradually. The heat release of per gram Li increases firstly and then reduces in a working battery.
[Display omitted]
A quantitative relationship between safety issues and dendritic lithium (Li) has been rarely investigated yet. Herein the thermal stability of Li deposits with distinct surface area against non-aqueous electrolyte in pouch-type Li metal batteries is probed. The thermal runaway temperatures of Li metal batteries obtained by accelerating rate calorimeter are reduced from 211 °C for Li foil to 111 °C for cycled Li. The initial exothermic temperature is reduced from 194 °C for routine Li foil to 142 °C for 49.5 m2 g−1 dendrite. Li with different specific surface areas can regulate the reaction routes during the temperature range from 50 to 300 °C. The mass percent of Li foil and highly dendritic Li reacting with ethylene carbonate is higher than that of moderately dendritic Li. This contribution can strengthen the understanding of the thermal runaway mechanism and shed fresh light on the rational design of safe Li metal batteries. |
| Author | Shi, Peng Yuan, Hong Zhang, Qiang Yang, Shi-Jie Ding, Jun-Fan Huang, Jia-Qi Cheng, Xin-Bing Liu, Lei Jiang, Feng-Ni Chen, Xiang |
| Author_xml | – sequence: 1 givenname: Feng-Ni surname: Jiang fullname: Jiang, Feng-Ni organization: College of Chemistry and Chemical Engineering, Taiyuan University of Technology, Taiyuan 030024, Shanxi, China – sequence: 2 givenname: Shi-Jie surname: Yang fullname: Yang, Shi-Jie organization: Advanced Research Institute of Multidisciplinary Science, Beijing Institute of Technology, Beijing 100081, China – sequence: 3 givenname: Xin-Bing surname: Cheng fullname: Cheng, Xin-Bing email: chengxb@seu.edu.cn organization: Beijing Key Laboratory of Green Chemical Reaction Engineering and Technology, Department of Chemical Engineering, Tsinghua University, Beijing 100084, China – sequence: 4 givenname: Peng surname: Shi fullname: Shi, Peng organization: Beijing Key Laboratory of Green Chemical Reaction Engineering and Technology, Department of Chemical Engineering, Tsinghua University, Beijing 100084, China – sequence: 5 givenname: Jun-Fan surname: Ding fullname: Ding, Jun-Fan organization: Advanced Research Institute of Multidisciplinary Science, Beijing Institute of Technology, Beijing 100081, China – sequence: 6 givenname: Xiang surname: Chen fullname: Chen, Xiang organization: Beijing Key Laboratory of Green Chemical Reaction Engineering and Technology, Department of Chemical Engineering, Tsinghua University, Beijing 100084, China – sequence: 7 givenname: Hong surname: Yuan fullname: Yuan, Hong organization: Advanced Research Institute of Multidisciplinary Science, Beijing Institute of Technology, Beijing 100081, China – sequence: 8 givenname: Lei surname: Liu fullname: Liu, Lei email: liulei@tyut.edu.cn organization: College of Chemistry and Chemical Engineering, Taiyuan University of Technology, Taiyuan 030024, Shanxi, China – sequence: 9 givenname: Jia-Qi surname: Huang fullname: Huang, Jia-Qi organization: Advanced Research Institute of Multidisciplinary Science, Beijing Institute of Technology, Beijing 100081, China – sequence: 10 givenname: Qiang orcidid: 0000-0002-3929-1541 surname: Zhang fullname: Zhang, Qiang email: zhang-qiang@mails.tsinghua.edu.cn organization: Beijing Key Laboratory of Green Chemical Reaction Engineering and Technology, Department of Chemical Engineering, Tsinghua University, Beijing 100084, China |
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| Keywords | Pouch-type cell Lithium dendrite growth Battery safety Lithium metal anode Thermal runaway |
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| Title | Thermal safety of dendritic lithium against non-aqueous electrolyte in pouch-type lithium metal batteries |
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