Dual-layer vermiculite nanosheet based hybrid film to suppress dendrite growth in lithium metal batteries

A dual-layer vermiculite nanosheet based hybrid film can achieve a dendrite-free lithium metal anode. [Display omitted] Lithium metal anode has become a favorable candidate for next-generation rechargeable batteries. However, the unstable interface between lithium metal and electrolyte leads to the...

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Published inJournal of energy chemistry Vol. 69; pp. 205 - 210
Main Authors Xu, Xiang-Qun, Jiang, Feng-Ni, Yang, Shi-Jie, Xiao, Ye, Liu, He, Liu, Fangyang, Liu, Lei, Cheng, Xin-Bing
Format Journal Article
LanguageEnglish
Published Elsevier B.V 01.06.2022
Subjects
Dendrite
Dual-layer interface
Lithium metal anode
Organic-inorganic hybrid layer
Two-dimensional vermiculite nanosheet
Dual-layer interface
Organic-inorganic hybrid layer
Lithium metal anode
Two-dimensional vermiculite nanosheet
Dendrite
Online AccessGet full text
ISSN2095-4956
DOI10.1016/j.jechem.2022.01.019

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Abstract A dual-layer vermiculite nanosheet based hybrid film can achieve a dendrite-free lithium metal anode. [Display omitted] Lithium metal anode has become a favorable candidate for next-generation rechargeable batteries. However, the unstable interface between lithium metal and electrolyte leads to the growth of dendrites, resulting in the low Coulombic efficiency and even the safety concerns. Herein, a rigid-flexible dual-layer vermiculite nanosheet (VN) based organic-inorganic hybrid film on lithium metal anode is proposed to suppress dendrite growth and relieve volume fluctuations. The inner mechanically robust VN layer (3 μm thick) enhances the mechanical properties of the protective layer, while the outer polymer (4 μm thick) can enhance the flexibility of the hybrid layer. The Li | Li symmetric cell with protected lithium shows an extended life of over 670 h. The full cell with Li anode protected by dual-layer interface exhibits a better capacity retention of 80% after 174 cycles in comparison to bare Li anode with 94 cycles. This study provides a novel approach and a significant step towards prolonging lifespan of lithium metal batteries.
AbstractList A dual-layer vermiculite nanosheet based hybrid film can achieve a dendrite-free lithium metal anode. [Display omitted] Lithium metal anode has become a favorable candidate for next-generation rechargeable batteries. However, the unstable interface between lithium metal and electrolyte leads to the growth of dendrites, resulting in the low Coulombic efficiency and even the safety concerns. Herein, a rigid-flexible dual-layer vermiculite nanosheet (VN) based organic-inorganic hybrid film on lithium metal anode is proposed to suppress dendrite growth and relieve volume fluctuations. The inner mechanically robust VN layer (3 μm thick) enhances the mechanical properties of the protective layer, while the outer polymer (4 μm thick) can enhance the flexibility of the hybrid layer. The Li | Li symmetric cell with protected lithium shows an extended life of over 670 h. The full cell with Li anode protected by dual-layer interface exhibits a better capacity retention of 80% after 174 cycles in comparison to bare Li anode with 94 cycles. This study provides a novel approach and a significant step towards prolonging lifespan of lithium metal batteries.
Author Liu, He
Xiao, Ye
Yang, Shi-Jie
Liu, Fangyang
Xu, Xiang-Qun
Liu, Lei
Cheng, Xin-Bing
Jiang, Feng-Ni
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  email: cxb12@mails.tsinghua.edu.cn
  organization: Beijing Key Laboratory of Green Chemical Reaction Engineering and Technology, Department of Chemical Engineering, Tsinghua University, Beijing 100084, China
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Keywords Dual-layer interface
Organic-inorganic hybrid layer
Lithium metal anode
Two-dimensional vermiculite nanosheet
Dendrite
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Snippet A dual-layer vermiculite nanosheet based hybrid film can achieve a dendrite-free lithium metal anode. [Display omitted] Lithium metal anode has become a...
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StartPage 205
SubjectTerms Dendrite
Dual-layer interface
Lithium metal anode
Organic-inorganic hybrid layer
Two-dimensional vermiculite nanosheet
Title Dual-layer vermiculite nanosheet based hybrid film to suppress dendrite growth in lithium metal batteries
URI https://dx.doi.org/10.1016/j.jechem.2022.01.019
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