A sulfur-rich small molecule as a bifunctional interfacial layer for stable perovskite solar cells with efficiencies exceeding 22
Remarkable progress has been made in perovskite solar cells (PSCs) recently. However, the defects present in the perovskite layer act as non-radiative recombination centers to decrease the stability and restrict the further performance improvement of the device. We report herein a sulfur-rich two-di...
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| Published in | Nano energy Vol. 79; p. 105462 |
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| Main Authors | , , , , , |
| Format | Journal Article |
| Language | English |
| Published |
Elsevier Ltd
01.01.2021
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| Subjects | |
| Online Access | Get full text |
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| Abstract | Remarkable progress has been made in perovskite solar cells (PSCs) recently. However, the defects present in the perovskite layer act as non-radiative recombination centers to decrease the stability and restrict the further performance improvement of the device. We report herein a sulfur-rich two-dimensional small molecule, SMe-TATPyr, as a bifunctional layer to efficiently passivate the surface defects of perovskite and facilitate the hole transfer at the perovskite/spiro-OMeTAD interface. X-ray photoelectron spectroscopy analyses show that the sulfur atoms of SMe-TATPyr can passivate the uncoordinated Pb2+ defects and suppress the Pb0 defect formation as Lewis bases. As a result, the power conversion efficiency of PSCs is distinctly increased from 20.4% to 22.3%. Moreover, this simple interfacial modification could effectively enhance the stability of unencapsulated PSCs to retain 95% of the initial efficiency after storage for 1500 h at ambient conditions, in contrast to 70% efficiency retention of the device without SMe-TATPyr under the same conditions.
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A sulfur-rich two-dimensional small molecule, SMe-TATPyr, has been used as a bifunctional interlayer to efficiently passivate the surface defects of perovskite and facilitate the hole transfer at the perovskite/spiro-OMeTAD interface. The SMe-TATPyr-treated perovskite solar cells demonstrate a remarkable efficiency of 22.3%, along with 95% retention of the initial efficiency under storage for 1500 h at ambient conditions.
•A sulfur-rich small molecule is designed as a bifunctional reagent for interfacial defect passivation and hole transfer.•The use of the interfacial layer leads to the efficiency enhancement from 20.4% to 22.3%.•The effect of interfacial defect passivation is fully supported by different physical measurements. |
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| AbstractList | Remarkable progress has been made in perovskite solar cells (PSCs) recently. However, the defects present in the perovskite layer act as non-radiative recombination centers to decrease the stability and restrict the further performance improvement of the device. We report herein a sulfur-rich two-dimensional small molecule, SMe-TATPyr, as a bifunctional layer to efficiently passivate the surface defects of perovskite and facilitate the hole transfer at the perovskite/spiro-OMeTAD interface. X-ray photoelectron spectroscopy analyses show that the sulfur atoms of SMe-TATPyr can passivate the uncoordinated Pb2+ defects and suppress the Pb0 defect formation as Lewis bases. As a result, the power conversion efficiency of PSCs is distinctly increased from 20.4% to 22.3%. Moreover, this simple interfacial modification could effectively enhance the stability of unencapsulated PSCs to retain 95% of the initial efficiency after storage for 1500 h at ambient conditions, in contrast to 70% efficiency retention of the device without SMe-TATPyr under the same conditions.
[Display omitted]
A sulfur-rich two-dimensional small molecule, SMe-TATPyr, has been used as a bifunctional interlayer to efficiently passivate the surface defects of perovskite and facilitate the hole transfer at the perovskite/spiro-OMeTAD interface. The SMe-TATPyr-treated perovskite solar cells demonstrate a remarkable efficiency of 22.3%, along with 95% retention of the initial efficiency under storage for 1500 h at ambient conditions.
•A sulfur-rich small molecule is designed as a bifunctional reagent for interfacial defect passivation and hole transfer.•The use of the interfacial layer leads to the efficiency enhancement from 20.4% to 22.3%.•The effect of interfacial defect passivation is fully supported by different physical measurements. |
| ArticleNumber | 105462 |
| Author | Hu, Jin-Song Shao, Jiang-Yang Li, Ming-Hua Wang, Yu-Duan Sun, Tian-Ge Zhong, Yu-Wu |
| Author_xml | – sequence: 1 givenname: Ming-Hua surname: Li fullname: Li, Ming-Hua organization: Beijing National Laboratory for Molecular Sciences, CAS Research/Education Center for Excellence in Molecular Sciences, Institute of Chemistry, Chinese Academy of Sciences, Beijing 100190, China – sequence: 2 givenname: Tian-Ge surname: Sun fullname: Sun, Tian-Ge organization: Beijing National Laboratory for Molecular Sciences, CAS Research/Education Center for Excellence in Molecular Sciences, Institute of Chemistry, Chinese Academy of Sciences, Beijing 100190, China – sequence: 3 givenname: Jiang-Yang surname: Shao fullname: Shao, Jiang-Yang email: shaojiangyang@iccas.ac.cn organization: Beijing National Laboratory for Molecular Sciences, CAS Research/Education Center for Excellence in Molecular Sciences, Institute of Chemistry, Chinese Academy of Sciences, Beijing 100190, China – sequence: 4 givenname: Yu-Duan surname: Wang fullname: Wang, Yu-Duan organization: Beijing National Laboratory for Molecular Sciences, CAS Research/Education Center for Excellence in Molecular Sciences, Institute of Chemistry, Chinese Academy of Sciences, Beijing 100190, China – sequence: 5 givenname: Jin-Song surname: Hu fullname: Hu, Jin-Song email: hujs@iccas.ac.cn organization: Beijing National Laboratory for Molecular Sciences, CAS Research/Education Center for Excellence in Molecular Sciences, Institute of Chemistry, Chinese Academy of Sciences, Beijing 100190, China – sequence: 6 givenname: Yu-Wu surname: Zhong fullname: Zhong, Yu-Wu email: zhongyuwu@iccas.ac organization: Beijing National Laboratory for Molecular Sciences, CAS Research/Education Center for Excellence in Molecular Sciences, Institute of Chemistry, Chinese Academy of Sciences, Beijing 100190, China |
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| Title | A sulfur-rich small molecule as a bifunctional interfacial layer for stable perovskite solar cells with efficiencies exceeding 22 |
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