An oxygen-sensitive cyclometalated platinum(II) complex with a triphenylamine modified acetylacetone derivative
[Display omitted] A cyclometalated Pt(II) complex [Pt(ppy)(TPA-dpa)] Pt2 with a triphenylamine (TPA) substituted diphenyl-1,3-propanedionate (dpa) as auxiliary ligand was designed and synthesized. The effects of the TPA moiety on the photophysical, electrochemical and oxygen sensing properties of th...
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| Published in | Tetrahedron letters Vol. 119; pp. 154427 - 154431 |
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| Main Authors | , , , |
| Format | Journal Article |
| Language | English |
| Published |
OXFORD
Elsevier Ltd
12.04.2023
Elsevier |
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| Online Access | Get full text |
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| Abstract | [Display omitted]
A cyclometalated Pt(II) complex [Pt(ppy)(TPA-dpa)] Pt2 with a triphenylamine (TPA) substituted diphenyl-1,3-propanedionate (dpa) as auxiliary ligand was designed and synthesized. The effects of the TPA moiety on the photophysical, electrochemical and oxygen sensing properties of the corresponding Pt(II) complex were systematically investigated compared with non-TPA-modified complexes [Pt(ppy)(dpa)] Pt1 and Pt(ppy)(acac). The maximum emission wavelength of Pt2 exhibits a notable redshift (71 nm) with respect to Pt(ppy)(acac). More importantly, the lifetime (25.52 µs) of Pt2 is significantly prolonged compared with those of Pt1 (0.32 µs) and Pt(ppy)(acac) (2.60 µs). Pt2 is highly sensitive to molecular oxygen when immobilized in an ethyl cellulose film. In addition, the oxygen sensing films have excellent reversibility during the quenching and recovering processes. |
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| AbstractList | [Display omitted]
A cyclometalated Pt(II) complex [Pt(ppy)(TPA-dpa)] Pt2 with a triphenylamine (TPA) substituted diphenyl-1,3-propanedionate (dpa) as auxiliary ligand was designed and synthesized. The effects of the TPA moiety on the photophysical, electrochemical and oxygen sensing properties of the corresponding Pt(II) complex were systematically investigated compared with non-TPA-modified complexes [Pt(ppy)(dpa)] Pt1 and Pt(ppy)(acac). The maximum emission wavelength of Pt2 exhibits a notable redshift (71 nm) with respect to Pt(ppy)(acac). More importantly, the lifetime (25.52 µs) of Pt2 is significantly prolonged compared with those of Pt1 (0.32 µs) and Pt(ppy)(acac) (2.60 µs). Pt2 is highly sensitive to molecular oxygen when immobilized in an ethyl cellulose film. In addition, the oxygen sensing films have excellent reversibility during the quenching and recovering processes. A cyclometalated Pt(II) complex [Pt(ppy)(TPA-dpa)] Pt2 with a triphenylamine (TPA) substituted diphe-nyl-1,3-propanedionate (dpa) as auxiliary ligand was designed and synthesized. The effects of the TPA moiety on the photophysical, electrochemical and oxygen sensing properties of the corresponding Pt (II) complex were systematically investigated compared with non-TPA-modified complexes [Pt(ppy) (dpa)] Pt1 and Pt(ppy)(acac). The maximum emission wavelength of Pt2 exhibits a notable redshift (71 nm) with respect to Pt(ppy)(acac). More importantly, the lifetime (25.52 mu s) of Pt2 is significantly prolonged compared with those of Pt1 (0.32 mu s) and Pt(ppy)(acac) (2.60 mu s). Pt2 is highly sensitive to molecular oxygen when immobilized in an ethyl cellulose film. In addition, the oxygen sensing films have excellent reversibility during the quenching and recovering processes.(c) 2023 Elsevier Ltd. All rights reserved. |
| ArticleNumber | 154427 |
| Author | Yan, Yingying Yu, Zhenni Wang, Junan Liu, Chun |
| Author_xml | – sequence: 1 givenname: Yingying surname: Yan fullname: Yan, Yingying – sequence: 2 givenname: Zhenni surname: Yu fullname: Yu, Zhenni – sequence: 3 givenname: Junan surname: Wang fullname: Wang, Junan – sequence: 4 givenname: Chun orcidid: 0000-0003-3521-8483 surname: Liu fullname: Liu, Chun email: cliu@dlut.edu.cn |
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| CitedBy_id | crossref_primary_10_1016_j_talanta_2023_125059 crossref_primary_10_1016_j_dyepig_2023_111719 crossref_primary_10_1016_j_cclet_2023_108819 |
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| Keywords | Optical sensor Reversibility Oxygen sensitivity Triphenylamine Cyclometalated platinum(II) complex DESIGN STATE PROPERTIES EMITTERS MOLECULAR-OXYGEN |
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A cyclometalated Pt(II) complex [Pt(ppy)(TPA-dpa)] Pt2 with a triphenylamine (TPA) substituted diphenyl-1,3-propanedionate (dpa) as auxiliary... A cyclometalated Pt(II) complex [Pt(ppy)(TPA-dpa)] Pt2 with a triphenylamine (TPA) substituted diphe-nyl-1,3-propanedionate (dpa) as auxiliary ligand was... |
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| SubjectTerms | Chemistry Chemistry, Organic Cyclometalated platinum(II) complex Optical sensor Oxygen sensitivity Physical Sciences Reversibility Science & Technology Triphenylamine |
| Title | An oxygen-sensitive cyclometalated platinum(II) complex with a triphenylamine modified acetylacetone derivative |
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