Construction of nanodiamonds/UiO-66-NH2 heterojunction for boosted visible-light photocatalytic degradation of antibiotics
•NDs/UiO-66-NH2 was prepared by a two-step route consisting of solvothermal and calcination;•Formation of NDs/UiO-66-NH2 heterojunction can enhance separation of photo-generated carriers;•NDs/UiO-66-NH2 exhibits the outstanding photocatalytic degradation activity of antibiotics. Photocatalytic degra...
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| Published in | Separation and purification technology Vol. 284; p. 120270 |
|---|---|
| Main Authors | , , , , , , , |
| Format | Journal Article |
| Language | English |
| Published |
Elsevier B.V
01.02.2022
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| Subjects | |
| Online Access | Get full text |
| ISSN | 1383-5866 1873-3794 |
| DOI | 10.1016/j.seppur.2021.120270 |
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| Abstract | •NDs/UiO-66-NH2 was prepared by a two-step route consisting of solvothermal and calcination;•Formation of NDs/UiO-66-NH2 heterojunction can enhance separation of photo-generated carriers;•NDs/UiO-66-NH2 exhibits the outstanding photocatalytic degradation activity of antibiotics.
Photocatalytic degradation of antibiotics is one of promising strategies to lessen environmental pollution and ecological damage. Pitifully, it is still challenging to achieve satisfactory photocatalytic degradation performance. Herein, nanodiamonds (NDs) coated on the surface of UiO-66-NH2 octahedrons to form NDs/UiO-66-NH2 heterojunction photocatalyst via a simple solvothermal method. The synthesized NDs/UiO-66-NH2 composite photocatalysts possess decent antibiotic degradation performance under visible light irradiation. Among all the composites, 3% NDs/UiO-66-NH2 composite exhibits the optimal degradation performance, which degraded more than 90% of TC pollutants within 120 min, 8.81 times higher than pristine UiO-66-NH2. The high photocatalytic performance of NDs/UiO-66-NH2 heterojunction is mainly attributed to the following three factors: (i) the introduction of NDs effectively increased the light absorption capacity of UiO-66-NH2; (ii) the Construction of heterojunction enhanced the separation efficiency of photogenerated carriers over UiO-66-NH2; (iii) The enriched functional groups of NDs could further promote the adsorption capacity of UiO-66-NH2. Our work broadens the application of NDs for the construction and synthesis of high-performance and stable semiconductor composite photocatalysts with visible light response in the area of environmental restoration. |
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| AbstractList | •NDs/UiO-66-NH2 was prepared by a two-step route consisting of solvothermal and calcination;•Formation of NDs/UiO-66-NH2 heterojunction can enhance separation of photo-generated carriers;•NDs/UiO-66-NH2 exhibits the outstanding photocatalytic degradation activity of antibiotics.
Photocatalytic degradation of antibiotics is one of promising strategies to lessen environmental pollution and ecological damage. Pitifully, it is still challenging to achieve satisfactory photocatalytic degradation performance. Herein, nanodiamonds (NDs) coated on the surface of UiO-66-NH2 octahedrons to form NDs/UiO-66-NH2 heterojunction photocatalyst via a simple solvothermal method. The synthesized NDs/UiO-66-NH2 composite photocatalysts possess decent antibiotic degradation performance under visible light irradiation. Among all the composites, 3% NDs/UiO-66-NH2 composite exhibits the optimal degradation performance, which degraded more than 90% of TC pollutants within 120 min, 8.81 times higher than pristine UiO-66-NH2. The high photocatalytic performance of NDs/UiO-66-NH2 heterojunction is mainly attributed to the following three factors: (i) the introduction of NDs effectively increased the light absorption capacity of UiO-66-NH2; (ii) the Construction of heterojunction enhanced the separation efficiency of photogenerated carriers over UiO-66-NH2; (iii) The enriched functional groups of NDs could further promote the adsorption capacity of UiO-66-NH2. Our work broadens the application of NDs for the construction and synthesis of high-performance and stable semiconductor composite photocatalysts with visible light response in the area of environmental restoration. |
| ArticleNumber | 120270 |
| Author | Shi, Weilong Sun, Haoran Pan, Jingjing Guo, Feng Xu, Zheng Shi, Yuxing Wang, Lijing Li, Lingling |
| Author_xml | – sequence: 1 givenname: Jingjing surname: Pan fullname: Pan, Jingjing organization: School of Energy and Power, Jiangsu University of Science and Technology, Zhenjiang, Jiangsu 212003, PR China – sequence: 2 givenname: Lijing surname: Wang fullname: Wang, Lijing organization: Henan Engineering Center of New Energy Battery Materials, Henan D&A Engineering Center of Advanced Battery Materials, College of Chemistry and Chemical Engineering, Institute of Architectural Engineering, Shangqiu Normal University, Shangqiu 476000, China – sequence: 3 givenname: Yuxing surname: Shi fullname: Shi, Yuxing organization: School of Energy and Power, Jiangsu University of Science and Technology, Zhenjiang, Jiangsu 212003, PR China – sequence: 4 givenname: Lingling surname: Li fullname: Li, Lingling organization: School of Energy and Power, Jiangsu University of Science and Technology, Zhenjiang, Jiangsu 212003, PR China – sequence: 5 givenname: Zheng surname: Xu fullname: Xu, Zheng organization: School of Energy and Power, Jiangsu University of Science and Technology, Zhenjiang, Jiangsu 212003, PR China – sequence: 6 givenname: Haoran surname: Sun fullname: Sun, Haoran organization: School of Energy and Power, Jiangsu University of Science and Technology, Zhenjiang, Jiangsu 212003, PR China – sequence: 7 givenname: Feng surname: Guo fullname: Guo, Feng email: gfeng0105@126.com organization: School of Energy and Power, Jiangsu University of Science and Technology, Zhenjiang, Jiangsu 212003, PR China – sequence: 8 givenname: Weilong surname: Shi fullname: Shi, Weilong email: shiwl@just.edu.cn organization: School of Material Science and Engineering, Jiangsu University of Science and Technology, Zhenjiang 212003, PR China |
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