Hydrogen oxidation reaction in alkaline media: From mechanism to recent electrocatalysts

The sluggish cathodic oxygen reduction reaction (ORR) of proton exchange membrane fuel cells (PEMFCs) heavily relies on the employment of a large quantity of unaffordable Pt-based electrocatalysts to accelerate the slow kinetics. As switching from acidic proton exchange membrane to alkaline hydroxid...

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Published inNano energy Vol. 44; pp. 288 - 303
Main Authors Cong, Yuanyuan, Yi, Baolian, Song, Yujiang
Format Journal Article
LanguageEnglish
Published Elsevier Ltd 01.02.2018
Subjects
Activity descriptors
Alkaline hydrogen oxidation reaction
Electrocatalysts
Hydroxide exchange membrane fuel cells
Mechanism
Hydroxide exchange membrane fuel cells
Alkaline hydrogen oxidation reaction
Electrocatalysts
Mechanism
Activity descriptors
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Abstract The sluggish cathodic oxygen reduction reaction (ORR) of proton exchange membrane fuel cells (PEMFCs) heavily relies on the employment of a large quantity of unaffordable Pt-based electrocatalysts to accelerate the slow kinetics. As switching from acidic proton exchange membrane to alkaline hydroxide one, it is highly promising to completely replace platinum group metal (PGM)-based ORR electrocatalysts with PGM-free counterparts. However, anodic hydrogen oxidation reaction (HOR), with a fast kinetics in PEMFCs even at a low Pt loading of 50μgPt cm−2 or less, becomes two orders of magnitude slower in alkaline media and thus requires a high loading of PGM-based electrocatalysts to accelerate the reaction rate. Alkaline HOR has drawn a great number of recent attentions, yet a comprehensive review is missing. Herein, this review covers diverse possible alkaline HOR mechanisms, hardly comparable electrocatalysts evaluation methods, two seemingly contradictive activity descriptors, as well as design and synthesis of PGM-based and PGM-free electrocatalysts with controlled structural parameters. Wherever is appropriate, this review describes our own point of view on certain subjects. Finally, future research directions are suggested. This review will provide knowledge and insights on fundamental and practical issues for the development of advanced alkaline HOR electrocatalysts and mechanism. Evaluation methods, reaction mechanism, activity descriptors, electrocatalysts, challenges and future directions of alkaline hydrogen oxidation reaction are reviewed. [Display omitted] •Typical evaluation methods of alkaline HOR electrocatalysts are introduced.•Rich alkaline HOR pathways and contradictive activity descriptors are collected.•Alkaline HOR electrocatalysts are reviewed and their performance is compared.•Challenges and future research directions of alkaline HOR field are discussed.
AbstractList The sluggish cathodic oxygen reduction reaction (ORR) of proton exchange membrane fuel cells (PEMFCs) heavily relies on the employment of a large quantity of unaffordable Pt-based electrocatalysts to accelerate the slow kinetics. As switching from acidic proton exchange membrane to alkaline hydroxide one, it is highly promising to completely replace platinum group metal (PGM)-based ORR electrocatalysts with PGM-free counterparts. However, anodic hydrogen oxidation reaction (HOR), with a fast kinetics in PEMFCs even at a low Pt loading of 50μgPt cm−2 or less, becomes two orders of magnitude slower in alkaline media and thus requires a high loading of PGM-based electrocatalysts to accelerate the reaction rate. Alkaline HOR has drawn a great number of recent attentions, yet a comprehensive review is missing. Herein, this review covers diverse possible alkaline HOR mechanisms, hardly comparable electrocatalysts evaluation methods, two seemingly contradictive activity descriptors, as well as design and synthesis of PGM-based and PGM-free electrocatalysts with controlled structural parameters. Wherever is appropriate, this review describes our own point of view on certain subjects. Finally, future research directions are suggested. This review will provide knowledge and insights on fundamental and practical issues for the development of advanced alkaline HOR electrocatalysts and mechanism. Evaluation methods, reaction mechanism, activity descriptors, electrocatalysts, challenges and future directions of alkaline hydrogen oxidation reaction are reviewed. [Display omitted] •Typical evaluation methods of alkaline HOR electrocatalysts are introduced.•Rich alkaline HOR pathways and contradictive activity descriptors are collected.•Alkaline HOR electrocatalysts are reviewed and their performance is compared.•Challenges and future research directions of alkaline HOR field are discussed.
Author Yi, Baolian
Song, Yujiang
Cong, Yuanyuan
Author_xml – sequence: 1
  givenname: Yuanyuan
  surname: Cong
  fullname: Cong, Yuanyuan
  organization: State Key Laboratory of Fine Chemicals, School of Chemical Engineering, Dalian University of Technology, 2 Linggong Road, Liaoning 116024, China
– sequence: 2
  givenname: Baolian
  surname: Yi
  fullname: Yi, Baolian
  organization: Dalian National Laboratories for Clean Energy, Dalian Institute of Chemical Physics, Chinese Academy of Sciences, Liaoning 116023, China
– sequence: 3
  givenname: Yujiang
  surname: Song
  fullname: Song, Yujiang
  email: yjsong@dlut.edu.cn
  organization: State Key Laboratory of Fine Chemicals, School of Chemical Engineering, Dalian University of Technology, 2 Linggong Road, Liaoning 116024, China
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Alkaline hydrogen oxidation reaction
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Snippet The sluggish cathodic oxygen reduction reaction (ORR) of proton exchange membrane fuel cells (PEMFCs) heavily relies on the employment of a large quantity of...
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Alkaline hydrogen oxidation reaction
Electrocatalysts
Hydroxide exchange membrane fuel cells
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Title Hydrogen oxidation reaction in alkaline media: From mechanism to recent electrocatalysts
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