“Superpermeability” and “pumping” of atomic hydrogen through palladium membranes
Permeation of atomic as well as molecular hydrogen through palladium membranes has been investigated experimentally in the temperature range from room temperature to 200 °C and at a higher incident flux of hydrogen atoms on palladium surface than in previous studies. The results demonstrate that phe...
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| Published in | Journal of membrane science Vol. 320; no. 1; pp. 528 - 532 |
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| Main Authors | , , , , , |
| Format | Journal Article |
| Language | English |
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Elsevier B.V
15.07.2008
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| Abstract | Permeation of atomic as well as molecular hydrogen through palladium membranes has been investigated experimentally in the temperature range from room temperature to 200
°C and at a higher incident flux of hydrogen atoms on palladium surface than in previous studies. The results demonstrate that phenomena of ‘superpermeability’ and ‘pumping’ of atomic gases through metal membranes are of a common nature. A theoretical model based on chemical thermodynamics and diffusion theory adequately describes the quantitative relationships observed in experiments. It was found that permeability of atomic hydrogen depends strongly on the magnitude of surface incident flux and membrane temperature. |
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| AbstractList | Permeation of atomic as well as molecular hydrogen through palladium membranes has been investigated experimentally in the temperature range from room temperature to 200
°C and at a higher incident flux of hydrogen atoms on palladium surface than in previous studies. The results demonstrate that phenomena of ‘superpermeability’ and ‘pumping’ of atomic gases through metal membranes are of a common nature. A theoretical model based on chemical thermodynamics and diffusion theory adequately describes the quantitative relationships observed in experiments. It was found that permeability of atomic hydrogen depends strongly on the magnitude of surface incident flux and membrane temperature. |
| Author | Vecher, A.A. Voropaev, A.G. Gusakov, A.G. Raspopov, S.A. Zheludkevich, M.L. Kozyrski, E.N. |
| Author_xml | – sequence: 1 givenname: M.L. surname: Zheludkevich fullname: Zheludkevich, M.L. email: mzheludkevich@ua.pt organization: Department of Chemistry, Belarus State University, 14 Leningradskaya Street, Minsk 220050, Belarus – sequence: 2 givenname: A.G. surname: Gusakov fullname: Gusakov, A.G. organization: Department of Chemistry, Belarus State University, 14 Leningradskaya Street, Minsk 220050, Belarus – sequence: 3 givenname: A.G. surname: Voropaev fullname: Voropaev, A.G. organization: Department of Chemistry, Belarus State University, 14 Leningradskaya Street, Minsk 220050, Belarus – sequence: 4 givenname: E.N. surname: Kozyrski fullname: Kozyrski, E.N. organization: Department of Chemistry, Belarus State University, 14 Leningradskaya Street, Minsk 220050, Belarus – sequence: 5 givenname: S.A. surname: Raspopov fullname: Raspopov, S.A. organization: Department of Chemistry, University of Waterloo, 200 University Avenue West, Waterloo, Ontario, N2L 3G1, Canada – sequence: 6 givenname: A.A. surname: Vecher fullname: Vecher, A.A. organization: Department of Chemistry, Belarus State University, 14 Leningradskaya Street, Minsk 220050, Belarus |
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| Cites_doi | 10.1016/S0022-3115(98)00094-4 10.1016/0022-3115(87)90273-X 10.1016/S0042-207X(79)80450-9 10.1016/j.fusengdes.2005.06.368 10.1016/S0920-3796(00)00332-X 10.1039/a905829j 10.1016/0022-3115(90)90329-L 10.1063/1.2804874 10.4028/www.scientific.net/MSF.76.195 10.1016/S0920-3796(03)00012-7 10.1016/0022-3115(94)00424-2 10.1016/0022-3115(87)90327-8 10.1039/a608475c 10.1016/S0022-3115(99)00243-3 10.1016/S0168-583X(01)00589-4 |
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| Keywords | Atomic hydrogen Thermodynamical model Superpermeability Palladium membrane Permeation |
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| Title | “Superpermeability” and “pumping” of atomic hydrogen through palladium membranes |
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