Co-gasification characteristics of Ca-rich sludge and Fe-rich sludge under CO2 atmosphere, and potential utilization of gasification residues as renewable catalyst in biomass pyrolysis
The co-gasification behaviors and performances of Ca-rich sludge (CS) and Fe-rich sludge (FS) were studied by thermogravimetric analyzer. The results showed that the comprehensive gasification index was highest at 40% CS ratio, which was 9.7 × 10−8 %2/(min2·°C3). The co-gasification resulted in more...
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| Published in | Renewable energy Vol. 224; p. 120118 |
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| Main Authors | , , , , , , , , |
| Format | Journal Article |
| Language | English |
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Elsevier Ltd
01.04.2024
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| Abstract | The co-gasification behaviors and performances of Ca-rich sludge (CS) and Fe-rich sludge (FS) were studied by thermogravimetric analyzer. The results showed that the comprehensive gasification index was highest at 40% CS ratio, which was 9.7 × 10−8 %2/(min2·°C3). The co-gasification resulted in more solid products generation due to that ash hindered contacts of gasifying agent and organics. By the sliding resistance furnace (SRF), in 80%CO2/20%N2, the evolution of gas compositions during the gasification process and impacts of different temperatures and blending ratios on co-gasification were evaluated. The evolution of gas compositions showed that the gas yields from CS gasification were higher than those from FS, and the interactions and ash catalytic effect during the co-gasification made the peak times earlier. The reaction temperatures and blending ratios had certain effects on the co-gasification process, affecting the mineral compositions and pores structures of sludge residues. Finally, considering the attributes of rich pores structure and Ca/Fe elements, the gasification residues can be used as ex-situ catalyst in the modification of biomass pyrolytic volatiles. Conducting the pyrolysis experiments by the SRF under N2 atmosphere, with adding gasification residues of sludge, the CO yield from biomass pyrolysis grew, but the yields of CO2, H2 and C2Hm reduced.
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| AbstractList | The co-gasification behaviors and performances of Ca-rich sludge (CS) and Fe-rich sludge (FS) were studied by thermogravimetric analyzer. The results showed that the comprehensive gasification index was highest at 40% CS ratio, which was 9.7 × 10−8 %2/(min2·°C3). The co-gasification resulted in more solid products generation due to that ash hindered contacts of gasifying agent and organics. By the sliding resistance furnace (SRF), in 80%CO2/20%N2, the evolution of gas compositions during the gasification process and impacts of different temperatures and blending ratios on co-gasification were evaluated. The evolution of gas compositions showed that the gas yields from CS gasification were higher than those from FS, and the interactions and ash catalytic effect during the co-gasification made the peak times earlier. The reaction temperatures and blending ratios had certain effects on the co-gasification process, affecting the mineral compositions and pores structures of sludge residues. Finally, considering the attributes of rich pores structure and Ca/Fe elements, the gasification residues can be used as ex-situ catalyst in the modification of biomass pyrolytic volatiles. Conducting the pyrolysis experiments by the SRF under N2 atmosphere, with adding gasification residues of sludge, the CO yield from biomass pyrolysis grew, but the yields of CO2, H2 and C2Hm reduced.
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| ArticleNumber | 120118 |
| Author | Liang, Hongxin Chen, Jianbiao Fang, Hua Wang, Fenfen Dai, Ying Zhu, Yuezhao Liu, Guojun Zhu, Jinjiao Tan, Jinzhu |
| Author_xml | – sequence: 1 givenname: Ying surname: Dai fullname: Dai, Ying organization: School of Mechanical and Power Engineering, Nanjing Tech University, Nanjing, 211816, Jiangsu, China – sequence: 2 givenname: Guojun surname: Liu fullname: Liu, Guojun organization: School of Energy Science and Engineering, Nanjing Tech University, Nanjing, 211816, Jiangsu, China – sequence: 3 givenname: Hongxin surname: Liang fullname: Liang, Hongxin organization: School of Energy Science and Engineering, Nanjing Tech University, Nanjing, 211816, Jiangsu, China – sequence: 4 givenname: Hua surname: Fang fullname: Fang, Hua organization: School of Energy Science and Engineering, Nanjing Tech University, Nanjing, 211816, Jiangsu, China – sequence: 5 givenname: Jianbiao orcidid: 0000-0002-9132-5817 surname: Chen fullname: Chen, Jianbiao email: jianbiaochen@njtech.edu.cn organization: School of Energy Science and Engineering, Nanjing Tech University, Nanjing, 211816, Jiangsu, China – sequence: 6 givenname: Fenfen surname: Wang fullname: Wang, Fenfen organization: School of Energy Science and Engineering, Nanjing Tech University, Nanjing, 211816, Jiangsu, China – sequence: 7 givenname: Jinjiao surname: Zhu fullname: Zhu, Jinjiao organization: School of Automotive Engineering, Yancheng Institute of Technology, Yancheng, 224051, Jiangsu, China – sequence: 8 givenname: Yuezhao surname: Zhu fullname: Zhu, Yuezhao organization: School of Energy Science and Engineering, Nanjing Tech University, Nanjing, 211816, Jiangsu, China – sequence: 9 givenname: Jinzhu surname: Tan fullname: Tan, Jinzhu organization: School of Mechanical and Power Engineering, Nanjing Tech University, Nanjing, 211816, Jiangsu, China |
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| Keywords | Gas composition Fe-rich sludge Ca-rich sludge Co-gasification Gasification residues |
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| SubjectTerms | Ca-rich sludge Co-gasification Fe-rich sludge Gas composition Gasification residues |
| Title | Co-gasification characteristics of Ca-rich sludge and Fe-rich sludge under CO2 atmosphere, and potential utilization of gasification residues as renewable catalyst in biomass pyrolysis |
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