Sr2GdF7:Tm3+/Yb3+ glass ceramic: A highly sensitive optical thermometer based on FIR technique
In this work, we present a highly sensitive optical thermometer, Tm3+/Yb3+ co-doped Sr2GdF7 transparent oxyfluoride glass ceramic (GC). Sr2GdF7:Tm3+/Yb3+ GC was synthesized by traditional melt-quenching method with further crystallization process. Its structural and optical properties were systemati...
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| Published in | Journal of alloys and compounds Vol. 735; pp. 2544 - 2550 |
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| Main Authors | , , , , , |
| Format | Journal Article |
| Language | English |
| Published |
Elsevier B.V
25.02.2018
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| Subjects | |
| Online Access | Get full text |
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| Abstract | In this work, we present a highly sensitive optical thermometer, Tm3+/Yb3+ co-doped Sr2GdF7 transparent oxyfluoride glass ceramic (GC). Sr2GdF7:Tm3+/Yb3+ GC was synthesized by traditional melt-quenching method with further crystallization process. Its structural and optical properties were systematically investigated by a series of characterization methods. The enrichment of Tm3+ into Sr2GdF7 lattice is confirmed by enhanced emission intensities, obvious Stark splitting and prolonged lifetimes of Tm3+ after crystallization. Based on fluorescence intensity ratio (FIR) of 3F3 → 3H6 and 1G4 → 3F4 transitions of Tm3+, the temperature thermometric properties of Sr2GdF7:Tm3+ GC were explored. Interestingly, maximum relative sensitivity SR-max reaches 1.97% K−1 at 353 K and the absolute sensitivity SA keeps increasing with temperature up to 3.90% K−1 at 563 K. Our investigation demonstrates that Sr2GdF7:Tm3+/Yb3+ GC may act as promising candidate for optical temperature sensor.
•Transparent Sr2GdF7:Tm3+/Yb3+ glass ceramic (GC) was successfully fabricated.•Up-conversion of Sr2GdF7:Tm3+/Yb3+ GC is high enhanced compared to that of PG.•Sr2GdF7:Tm3+/Yb3+ GC present large energy gap (2207 cm−1) and high relative sensitivity (SR-max reaches 1.97%K−1 at 353 K).•Sr2GdF7:Tm3+/Yb3+ GC may find application in FIR-based temperature sensors. |
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| AbstractList | In this work, we present a highly sensitive optical thermometer, Tm3+/Yb3+ co-doped Sr2GdF7 transparent oxyfluoride glass ceramic (GC). Sr2GdF7:Tm3+/Yb3+ GC was synthesized by traditional melt-quenching method with further crystallization process. Its structural and optical properties were systematically investigated by a series of characterization methods. The enrichment of Tm3+ into Sr2GdF7 lattice is confirmed by enhanced emission intensities, obvious Stark splitting and prolonged lifetimes of Tm3+ after crystallization. Based on fluorescence intensity ratio (FIR) of 3F3 → 3H6 and 1G4 → 3F4 transitions of Tm3+, the temperature thermometric properties of Sr2GdF7:Tm3+ GC were explored. Interestingly, maximum relative sensitivity SR-max reaches 1.97% K−1 at 353 K and the absolute sensitivity SA keeps increasing with temperature up to 3.90% K−1 at 563 K. Our investigation demonstrates that Sr2GdF7:Tm3+/Yb3+ GC may act as promising candidate for optical temperature sensor.
•Transparent Sr2GdF7:Tm3+/Yb3+ glass ceramic (GC) was successfully fabricated.•Up-conversion of Sr2GdF7:Tm3+/Yb3+ GC is high enhanced compared to that of PG.•Sr2GdF7:Tm3+/Yb3+ GC present large energy gap (2207 cm−1) and high relative sensitivity (SR-max reaches 1.97%K−1 at 353 K).•Sr2GdF7:Tm3+/Yb3+ GC may find application in FIR-based temperature sensors. |
| Author | Chen, LiPing Guo, Hai Hu, FangFang Cao, JiangKun Wei, RongFei Chen, WeiPing |
| Author_xml | – sequence: 1 givenname: WeiPing surname: Chen fullname: Chen, WeiPing – sequence: 2 givenname: JiangKun surname: Cao fullname: Cao, JiangKun – sequence: 3 givenname: FangFang surname: Hu fullname: Hu, FangFang – sequence: 4 givenname: RongFei surname: Wei fullname: Wei, RongFei – sequence: 5 givenname: LiPing surname: Chen fullname: Chen, LiPing – sequence: 6 givenname: Hai surname: Guo fullname: Guo, Hai email: ghh@zjnu.cn |
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| Snippet | In this work, we present a highly sensitive optical thermometer, Tm3+/Yb3+ co-doped Sr2GdF7 transparent oxyfluoride glass ceramic (GC). Sr2GdF7:Tm3+/Yb3+ GC... |
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| SubjectTerms | Glass ceramic Optical thermometry Sr2GdF7:Tm3+/Yb3 Up-conversion |
| Title | Sr2GdF7:Tm3+/Yb3+ glass ceramic: A highly sensitive optical thermometer based on FIR technique |
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