Symmetry effect on the mechanism of the optical absorption of phosphorene quantum dots
Based on a rectangular phosphorene quantum dot (PQD) we perform a systematical investigation into the mechanism of the optical absorption of the PQD. It is found that it is the symmetries of the related initial and final states of the PQD, together with the symmetry of the PQD structure, that determ...
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| Published in | Physica. E, Low-dimensional systems & nanostructures Vol. 107; pp. 137 - 141 |
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| Main Authors | , , , , |
| Format | Journal Article |
| Language | English |
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Elsevier B.V
01.03.2019
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| Abstract | Based on a rectangular phosphorene quantum dot (PQD) we perform a systematical investigation into the mechanism of the optical absorption of the PQD. It is found that it is the symmetries of the related initial and final states of the PQD, together with the symmetry of the PQD structure, that determines whether the optical absorption can occur, as well as the absorption strength. More fundamentally speaking, the optical absorption spectra are determined by the symmetry of the confined PQD structure, the symmetry of phosphorene, and the chemical property of phosphorus atoms. The universality of the above conclusion is further verified in other three typical PQDs of different symmetries including the triangular, romboidal, and hexagonal PQDs. We want to emphasize that our conclusion should be also applicable in understanding the optical absorption of the quantum dots formed in other materials. |
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| AbstractList | Based on a rectangular phosphorene quantum dot (PQD) we perform a systematical investigation into the mechanism of the optical absorption of the PQD. It is found that it is the symmetries of the related initial and final states of the PQD, together with the symmetry of the PQD structure, that determines whether the optical absorption can occur, as well as the absorption strength. More fundamentally speaking, the optical absorption spectra are determined by the symmetry of the confined PQD structure, the symmetry of phosphorene, and the chemical property of phosphorus atoms. The universality of the above conclusion is further verified in other three typical PQDs of different symmetries including the triangular, romboidal, and hexagonal PQDs. We want to emphasize that our conclusion should be also applicable in understanding the optical absorption of the quantum dots formed in other materials. |
| Author | Liang, F.X. Jiang, Z.T. Ren, Y.H. Lv, Z.T. Han, Q.Z. |
| Author_xml | – sequence: 1 givenname: Z.T. surname: Jiang fullname: Jiang, Z.T. email: jiangzhaotan@hotmail.com organization: School of Physics, Beijing Institute of Technology, Beijing, 100081, China – sequence: 2 givenname: F.X. surname: Liang fullname: Liang, F.X. email: liangfeixia@hotmail.com organization: School of Physics, Beijing Institute of Technology, Beijing, 100081, China – sequence: 3 givenname: Z.T. surname: Lv fullname: Lv, Z.T. organization: School of Physics, Beijing Institute of Technology, Beijing, 100081, China – sequence: 4 givenname: Y.H. surname: Ren fullname: Ren, Y.H. organization: School of Physics, Beijing Institute of Technology, Beijing, 100081, China – sequence: 5 givenname: Q.Z. surname: Han fullname: Han, Q.Z. organization: State Key Laboratory of Multiphase Complex System, Institute of Process Engineering, Chinese Academy of Sciences, Beijing, 100190, China |
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| Cites_doi | 10.1021/ar5002846 10.1016/j.physe.2007.06.020 10.1038/nnano.2014.35 10.1021/acssensors.7b00102 10.1021/nl301702r 10.1021/acs.jpclett.5b02457 10.1088/0957-4484/27/6/065708 10.1038/srep42357 10.1063/1.2407388 10.1103/PhysRevB.89.201408 10.1038/ncomms7647 10.1002/adom.201700257 10.1063/1.4955222 10.1021/nn502362b 10.1002/adma.201103411 10.1038/srep27307 10.1021/acs.nanolett.5b04593 10.1021/nl200631m 10.1039/C7MH00543A 10.1038/nnano.2012.193 10.1016/j.mseb.2017.03.011 10.1021/acs.jpclett.5b01686 10.1103/PhysRevLett.99.216802 10.1021/nn5052376 10.1063/1.4803920 10.1038/ncomms5475 10.1016/j.cplett.2017.07.033 10.1002/advs.201600435 10.1002/anie.201409400 |
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| Snippet | Based on a rectangular phosphorene quantum dot (PQD) we perform a systematical investigation into the mechanism of the optical absorption of the PQD. It is... |
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