Semi-transparent perovskite solar cells with directly sputtered amorphous InZnSnO top cathodes for building integrated photovoltaics
We report on a low plasma damage sputtering amorphous InZnSnO (IZTO) top cathode prepared using linear facing target sputtering (LFTS) at room temperature for semi-transparent perovskite solar cells (PSCs) to be applied as building integrated photovoltaics. The effective confinement of high-density...
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Published in | Organic electronics Vol. 78; p. 105560 |
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Main Authors | , , , , , |
Format | Journal Article |
Language | English |
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Elsevier B.V
01.03.2020
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Abstract | We report on a low plasma damage sputtering amorphous InZnSnO (IZTO) top cathode prepared using linear facing target sputtering (LFTS) at room temperature for semi-transparent perovskite solar cells (PSCs) to be applied as building integrated photovoltaics. The effective confinement of high-density plasma between InZnO and InSnO targets by directional magnet fields and negative bias applied simultaneously on both targets led to the successful sputtering of the amorphous IZTO top cathode on the semi-transparent PSCs without plasma damage or degradation of PSC performance. At an optimal sputtering condition of the IZTO top cathode, the semi-transparent PSC showed an open circuit voltage (1.056 V), short circuit current (16.79 mA/cm2), fill factor (51.19%), and power conversion efficiency (9.081%) comparable to those of reference PSC with an Ag metal top cathode. Based on synchrotron GIWAXS and high-resolution transmission electron microscopy examinations, we suggested a possible mechanism with which to explain the plasma damage effect on the performance of PCSs while sputtering IZTO top cathode on semi-transparent PSCs.
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•Semi-transparent perovskite solar cells with sputtered IZTO top cathodes.•Plasma damage free sputtering of IZTO top cathode on perovskite solar cells using a linear facing target sputtering.•Semi-transparent perovskite solar cells for building integrated photovoltaics.•Plasma damage mechanism of perovskite solar cells during sputtering. |
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AbstractList | We report on a low plasma damage sputtering amorphous InZnSnO (IZTO) top cathode prepared using linear facing target sputtering (LFTS) at room temperature for semi-transparent perovskite solar cells (PSCs) to be applied as building integrated photovoltaics. The effective confinement of high-density plasma between InZnO and InSnO targets by directional magnet fields and negative bias applied simultaneously on both targets led to the successful sputtering of the amorphous IZTO top cathode on the semi-transparent PSCs without plasma damage or degradation of PSC performance. At an optimal sputtering condition of the IZTO top cathode, the semi-transparent PSC showed an open circuit voltage (1.056 V), short circuit current (16.79 mA/cm2), fill factor (51.19%), and power conversion efficiency (9.081%) comparable to those of reference PSC with an Ag metal top cathode. Based on synchrotron GIWAXS and high-resolution transmission electron microscopy examinations, we suggested a possible mechanism with which to explain the plasma damage effect on the performance of PCSs while sputtering IZTO top cathode on semi-transparent PSCs.
[Display omitted]
•Semi-transparent perovskite solar cells with sputtered IZTO top cathodes.•Plasma damage free sputtering of IZTO top cathode on perovskite solar cells using a linear facing target sputtering.•Semi-transparent perovskite solar cells for building integrated photovoltaics.•Plasma damage mechanism of perovskite solar cells during sputtering. |
ArticleNumber | 105560 |
Author | Lee, Jae-Hoon Kim, Yunseok Na, Seok-In Lee, Hyun Hwi Kim, Han-Ki Kim, Jae-Gyeong |
Author_xml | – sequence: 1 givenname: Jae-Gyeong surname: Kim fullname: Kim, Jae-Gyeong organization: School of Advanced Materials Science & Engineering, Sungkyunkwan University, 2066 Seobu-ro, Jangan-gu, Suwon, Gyeonggi-do, 440-746, Republic of Korea – sequence: 2 givenname: Jae-Hoon surname: Lee fullname: Lee, Jae-Hoon organization: School of Advanced Materials Science & Engineering, Sungkyunkwan University, 2066 Seobu-ro, Jangan-gu, Suwon, Gyeonggi-do, 440-746, Republic of Korea – sequence: 3 givenname: Seok-In surname: Na fullname: Na, Seok-In organization: Professional Graduate School of Flexible and Printable Electronics and Polymer Materials Fusion Research Center, Chonbuk National University, Deokjin-dong 664-14, Jeonju-si, Jeollabuk-do, 561-756, Republic of Korea – sequence: 4 givenname: Hyun Hwi surname: Lee fullname: Lee, Hyun Hwi organization: Pohang Accelerator Laboratory, POSTECH, Pohang, 790-784, Republic of Korea – sequence: 5 givenname: Yunseok surname: Kim fullname: Kim, Yunseok organization: School of Advanced Materials Science & Engineering, Sungkyunkwan University, 2066 Seobu-ro, Jangan-gu, Suwon, Gyeonggi-do, 440-746, Republic of Korea – sequence: 6 givenname: Han-Ki orcidid: 0000-0003-4650-6245 surname: Kim fullname: Kim, Han-Ki email: hankikim@skku.edu organization: School of Advanced Materials Science & Engineering, Sungkyunkwan University, 2066 Seobu-ro, Jangan-gu, Suwon, Gyeonggi-do, 440-746, Republic of Korea |
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Keywords | InZnSnO Top cathode Linear facing target sputtering Low plasma damage Semi-transparent perovskite solar cells |
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Snippet | We report on a low plasma damage sputtering amorphous InZnSnO (IZTO) top cathode prepared using linear facing target sputtering (LFTS) at room temperature for... |
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SubjectTerms | InZnSnO Linear facing target sputtering Low plasma damage Semi-transparent perovskite solar cells Top cathode |
Title | Semi-transparent perovskite solar cells with directly sputtered amorphous InZnSnO top cathodes for building integrated photovoltaics |
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