Progress on hydrogen sulfide removal: From catalytic oxidation to plasma-assisted treatment
Air pollution is a long-standing environmental challenge as well an important economic subject. Hydrogen sulfide is one the major pollutants in the industrial releases. This review focuses on the thermochemical treatment of hydrogen sulfide based on the most recent works to date regarding its remova...
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| Published in | Chemosphere (Oxford) Vol. 364; p. 143174 |
|---|---|
| Main Authors | , , , , , |
| Format | Journal Article |
| Language | English |
| Published |
England
Elsevier Ltd
01.09.2024
Elsevier |
| Subjects | |
| Online Access | Get full text |
| ISSN | 0045-6535 1879-1298 1879-1298 |
| DOI | 10.1016/j.chemosphere.2024.143174 |
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| Abstract | Air pollution is a long-standing environmental challenge as well an important economic subject. Hydrogen sulfide is one the major pollutants in the industrial releases. This review focuses on the thermochemical treatment of hydrogen sulfide based on the most recent works to date regarding its removal. By analyzing fundamental steps in chemical reaction engineering, some useful factors are emphasized since they are often neglected in scientific studies, catalysts design and process scale-up. From processing side, the fluid flow conditions including velocity, H2S concentration, relative humidity, temperature and pressure strongly influence the kinetic behavior and so the catalytic performance of the H2S removal reactor. From material side, the catalyst properties including nature, porosity, pore types, size, sites distribution and layer structuration largely influence the removal performance via among others the accessibility to catalytic sites, pores connection and mass transfer resistance. Plasma-assisted catalytic removal of H2S combines many novelties in comparison with a classical thermo-catalytic process. From patents review, we can see that main concerns are about electrodes mounting, reactor lifetime and modular design to solve the problems in the industrial practice. We attempt to provide for scientists, engineers and industrialists a guidance on the design of catalysts and processes for H2S removal which could be applied in laboratorial studies and industrial processes as well.
[Display omitted]
•Thermo-catalytic oxidation of H2S and their latest progress.•The influence of fluid's flow on kinetic behaviour and catalytic performance.•Porous characteristics and layer structure largely influence H2S removal.•Plasma technologies became attractive for high-efficient H2S abatement.•Modular design and electrodes mounting are the keys to industrial problems. |
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| AbstractList | Air pollution is a long-standing environmental challenge as well an important economic subject. Hydrogen sulfide is one the major pollutants in the industrial releases. This review focuses on the thermochemical treatment of hydrogen sulfide based on the most recent works to date regarding its removal. By analyzing fundamental steps in chemical reaction engineering, some useful factors are emphasized since they are often neglected in scientific studies, catalysts design and process scale-up. From processing side, the fluid flow conditions including velocity, H
S concentration, relative humidity, temperature and pressure strongly influence the kinetic behavior and so the catalytic performance of the H
S removal reactor. From material side, the catalyst properties including nature, porosity, pore types, size, sites distribution and layer structuration largely influence the removal performance via among others the accessibility to catalytic sites, pores connection and mass transfer resistance. Plasma-assisted catalytic removal of H
S combines many novelties in comparison with a classical thermo-catalytic process. From patents review, we can see that main concerns are about electrodes mounting, reactor lifetime and modular design to solve the problems in the industrial practice. We attempt to provide for scientists, engineers and industrialists a guidance on the design of catalysts and processes for H
S removal which could be applied in laboratorial studies and industrial processes as well. Air pollution is a long-standing environmental challenge as well an important economic subject. Hydrogen sulfide is one the major pollutants in the industrial releases. This review focuses on the thermochemical treatment of hydrogen sulfide based on the most recent works to date regarding its removal. By analyzing fundamental steps in chemical reaction engineering, some useful factors are emphasized since they are often neglected in scientific studies, catalysts design and process scale-up. From processing side, the fluid flow conditions including velocity, H2S concentration, relative humidity, temperature and pressure strongly influence the kinetic behavior and so the catalytic performance of the H2S removal reactor. From material side, the catalyst properties including nature, porosity, pore types, size, sites distribution and layer structuration largely influence the removal performance via among others the accessibility to catalytic sites, pores connection and mass transfer resistance. Plasma-assisted catalytic removal of H2S combines many novelties in comparison with a classical thermo-catalytic process. From patents review, we can see that main concerns are about electrodes mounting, reactor lifetime and modular design to solve the problems in the industrial practice. We attempt to provide for scientists, engineers and industrialists a guidance on the design of catalysts and processes for H2S removal which could be applied in laboratorial studies and industrial processes as well. Air pollution is a long-standing environmental challenge as well an important economic subject. Hydrogen sulfide is one the major pollutants in the industrial releases. This review focuses on the thermochemical treatment of hydrogen sulfide based on the most recent works to date regarding its removal. By analyzing fundamental steps in chemical reaction engineering, some useful factors are emphasized since they are often neglected in scientific studies, catalysts design and process scale-up. From processing side, the fluid flow conditions including velocity, H2S concentration, relative humidity, temperature and pressure strongly influence the kinetic behavior and so the catalytic performance of the H2S removal reactor. From material side, the catalyst properties including nature, porosity, pore types, size, sites distribution and layer structuration largely influence the removal performance via among others the accessibility to catalytic sites, pores connection and mass transfer resistance. Plasma-assisted catalytic removal of H2S combines many novelties in comparison with a classical thermo-catalytic process. From patents review, we can see that main concerns are about electrodes mounting, reactor lifetime and modular design to solve the problems in the industrial practice. We attempt to provide for scientists, engineers and industrialists a guidance on the design of catalysts and processes for H2S removal which could be applied in laboratorial studies and industrial processes as well.Air pollution is a long-standing environmental challenge as well an important economic subject. Hydrogen sulfide is one the major pollutants in the industrial releases. This review focuses on the thermochemical treatment of hydrogen sulfide based on the most recent works to date regarding its removal. By analyzing fundamental steps in chemical reaction engineering, some useful factors are emphasized since they are often neglected in scientific studies, catalysts design and process scale-up. From processing side, the fluid flow conditions including velocity, H2S concentration, relative humidity, temperature and pressure strongly influence the kinetic behavior and so the catalytic performance of the H2S removal reactor. From material side, the catalyst properties including nature, porosity, pore types, size, sites distribution and layer structuration largely influence the removal performance via among others the accessibility to catalytic sites, pores connection and mass transfer resistance. Plasma-assisted catalytic removal of H2S combines many novelties in comparison with a classical thermo-catalytic process. From patents review, we can see that main concerns are about electrodes mounting, reactor lifetime and modular design to solve the problems in the industrial practice. We attempt to provide for scientists, engineers and industrialists a guidance on the design of catalysts and processes for H2S removal which could be applied in laboratorial studies and industrial processes as well. Air pollution is a long-standing environmental challenge as well an important economic subject. Hydrogen sulfide is one the major pollutants in the industrial releases. This review focuses on the thermochemical treatment of hydrogen sulfide based on the most recent works to date regarding its removal. By analyzing fundamental steps in chemical reaction engineering, some useful factors are emphasized since they are often neglected in scientific studies, catalysts design and process scale-up. From processing side, the fluid flow conditions including velocity, H₂S concentration, relative humidity, temperature and pressure strongly influence the kinetic behavior and so the catalytic performance of the H₂S removal reactor. From material side, the catalyst properties including nature, porosity, pore types, size, sites distribution and layer structuration largely influence the removal performance via among others the accessibility to catalytic sites, pores connection and mass transfer resistance. Plasma-assisted catalytic removal of H₂S combines many novelties in comparison with a classical thermo-catalytic process. From patents review, we can see that main concerns are about electrodes mounting, reactor lifetime and modular design to solve the problems in the industrial practice. We attempt to provide for scientists, engineers and industrialists a guidance on the design of catalysts and processes for H₂S removal which could be applied in laboratorial studies and industrial processes as well. Air pollution is a long-standing environmental challenge as well an important economic subject. Hydrogen sulfide is one the major pollutants in the industrial releases. This review focuses on the thermochemical treatment of hydrogen sulfide based on the most recent works to date regarding its removal. By analyzing fundamental steps in chemical reaction engineering, some useful factors are emphasized since they are often neglected in scientific studies, catalysts design and process scale-up. From processing side, the fluid flow conditions including velocity, H2S concentration, relative humidity, temperature and pressure strongly influence the kinetic behavior and so the catalytic performance of the H2S removal reactor. From material side, the catalyst properties including nature, porosity, pore types, size, sites distribution and layer structuration largely influence the removal performance via among others the accessibility to catalytic sites, pores connection and mass transfer resistance. Plasma-assisted catalytic removal of H2S combines many novelties in comparison with a classical thermo-catalytic process. From patents review, we can see that main concerns are about electrodes mounting, reactor lifetime and modular design to solve the problems in the industrial practice. We attempt to provide for scientists, engineers and industrialists a guidance on the design of catalysts and processes for H2S removal which could be applied in laboratorial studies and industrial processes as well. [Display omitted] •Thermo-catalytic oxidation of H2S and their latest progress.•The influence of fluid's flow on kinetic behaviour and catalytic performance.•Porous characteristics and layer structure largely influence H2S removal.•Plasma technologies became attractive for high-efficient H2S abatement.•Modular design and electrodes mounting are the keys to industrial problems. |
| ArticleNumber | 143174 |
| Author | Fulcheri, Laurent Rohani, Vandad Leroux, Patrick Nastasi, Valerie Wang, Shengfei Gracian, Catherine |
| Author_xml | – sequence: 1 givenname: Shengfei surname: Wang fullname: Wang, Shengfei email: shengfei.wang@minesparis.psl.eu organization: Mines Paris, Université PSL, Centre Procédés Energies Renouvelables et Systèmes Energétiques (PERSEE), 06904, Sophia Antipolis, France – sequence: 2 givenname: Vandad surname: Rohani fullname: Rohani, Vandad email: vandad-julien.rohani@minesparis.psl.eu organization: Mines Paris, Université PSL, Centre Procédés Energies Renouvelables et Systèmes Energétiques (PERSEE), 06904, Sophia Antipolis, France – sequence: 3 givenname: Patrick surname: Leroux fullname: Leroux, Patrick email: patrick.leroux@minesparis.psl.eu organization: Mines Paris, Université PSL, Centre Procédés Energies Renouvelables et Systèmes Energétiques (PERSEE), 06904, Sophia Antipolis, France – sequence: 4 givenname: Catherine surname: Gracian fullname: Gracian, Catherine email: catherine.gracian@suez.com organization: Suez International, Tour CB21, 16 Place de l’Iris, 92040, Paris La Défense, France – sequence: 5 givenname: Valerie surname: Nastasi fullname: Nastasi, Valerie email: valerie.nastasi@suez.com organization: Suez International, Tour CB21, 16 Place de l’Iris, 92040, Paris La Défense, France – sequence: 6 givenname: Laurent surname: Fulcheri fullname: Fulcheri, Laurent email: laurent.fulcheri@minesparis.psl.eu organization: Mines Paris, Université PSL, Centre Procédés Energies Renouvelables et Systèmes Energétiques (PERSEE), 06904, Sophia Antipolis, France |
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| Keywords | H2S Industrial practice Catalytic oxidation Non-thermal plasma Mass transfer Scale-up HS |
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| SubjectTerms | air pollution catalysts catalytic activity Catalytic oxidation Engineering Sciences H2S hydrogen sulfide Industrial practice Mass transfer Non-thermal plasma oxidation porosity relative humidity Scale-up temperature |
| Title | Progress on hydrogen sulfide removal: From catalytic oxidation to plasma-assisted treatment |
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