Magnetic properties and large reversible magnetocaloric effect in TmMn2Si2
•Magnetic and magnetocaloric properties in TmMn2Si2 were studied.•A large reversible magnetocaloric effect in TmMn2Si2 was observed.•TmMn2Si2 could be a candidate for low temperature magnetic refrigeration. The magnetic properties and magnetocaloric effect (MCE) in the ternary intermetallic compound...
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| Published in | Journal of alloys and compounds Vol. 582; pp. 670 - 673 |
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| Main Authors | , , , , |
| Format | Journal Article |
| Language | English |
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Kidlington
Elsevier B.V
05.01.2014
Elsevier |
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| Abstract | •Magnetic and magnetocaloric properties in TmMn2Si2 were studied.•A large reversible magnetocaloric effect in TmMn2Si2 was observed.•TmMn2Si2 could be a candidate for low temperature magnetic refrigeration.
The magnetic properties and magnetocaloric effect (MCE) in the ternary intermetallic compound TmMn2Si2 have been studied via magnetization and heat capacity measurements. A large reversible MCE has been observed in TmMn2Si2 accompanied by a second order magnetic phase transition from paramagnetic to ferromagnetic at ∼5.5K. Under a field change of 5T, the maximum values of magnetic entropy change (-ΔSMmax) and adiabatic temperature change (ΔTadmax) are 22.7J/kgK and 10.1K, respectively, the corresponding relative cooling power (RCP) is 250J/kg. The large magnetic entropy change together with the absence of thermal and field hysteresis makes the TmMn2Si2 compound could be a good candidate for low temperature magnetic refrigeration. |
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| AbstractList | The magnetic properties and magnetocaloric effect (MCE) in the ternary intermetallic compound TmMn2Si2 have been studied via magnetization and heat capacity measurements. A large reversible MCE has been observed in TmMn2Si2 accompanied by a second order magnetic phase transition from paramagnetic to ferromagnetic at similar to 5.5 K. Under a field change of 5 T, the maximum values of magnetic entropy change (- Delta SMmax) and adiabatic temperature change ( Delta Tadmax) are 22.7 J/kg K and 10.1 K, respectively, the corresponding relative cooling power (RCP) is 250 J/kg. The large magnetic entropy change together with the absence of thermal and field hysteresis makes the TmMn2Si2 compound could be a good candidate for low temperature magnetic refrigeration. •Magnetic and magnetocaloric properties in TmMn2Si2 were studied.•A large reversible magnetocaloric effect in TmMn2Si2 was observed.•TmMn2Si2 could be a candidate for low temperature magnetic refrigeration. The magnetic properties and magnetocaloric effect (MCE) in the ternary intermetallic compound TmMn2Si2 have been studied via magnetization and heat capacity measurements. A large reversible MCE has been observed in TmMn2Si2 accompanied by a second order magnetic phase transition from paramagnetic to ferromagnetic at ∼5.5K. Under a field change of 5T, the maximum values of magnetic entropy change (-ΔSMmax) and adiabatic temperature change (ΔTadmax) are 22.7J/kgK and 10.1K, respectively, the corresponding relative cooling power (RCP) is 250J/kg. The large magnetic entropy change together with the absence of thermal and field hysteresis makes the TmMn2Si2 compound could be a good candidate for low temperature magnetic refrigeration. |
| Author | Saensunon, Banchachit Huo, Dexuan Li, Lingwei Nishimura, Katsuhiko Hutchison, Wayne D. |
| Author_xml | – sequence: 1 givenname: Lingwei surname: Li fullname: Li, Lingwei email: wei0396@hotmail.com organization: Institute of Materials Physics, Hangzhou Dianzi University, Hangzhou 310018, China – sequence: 2 givenname: Banchachit surname: Saensunon fullname: Saensunon, Banchachit organization: School of Physical, Environmental & Mathematical Sciences, The University of New South Wales, Canberra, ACT 2610, Australia – sequence: 3 givenname: Wayne D. surname: Hutchison fullname: Hutchison, Wayne D. organization: School of Physical, Environmental & Mathematical Sciences, The University of New South Wales, Canberra, ACT 2610, Australia – sequence: 4 givenname: Dexuan surname: Huo fullname: Huo, Dexuan organization: Institute of Materials Physics, Hangzhou Dianzi University, Hangzhou 310018, China – sequence: 5 givenname: Katsuhiko surname: Nishimura fullname: Nishimura, Katsuhiko organization: Graduate School of Science and Engineering, University of Toyama, Toyama 930-8555, Japan |
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| Cites_doi | 10.1063/1.4752738 10.1063/1.4704155 10.1088/0034-4885/68/6/R04 10.1103/PhysRevLett.110.217211 10.1063/1.4804576 10.1016/j.jmmm.2012.08.007 10.1103/PhysRevB.63.174440 10.1038/nmat3334 10.1016/0031-9163(64)91158-8 10.1016/S0022-0248(02)01689-5 10.1063/1.2798594 10.1016/j.jallcom.2013.03.109 10.1016/j.ijrefrig.2009.11.005 10.1016/j.jallcom.2013.04.081 10.1016/j.scriptamat.2012.04.037 10.1063/1.3526380 10.1016/j.jallcom.2012.01.156 10.1063/1.3518556 10.1063/1.3599456 10.1063/1.4709761 10.1002/adma.201002180 10.1016/j.jallcom.2013.03.185 |
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| Keywords | RMn2Si2 compounds Magnetocaloric effect Magnetic phase transition Active magnetic refrigeration materials Reversible processes Magnetization Intermetallic compounds Magnetic transitions Magnetic refrigerators Specific heat Silicon alloys RMn Magnetocaloric effects Si Manganese alloys Thulium alloys Rare earth alloys compounds Ferromagnetic-paramagnetic transitions Transition element alloys |
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| SubjectTerms | Active magnetic refrigeration materials Alloys Condensed matter: electronic structure, electrical, magnetic, and optical properties Entropy Exact sciences and technology Ferromagnetism Heat capacity Hysteresis Magnetic phase transition Magnetic properties Magnetic properties and materials Magnetically ordered materials: other intrinsic properties Magnetization Magnetocaloric effect Magnetocaloric effect, magnetic cooling Physics Refrigeration RMn2Si2 compounds |
| Title | Magnetic properties and large reversible magnetocaloric effect in TmMn2Si2 |
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