Spatially Resolved Contact Pressure and Contact Resistance Measurements at the Gas Diffusion Layer: A Tool for PEM Fuel Cell Development
A device and a method for direct measurement of the local contact pressures of gas diffusion layers (GDL) are presented. The new tool determines the spatially resolved contact pressure on the GDL side opposite to the flow-field/GDL interface which is relevant to good electrical contact between the G...
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Published in | Journal of the Electrochemical Society Vol. 159; no. 6; pp. B709 - B713 |
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Main Authors | , , , , |
Format | Journal Article |
Language | English |
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The Electrochemical Society, Inc
01.01.2012
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Abstract | A device and a method for direct measurement of the local contact pressures of gas diffusion layers (GDL) are presented. The new tool determines the spatially resolved contact pressure on the GDL side opposite to the flow-field/GDL interface which is relevant to good electrical contact between the GDL and the catalyst coated membrane (CCM) in a practical fuel cell setting. In a second step, using a fit function determined by separate two and four point resistance measurements, the method is extended to deliver spatially resolved contact resistance data. These experimental methods, in addition to shear-force measurements, are applied to a range of state-of-the-art GDL media. Whereas the shear-force measurements correlate well with data from recent work in the literature, the comparison of a non-woven and a paper based GDL with distinct differences in their shear moduli shows almost the same contact pressures underneath the flow field channel. This result indicates that shear-force data alone is of limited use for predicting contact pressure underneath flow field channels. In-situ current/voltage curves confirm the predictive power of a direct measurement of the contact pressure which highlights the importance for future GDL development and modeling activities. |
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AbstractList | A device and a method for direct measurement of the local contact pressures of gas diffusion layers (GDL) are presented. The new tool determines the spatially resolved contact pressure on the GDL side opposite to the flow-field/GDL interface which is relevant to good electrical contact between the GDL and the catalyst coated membrane (CCM) in a practical fuel cell setting. In a second step, using a fit function determined by separate two and four point resistance measurements, the method is extended to deliver spatially resolved contact resistance data. These experimental methods, in addition to shear-force measurements, are applied to a range of state-of-the-art GDL media. Whereas the shear-force measurements correlate well with data from recent work in the literature, the comparison of a non-woven and a paper based GDL with distinct differences in their shear moduli shows almost the same contact pressures underneath the flow field channel. This result indicates that shear-force data alone is of limited use for predicting contact pressure underneath flow field channels. In-situ current/voltage curves confirm the predictive power of a direct measurement of the contact pressure which highlights the importance for future GDL development and modeling activities. |
Author | Roth, Christina Butsch, Hanno Bock, Achim Hoogers, Gregor Ritzinger, Dietrich |
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CitedBy_id | crossref_primary_10_1016_j_jpowsour_2015_08_099 crossref_primary_10_1021_acs_energyfuels_3c01629 crossref_primary_10_1016_j_energy_2016_07_074 crossref_primary_10_1016_j_ijhydene_2013_01_151 crossref_primary_10_1016_j_jpowsour_2021_229540 crossref_primary_10_1016_j_jpowsour_2013_03_165 crossref_primary_10_1149_2_0691706jes |
Cites_doi | 10.1093/biomet/52.3-4.591 10.1016/j.jpowsour.2009.05.019 10.1016/j.jpowsour.2006.07.070 10.1016/j.jpowsour.2005.12.080 10.1093/biomet/34.1-2.28 10.1149/1.3210555 10.1016/j.jpowsour.2007.12.065 10.1016/j.jpowsour.2008.09.026 10.1016/j.jpowsour.2008.03.069 10.1149/1.3187913 10.1201/9781420041552 10.1016/j.ijhydene.2010.12.031 10.1149/1.3247585 10.1149/1.3496616 10.1149/1.3043422 10.1149/1.2345591 |
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Title | Spatially Resolved Contact Pressure and Contact Resistance Measurements at the Gas Diffusion Layer: A Tool for PEM Fuel Cell Development |
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