Black phosphorus composites with engineered interfaces for high-rate high-capacity lithium storage
A focus of battery research has been the development of a range of lithium, sodium, and potassium cathodes, but improving anode materials is also an important goal. Silicon has shown some promise for replacing graphite because of its exceptional capacity, but the dramatic volume change during lithia...
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| Published in | Science (American Association for the Advancement of Science) Vol. 370; no. 6513; pp. 192 - 197 |
|---|---|
| Main Authors | , , , , , , , , , , , , , , , , |
| Format | Journal Article |
| Language | English |
| Published |
Washington
The American Association for the Advancement of Science
09.10.2020
|
| Subjects | |
| Online Access | Get full text |
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| Abstract | A focus of battery research has been the development of a range of lithium, sodium, and potassium cathodes, but improving anode materials is also an important goal. Silicon has shown some promise for replacing graphite because of its exceptional capacity, but the dramatic volume change during lithiation-delithiation processes often leads to failure. Jin
et al.
developed a composite that is made of black phosphorous and graphite in its core and covered with swollen polyaniline. In contrast to previous efforts, bonding between the carbon and phosphorous allows for a high charging rate without sacrifices in capacity and cycling stability.
Science
, this issue p.
192
Black phosphorus composites with engineered interfaces deliver high capacity, high rate capability, and long cycle life.
High-rate lithium (Li) ion batteries that can be charged in minutes and store enough energy for a 350-mile driving range are highly desired for all-electric vehicles. A high charging rate usually leads to sacrifices in capacity and cycling stability. We report use of black phosphorus (BP) as the active anode for high-rate, high-capacity Li storage. The formation of covalent bonds with graphitic carbon restrains edge reconstruction in layered BP particles to ensure open edges for fast Li
+
entry; the coating of the covalently bonded BP-graphite particles with electrolyte-swollen polyaniline yields a stable solid–electrolyte interphase and inhibits the continuous growth of poorly conducting Li fluorides and carbonates to ensure efficient Li
+
transport. The resultant composite anode demonstrates an excellent combination of capacity, rate, and cycling endurance. |
|---|---|
| AbstractList | High-rate lithium (Li) ion batteries that can be charged in minutes and store enough energy for a 350-mile driving range are highly desired for all-electric vehicles. A high charging rate usually leads to sacrifices in capacity and cycling stability. We report use of black phosphorus (BP) as the active anode for high-rate, high-capacity Li storage. The formation of covalent bonds with graphitic carbon restrains edge reconstruction in layered BP particles to ensure open edges for fast Li+ entry; the coating of the covalently bonded BP-graphite particles with electrolyte-swollen polyaniline yields a stable solid-electrolyte interphase and inhibits the continuous growth of poorly conducting Li fluorides and carbonates to ensure efficient Li+ transport. The resultant composite anode demonstrates an excellent combination of capacity, rate, and cycling endurance.High-rate lithium (Li) ion batteries that can be charged in minutes and store enough energy for a 350-mile driving range are highly desired for all-electric vehicles. A high charging rate usually leads to sacrifices in capacity and cycling stability. We report use of black phosphorus (BP) as the active anode for high-rate, high-capacity Li storage. The formation of covalent bonds with graphitic carbon restrains edge reconstruction in layered BP particles to ensure open edges for fast Li+ entry; the coating of the covalently bonded BP-graphite particles with electrolyte-swollen polyaniline yields a stable solid-electrolyte interphase and inhibits the continuous growth of poorly conducting Li fluorides and carbonates to ensure efficient Li+ transport. The resultant composite anode demonstrates an excellent combination of capacity, rate, and cycling endurance. A focus of battery research has been the development of a range of lithium, sodium, and potassium cathodes, but improving anode materials is also an important goal. Silicon has shown some promise for replacing graphite because of its exceptional capacity, but the dramatic volume change during lithiation-delithiation processes often leads to failure. Jin et al. developed a composite that is made of black phosphorous and graphite in its core and covered with swollen polyaniline. In contrast to previous efforts, bonding between the carbon and phosphorous allows for a high charging rate without sacrifices in capacity and cycling stability. Science , this issue p. 192 Black phosphorus composites with engineered interfaces deliver high capacity, high rate capability, and long cycle life. High-rate lithium (Li) ion batteries that can be charged in minutes and store enough energy for a 350-mile driving range are highly desired for all-electric vehicles. A high charging rate usually leads to sacrifices in capacity and cycling stability. We report use of black phosphorus (BP) as the active anode for high-rate, high-capacity Li storage. The formation of covalent bonds with graphitic carbon restrains edge reconstruction in layered BP particles to ensure open edges for fast Li + entry; the coating of the covalently bonded BP-graphite particles with electrolyte-swollen polyaniline yields a stable solid–electrolyte interphase and inhibits the continuous growth of poorly conducting Li fluorides and carbonates to ensure efficient Li + transport. The resultant composite anode demonstrates an excellent combination of capacity, rate, and cycling endurance. Engineering phosphorous anodesA focus of battery research has been the development of a range of lithium, sodium, and potassium cathodes, but improving anode materials is also an important goal. Silicon has shown some promise for replacing graphite because of its exceptional capacity, but the dramatic volume change during lithiation-delithiation processes often leads to failure. Jin et al. developed a composite that is made of black phosphorous and graphite in its core and covered with swollen polyaniline. In contrast to previous efforts, bonding between the carbon and phosphorous allows for a high charging rate without sacrifices in capacity and cycling stability.Science, this issue p. 192High-rate lithium (Li) ion batteries that can be charged in minutes and store enough energy for a 350-mile driving range are highly desired for all-electric vehicles. A high charging rate usually leads to sacrifices in capacity and cycling stability. We report use of black phosphorus (BP) as the active anode for high-rate, high-capacity Li storage. The formation of covalent bonds with graphitic carbon restrains edge reconstruction in layered BP particles to ensure open edges for fast Li+ entry; the coating of the covalently bonded BP-graphite particles with electrolyte-swollen polyaniline yields a stable solid–electrolyte interphase and inhibits the continuous growth of poorly conducting Li fluorides and carbonates to ensure efficient Li+ transport. The resultant composite anode demonstrates an excellent combination of capacity, rate, and cycling endurance. |
| Author | Lu, Ying-Rui Chan, Ting-Shan Ji, Hengxing Duan, Xiangfeng Yan, Wensheng Wang, Haiyun Goodenough, John B. Li, Wangda Qi, Zhikai Xin, Sen Xie, Huanyu Jin, Hongchang Zhang, Taiming Zhu, Jian Chuang, Chenghao Wu, Xiaojun Wan, Yangyang |
| Author_xml | – sequence: 1 givenname: Hongchang orcidid: 0000-0002-3717-2696 surname: Jin fullname: Jin, Hongchang organization: Hefei National Laboratory for Physical Sciences at the Microscale, CAS Key Laboratory of Materials for Energy Conversion, School of Chemistry and Materials Science, University of Science and Technology of China, Hefei 230026, China – sequence: 2 givenname: Sen surname: Xin fullname: Xin, Sen organization: CAS Key Laboratory of Molecular Nanostructure and Nanotechnology, Beijing National Laboratory for Molecular Sciences (BNLMS), Institute of Chemistry, Chinese Academy of Sciences (CAS), Beijing 100190, China., Department of Mechanical Engineering, The University of Texas at Austin, Austin, TX 78712, USA – sequence: 3 givenname: Chenghao orcidid: 0000-0001-8161-1521 surname: Chuang fullname: Chuang, Chenghao organization: Department of Physics, Tamkang University, Tamsui 251, New Taipei City, Taiwan – sequence: 4 givenname: Wangda orcidid: 0000-0001-8103-4285 surname: Li fullname: Li, Wangda organization: Department of Mechanical Engineering, The University of Texas at Austin, Austin, TX 78712, USA – sequence: 5 givenname: Haiyun orcidid: 0000-0003-1345-2690 surname: Wang fullname: Wang, Haiyun organization: Hefei National Laboratory for Physical Sciences at the Microscale, CAS Key Laboratory of Materials for Energy Conversion, School of Chemistry and Materials Science, University of Science and Technology of China, Hefei 230026, China – sequence: 6 givenname: Jian orcidid: 0000-0001-9852-1645 surname: Zhu fullname: Zhu, Jian organization: State Key Laboratory for Chemo/Biosensing and Chemometrics, College of Chemistry and Chemical Engineering, Hunan University, Changsha 410082, China – sequence: 7 givenname: Huanyu orcidid: 0000-0003-1470-1951 surname: Xie fullname: Xie, Huanyu organization: Hefei National Laboratory for Physical Sciences at the Microscale, CAS Key Laboratory of Materials for Energy Conversion, School of Chemistry and Materials Science, University of Science and Technology of China, Hefei 230026, China – sequence: 8 givenname: Taiming orcidid: 0000-0002-0623-652X surname: Zhang fullname: Zhang, Taiming organization: Hefei National Laboratory for Physical Sciences at the Microscale, CAS Key Laboratory of Materials for Energy Conversion, School of Chemistry and Materials Science, University of Science and Technology of China, Hefei 230026, China – sequence: 9 givenname: Yangyang surname: Wan fullname: Wan, Yangyang organization: Hefei National Laboratory for Physical Sciences at the Microscale, CAS Key Laboratory of Materials for Energy Conversion, School of Chemistry and Materials Science, University of Science and Technology of China, Hefei 230026, China – sequence: 10 givenname: Zhikai orcidid: 0000-0002-0985-8316 surname: Qi fullname: Qi, Zhikai organization: Hefei National Laboratory for Physical Sciences at the Microscale, CAS Key Laboratory of Materials for Energy Conversion, School of Chemistry and Materials Science, University of Science and Technology of China, Hefei 230026, China – sequence: 11 givenname: Wensheng surname: Yan fullname: Yan, Wensheng organization: National Synchrotron Radiation Laboratory, University of Science and Technology of China, Hefei 230029, China – sequence: 12 givenname: Ying-Rui orcidid: 0000-0002-6002-5627 surname: Lu fullname: Lu, Ying-Rui organization: National Synchrotron Radiation Research Center, 300 Hsinchu, Taiwan – sequence: 13 givenname: Ting-Shan orcidid: 0000-0001-5220-1611 surname: Chan fullname: Chan, Ting-Shan organization: National Synchrotron Radiation Research Center, 300 Hsinchu, Taiwan – sequence: 14 givenname: Xiaojun orcidid: 0000-0003-3606-1211 surname: Wu fullname: Wu, Xiaojun organization: Hefei National Laboratory for Physical Sciences at the Microscale, CAS Key Laboratory of Materials for Energy Conversion, School of Chemistry and Materials Science, University of Science and Technology of China, Hefei 230026, China – sequence: 15 givenname: John B. orcidid: 0000-0001-9350-3034 surname: Goodenough fullname: Goodenough, John B. organization: Department of Mechanical Engineering, The University of Texas at Austin, Austin, TX 78712, USA – sequence: 16 givenname: Hengxing orcidid: 0000-0003-2851-9878 surname: Ji fullname: Ji, Hengxing organization: Hefei National Laboratory for Physical Sciences at the Microscale, CAS Key Laboratory of Materials for Energy Conversion, School of Chemistry and Materials Science, University of Science and Technology of China, Hefei 230026, China – sequence: 17 givenname: Xiangfeng orcidid: 0000-0002-4321-6288 surname: Duan fullname: Duan, Xiangfeng organization: Department of Chemistry and Biochemistry, University of California, Los Angeles, CA 90095, USA |
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| SubjectTerms | Anodes Batteries Carbon Carbonates Cathodes Charging Covalent bonds Electric vehicles Electrode materials Electrolytes Fluorides Graphite Interfaces Lithium Phosphorus Polyanilines Stability Storage batteries |
| Title | Black phosphorus composites with engineered interfaces for high-rate high-capacity lithium storage |
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| Volume | 370 |
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