Optical thermometry based on up-conversion luminescence of Tm3+ doped transparent Sr2YF7 glass ceramics
Tm3+/Yb3+ co-doped transparent glass ceramics (GC) containing Sr2YF7 nanocrystals were successfully manufactured by traditional melt-quenching technique. Their structural and up-conversion luminescent properties were systemically investigated through X-ray diffraction (XRD), transmission electron mi...
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| Published in | Journal of luminescence Vol. 192; pp. 303 - 309 |
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| Main Authors | , , , , , |
| Format | Journal Article |
| Language | English |
| Published |
Elsevier B.V
01.12.2017
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| Subjects | |
| Online Access | Get full text |
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| Abstract | Tm3+/Yb3+ co-doped transparent glass ceramics (GC) containing Sr2YF7 nanocrystals were successfully manufactured by traditional melt-quenching technique. Their structural and up-conversion luminescent properties were systemically investigated through X-ray diffraction (XRD), transmission electron microscope (TEM) and a series of spectroscopy methods. Tremendously enhanced up-conversion emissions with obvious Stark splitting and prolonged luminescence lifetime were observed after crystallization. These optical spectroscopy results manifest that Tm3+ ions have incorporated into the Sr2YF7 crystalline lattice with low phonon energy (~ 400cm−1) after heat-treatment. The 3F2,3 and 3H4 levels of Tm3+ can be explored as thermally coupled energy levels (TCEL) for temperature sensing because of their befitting energy gap (~ 2000cm−1). At the same time, the population of 1G4 state of Tm3+ is indirectly originated from 3H4 one. Therefore the temperature sensing performances of Tm3+ doped Sr2YF7 GC were investigated by fluorescence intensity ratio (FIR) between 3F2,3 → 3H6 and 1G4 → 3F4 up-conversion emissions of Tm3+. Results show that the theoretical maximum value of relative sensitivity SR-max is 1.16%K−1 at 428 K, and absolute sensitivity SA keeps increasing with temperature. Such Tm3+/Yb3+ co-doped Sr2YF7 GC may be excellent candidate for optical temperature sensors. |
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| AbstractList | Tm3+/Yb3+ co-doped transparent glass ceramics (GC) containing Sr2YF7 nanocrystals were successfully manufactured by traditional melt-quenching technique. Their structural and up-conversion luminescent properties were systemically investigated through X-ray diffraction (XRD), transmission electron microscope (TEM) and a series of spectroscopy methods. Tremendously enhanced up-conversion emissions with obvious Stark splitting and prolonged luminescence lifetime were observed after crystallization. These optical spectroscopy results manifest that Tm3+ ions have incorporated into the Sr2YF7 crystalline lattice with low phonon energy (~ 400cm−1) after heat-treatment. The 3F2,3 and 3H4 levels of Tm3+ can be explored as thermally coupled energy levels (TCEL) for temperature sensing because of their befitting energy gap (~ 2000cm−1). At the same time, the population of 1G4 state of Tm3+ is indirectly originated from 3H4 one. Therefore the temperature sensing performances of Tm3+ doped Sr2YF7 GC were investigated by fluorescence intensity ratio (FIR) between 3F2,3 → 3H6 and 1G4 → 3F4 up-conversion emissions of Tm3+. Results show that the theoretical maximum value of relative sensitivity SR-max is 1.16%K−1 at 428 K, and absolute sensitivity SA keeps increasing with temperature. Such Tm3+/Yb3+ co-doped Sr2YF7 GC may be excellent candidate for optical temperature sensors. |
| Author | Chen, LiPing Guo, Hai Zeng, QingGuang Hu, FangFang Wei, RongFei Chen, WeiPing |
| Author_xml | – sequence: 1 givenname: WeiPing surname: Chen fullname: Chen, WeiPing organization: Department of Physics, Zhejiang Normal University, Jinhua, Zhejiang 321004, China – sequence: 2 givenname: FangFang surname: Hu fullname: Hu, FangFang organization: Department of Physics, Zhejiang Normal University, Jinhua, Zhejiang 321004, China – sequence: 3 givenname: RongFei surname: Wei fullname: Wei, RongFei organization: Department of Physics, Zhejiang Normal University, Jinhua, Zhejiang 321004, China – sequence: 4 givenname: QingGuang surname: Zeng fullname: Zeng, QingGuang organization: School of Applied Physics and Materials, Wu Yi University, Jiangmen, Guangdong 529020, China – sequence: 5 givenname: LiPing surname: Chen fullname: Chen, LiPing organization: Department of Physics, Zhejiang Normal University, Jinhua, Zhejiang 321004, China – sequence: 6 givenname: Hai surname: Guo fullname: Guo, Hai email: ghh@zjnu.cn organization: Department of Physics, Zhejiang Normal University, Jinhua, Zhejiang 321004, China |
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| Snippet | Tm3+/Yb3+ co-doped transparent glass ceramics (GC) containing Sr2YF7 nanocrystals were successfully manufactured by traditional melt-quenching technique. Their... |
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| Title | Optical thermometry based on up-conversion luminescence of Tm3+ doped transparent Sr2YF7 glass ceramics |
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