Emission color tuning and phase transition determination based on high-pressure up-conversion luminescence in YVO4: Yb3+, Er3+ nanoparticles
Compression of up-converting (UC) YVO4 nanocrystals doped with Yb3+ and Er3+ ions leads to the luminescence color tuning, which can be used for the determination of pressure-induced zircon-to-scheelite phase transition. Spherical (≈20 nm), tetragonal YVO4: Yb3+-Er3+ UC nanoparticles (NPs) were synth...
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Published in | Journal of luminescence Vol. 209; pp. 321 - 327 |
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Format | Journal Article |
Language | English |
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Elsevier B.V
01.05.2019
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Abstract | Compression of up-converting (UC) YVO4 nanocrystals doped with Yb3+ and Er3+ ions leads to the luminescence color tuning, which can be used for the determination of pressure-induced zircon-to-scheelite phase transition. Spherical (≈20 nm), tetragonal YVO4: Yb3+-Er3+ UC nanoparticles (NPs) were synthesized by the hydrothermal method. The high-pressure spectroscopic analysis (up to ≈11 GPa) of the material was carried out in a diamond anvil cell (DAC), in a compression-decompression run. With the increasing pressure values, the intensity of UC emission (λex= 975 nm) decreased along with shifts of the band centroids. The maximum shifts was ≈ 0.39 nm/GPa, for the 4F9/2→4I15/2 transition. Broadening of the bands and overlapping of the split Stark sub-levels were also observed. The sudden and huge change in the band ratios, and deviations from the linear shift tendency of chromaticity coordinates in the CIE diagram around ≈ 8 GPa, clearly shows the influence of phase transition on the luminescence properties of the material, under high pressure conditions.
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AbstractList | Compression of up-converting (UC) YVO4 nanocrystals doped with Yb3+ and Er3+ ions leads to the luminescence color tuning, which can be used for the determination of pressure-induced zircon-to-scheelite phase transition. Spherical (≈20 nm), tetragonal YVO4: Yb3+-Er3+ UC nanoparticles (NPs) were synthesized by the hydrothermal method. The high-pressure spectroscopic analysis (up to ≈11 GPa) of the material was carried out in a diamond anvil cell (DAC), in a compression-decompression run. With the increasing pressure values, the intensity of UC emission (λex= 975 nm) decreased along with shifts of the band centroids. The maximum shifts was ≈ 0.39 nm/GPa, for the 4F9/2→4I15/2 transition. Broadening of the bands and overlapping of the split Stark sub-levels were also observed. The sudden and huge change in the band ratios, and deviations from the linear shift tendency of chromaticity coordinates in the CIE diagram around ≈ 8 GPa, clearly shows the influence of phase transition on the luminescence properties of the material, under high pressure conditions.
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Author | Lis, Stefan Runowski, Marcin Woźny, Przemysław |
Author_xml | – sequence: 1 givenname: Przemysław surname: Woźny fullname: Woźny, Przemysław – sequence: 2 givenname: Marcin surname: Runowski fullname: Runowski, Marcin email: runowski@amu.edu.pl – sequence: 3 givenname: Stefan orcidid: 0000-0002-3989-3913 surname: Lis fullname: Lis, Stefan |
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Keywords | Up-converting luminescent nanomaterials Lanthanides Yttrium vanadates High pressure phase transitions Upconversion band shift Tunable emission |
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Snippet | Compression of up-converting (UC) YVO4 nanocrystals doped with Yb3+ and Er3+ ions leads to the luminescence color tuning, which can be used for the... |
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SubjectTerms | High pressure phase transitions Lanthanides Tunable emission Up-converting luminescent nanomaterials Upconversion band shift Yttrium vanadates |
Title | Emission color tuning and phase transition determination based on high-pressure up-conversion luminescence in YVO4: Yb3+, Er3+ nanoparticles |
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