Carbon quantum dots/TiO2 composites for efficient photocatalytic hydrogen evolution
Carbon quantum dots modified P25 TiO₂ composites (CQDs/P25) with a “dyade”-like structure were prepared via a facile one-step hydrothermal reaction. CQDs/P25 exhibited improved photocatalytic H₂ evolution under UV-Vis and visible light (λ > 450 nm) irradiation without loading any noble metal coca...
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| Published in | Journal of materials chemistry. A, Materials for energy and sustainability Vol. 2; no. 10; pp. 3344 - 3351 |
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| Main Authors | , , , , , , , , |
| Format | Journal Article |
| Language | English |
| Published |
01.01.2014
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| Subjects | |
| Online Access | Get full text |
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| Abstract | Carbon quantum dots modified P25 TiO₂ composites (CQDs/P25) with a “dyade”-like structure were prepared via a facile one-step hydrothermal reaction. CQDs/P25 exhibited improved photocatalytic H₂ evolution under UV-Vis and visible light (λ > 450 nm) irradiation without loading any noble metal cocatalyst, compared to pure P25. A possible mechanism of the photocatalytic H₂ production activity over CQDs/P25 was proposed based on detailed measurements of the transient photocurrent response, surface photovoltage and hydroxyl radicals. CQDs play dual roles on the improved photocatalytic activity of CQDs/P25. Under UV-Vis light irradiation CQDs act as an electron reservoir to improve the efficient separation of the photoinduced electron–hole pairs of P25. However, under visible light irradiation CQDs act as a photosensitizer to sensitize P25 into a visible light response “dyade” structure for H₂ evolution. |
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| AbstractList | Carbon quantum dots modified P25 TiO₂ composites (CQDs/P25) with a “dyade”-like structure were prepared via a facile one-step hydrothermal reaction. CQDs/P25 exhibited improved photocatalytic H₂ evolution under UV-Vis and visible light (λ > 450 nm) irradiation without loading any noble metal cocatalyst, compared to pure P25. A possible mechanism of the photocatalytic H₂ production activity over CQDs/P25 was proposed based on detailed measurements of the transient photocurrent response, surface photovoltage and hydroxyl radicals. CQDs play dual roles on the improved photocatalytic activity of CQDs/P25. Under UV-Vis light irradiation CQDs act as an electron reservoir to improve the efficient separation of the photoinduced electron–hole pairs of P25. However, under visible light irradiation CQDs act as a photosensitizer to sensitize P25 into a visible light response “dyade” structure for H₂ evolution. |
| Author | Zhang, Tierui Zhao, Yufei Zhou, Chao Shang, Lu Peng, Yong Cao, Yinhu Wu, Li-Zhu Tung, Chen-Ho Yu, Huijun |
| Author_xml | – sequence: 1 givenname: Huijun surname: Yu fullname: Yu, Huijun – sequence: 2 givenname: Yufei surname: Zhao fullname: Zhao, Yufei – sequence: 3 givenname: Chao surname: Zhou fullname: Zhou, Chao – sequence: 4 givenname: Lu surname: Shang fullname: Shang, Lu – sequence: 5 givenname: Yong surname: Peng fullname: Peng, Yong – sequence: 6 givenname: Yinhu surname: Cao fullname: Cao, Yinhu – sequence: 7 givenname: Li-Zhu surname: Wu fullname: Wu, Li-Zhu – sequence: 8 givenname: Chen-Ho surname: Tung fullname: Tung, Chen-Ho – sequence: 9 givenname: Tierui surname: Zhang fullname: Zhang, Tierui |
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| Snippet | Carbon quantum dots modified P25 TiO₂ composites (CQDs/P25) with a “dyade”-like structure were prepared via a facile one-step hydrothermal reaction. CQDs/P25... |
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| SubjectTerms | carbon quantum dots catalysts electric current hydrogen hydrogen production hydroxyl radicals irradiation light photocatalysis photosensitizing agents titanium dioxide ultraviolet-visible spectroscopy |
| Title | Carbon quantum dots/TiO2 composites for efficient photocatalytic hydrogen evolution |
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