Influence of paraments on the transformation behaviors and directional adjustment strategies of phosphorus forms during different thermochemical treatments of sludge

[Display omitted] •Influence mechanism of technique type and paraments on P forms were clarified.•Controlling factors on the conversion of P forms were identified.•Correlation mechanism between P and accessory elements is well explained.•The conversion pathways of P forms during thermal treatments w...

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Published inFuel (Guildford) Vol. 333; p. 126544
Main Authors Fang, Zhenquan, Zhuang, Xiuzheng, Zhang, Xinghua, Li, Yanlong, Li, Rundong, Ma, Longlong
Format Journal Article
LanguageEnglish
Published Elsevier Ltd 01.02.2023
Subjects
Forms regulating
P recovery
Technology optimization
Transformation mechanisms
Forms regulating
Transformation mechanisms
P recovery
Technology optimization
Online AccessGet full text
ISSN0016-2361
DOI10.1016/j.fuel.2022.126544

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Abstract [Display omitted] •Influence mechanism of technique type and paraments on P forms were clarified.•Controlling factors on the conversion of P forms were identified.•Correlation mechanism between P and accessory elements is well explained.•The conversion pathways of P forms during thermal treatments were proposed.•Strategies for form regulation and technical optimization were provided. A variety of sludge originating from wastewater treatment is increasingly accumulating worldwide, especially in the developed regions. Fortunately, phosphorus (P) in sludge can potentially be recovered via thermal treatment, and P forms are crucial to the quality of the recovered products. This review provides an overview related to the transformation of P and its regulation strategies in the different thermal treatment processes, highlighting the current knowledge regarding the influence factors and mechanisms of transformation. First, the current researches with P recovery by thermal treatments (i.e., incineration, pyrolysis, and hydrothermal carbonization) were illustrated and critically discussed, which indicates that the selection of appropriate method significantly affects the recovery effects, such as the proportion of Apatite Phosphorus (AP) or Ca-P (P combing with Ca). Furthermore, the effects of various factors (e.g., treatment techniques, temperature, additives, the composition of sludge, pH and metals ions) on the transformation or regulation of P forms were critically discussed, suggesting that temperature and Ca/Cl-based additives are the two crucial factors, which have the considerable effects on the emergence of Ca-P. Especially the Ca-based additives, which have the highest combining ability with P and the uppermost impact on hydroxyapatite formation. In addition, an overall comparison of incineration, pyrolysis, and hydrothermal carbonization technologies in practical applications is provided, focusing on the recovery efficiency, advantages, and disadvantages, demonstrating that HTC will be more predominant for P recovery from sludge in the future. Finally, challenges and potential development directions regarding the transformation mechanisms of P forms and regulate strategies are identified. This review will become the foundation for future research devoted to improving the quality of the recovered products.
AbstractList [Display omitted] •Influence mechanism of technique type and paraments on P forms were clarified.•Controlling factors on the conversion of P forms were identified.•Correlation mechanism between P and accessory elements is well explained.•The conversion pathways of P forms during thermal treatments were proposed.•Strategies for form regulation and technical optimization were provided. A variety of sludge originating from wastewater treatment is increasingly accumulating worldwide, especially in the developed regions. Fortunately, phosphorus (P) in sludge can potentially be recovered via thermal treatment, and P forms are crucial to the quality of the recovered products. This review provides an overview related to the transformation of P and its regulation strategies in the different thermal treatment processes, highlighting the current knowledge regarding the influence factors and mechanisms of transformation. First, the current researches with P recovery by thermal treatments (i.e., incineration, pyrolysis, and hydrothermal carbonization) were illustrated and critically discussed, which indicates that the selection of appropriate method significantly affects the recovery effects, such as the proportion of Apatite Phosphorus (AP) or Ca-P (P combing with Ca). Furthermore, the effects of various factors (e.g., treatment techniques, temperature, additives, the composition of sludge, pH and metals ions) on the transformation or regulation of P forms were critically discussed, suggesting that temperature and Ca/Cl-based additives are the two crucial factors, which have the considerable effects on the emergence of Ca-P. Especially the Ca-based additives, which have the highest combining ability with P and the uppermost impact on hydroxyapatite formation. In addition, an overall comparison of incineration, pyrolysis, and hydrothermal carbonization technologies in practical applications is provided, focusing on the recovery efficiency, advantages, and disadvantages, demonstrating that HTC will be more predominant for P recovery from sludge in the future. Finally, challenges and potential development directions regarding the transformation mechanisms of P forms and regulate strategies are identified. This review will become the foundation for future research devoted to improving the quality of the recovered products.
ArticleNumber 126544
Author Zhuang, Xiuzheng
Ma, Longlong
Zhang, Xinghua
Li, Rundong
Fang, Zhenquan
Li, Yanlong
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  surname: Fang
  fullname: Fang, Zhenquan
  organization: Key Laboratory of Energy Thermal Conversion and Control of Ministry of Education, School of Energy and Environment, Southeast University, Nanjing 210096, PR China
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  givenname: Xiuzheng
  surname: Zhuang
  fullname: Zhuang, Xiuzheng
  organization: Key Laboratory of Energy Thermal Conversion and Control of Ministry of Education, School of Energy and Environment, Southeast University, Nanjing 210096, PR China
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  givenname: Xinghua
  surname: Zhang
  fullname: Zhang, Xinghua
  email: zhangxh@seu.edu.cn
  organization: Key Laboratory of Energy Thermal Conversion and Control of Ministry of Education, School of Energy and Environment, Southeast University, Nanjing 210096, PR China
– sequence: 4
  givenname: Yanlong
  surname: Li
  fullname: Li, Yanlong
  organization: Key Laboratory of Clean Energy of Liaoning Province, College of Energy and Environment, Shenyang Aerospace University, Shenyang 110136, PR China
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  givenname: Rundong
  surname: Li
  fullname: Li, Rundong
  organization: Key Laboratory of Clean Energy of Liaoning Province, College of Energy and Environment, Shenyang Aerospace University, Shenyang 110136, PR China
– sequence: 6
  givenname: Longlong
  surname: Ma
  fullname: Ma, Longlong
  email: mall@seu.edu.cn
  organization: Key Laboratory of Energy Thermal Conversion and Control of Ministry of Education, School of Energy and Environment, Southeast University, Nanjing 210096, PR China
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Snippet [Display omitted] •Influence mechanism of technique type and paraments on P forms were clarified.•Controlling factors on the conversion of P forms were...
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SubjectTerms Forms regulating
P recovery
Technology optimization
Transformation mechanisms
Title Influence of paraments on the transformation behaviors and directional adjustment strategies of phosphorus forms during different thermochemical treatments of sludge
URI https://dx.doi.org/10.1016/j.fuel.2022.126544
Volume 333
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