Discussion on “Design of acid-geopolymers based on clays by-products for methylene blue removal from wastewater” [Applied Clay Science 245 (2023) 107126]
The subject paper deals with the sorption of dyes (mainly methylene blue) on originally prepared geopolymers based on clay-rich wastes from the phosphate industry. However, the results of sorption experiments are marred by errors of interpretation that limit their validity. In particular, it is well...
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| Published in | Applied clay science Vol. 254; p. 107375 |
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| Main Authors | , , , |
| Format | Journal Article |
| Language | English |
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15.06.2024
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| Abstract | The subject paper deals with the sorption of dyes (mainly methylene blue) on originally prepared geopolymers based on clay-rich wastes from the phosphate industry. However, the results of sorption experiments are marred by errors of interpretation that limit their validity. In particular, it is well known that linearization of the equations used to model sorption kinetics (pseudo-first and pseudo-second order) and isotherms (Langmuir and Freundlich) should be avoided, as this may bias the calculated values. In addition, other selected models use incorrect equations, as in the case of the intra-particular diffusion kinetic model and the Temkin isotherm. Some additional results are inaccurate or illogical, such as the study of the influence of pH. We hope that our comments and suggestions will serve to correct the discussed paper and avoid repetition of these errors in future scientific literature. |
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| AbstractList | The subject paper deals with the sorption of dyes (mainly methylene blue) on originally prepared geopolymers based on clay-rich wastes from the phosphate industry. However, the results of sorption experiments are marred by errors of interpretation that limit their validity. In particular, it is well known that linearization of the equations used to model sorption kinetics (pseudo-first and pseudo-second order) and isotherms (Langmuir and Freundlich) should be avoided, as this may bias the calculated values. In addition, other selected models use incorrect equations, as in the case of the intra-particular diffusion kinetic model and the Temkin isotherm. Some additional results are inaccurate or illogical, such as the study of the influence of pH. We hope that our comments and suggestions will serve to correct the discussed paper and avoid repetition of these errors in future scientific literature. |
| ArticleNumber | 107375 |
| Author | Salvestrini, Stefano Bollinger, Jean-Claude Mouni, Lotfi Chu, Khim Hoong |
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| References | Salvestrini, Leone, Iovino, Canzano, Capasso (bb0070) 2014; 68 En-naji, Ghazi, Mabroum, Mabroum, Khatib, Taha, García Lodeiro, Hakkou (bb0030) 2023; 245 Schwaab, Steffani, Barbosa-Coutinho, Severo Júnior (bb0080) 2017; 173 Tran, You, Hosseini-Bandegharaei, Chao (bb0085) 2017; 120 Badertscher, Pretsch (bb0005) 2006; 25 Pourret, Bollinger, Hurtshouse, van Hullebusch (bb0060) 2022; 838 Bolster, Hornberger (bb0015) 2007; 72 Chu (bb0025) 2021; 60 Bollinger, Tran, Lima (bb0010) 2023; 210 Mouni, Belkhiri, Bollinger, Bouzaza, Assadi, Tirri, Dahmoune, Madani, Remini (bb0050) 2018; 153 Salvestrini, Bollinger (bb0065) 2022; 373 Nguyen, Juang (bb0055) 2019; 99 Wang, Giammar (bb0090) 2019; 53 Salvestrini, Ambrosone, Kopinke (bb0075) 2022; 352 Canzano, Iovino, Leone, Salvestrini, Capasso (bb0020) 2012; 30 Hubbe (bb0040) 2022; 51 Lima, Sher, Guleria, Saeb, Anastopoulos, Tran, Hosseini-Bandegharaei (bb0045) 2021; 9 González-López, Laureano-Anzaldo, Pérez-Fonseca, Arellano, Robledo-Ortíz (bb0035) 2022; 51 Nguyen (10.1016/j.clay.2024.107375_bb0055) 2019; 99 Tran (10.1016/j.clay.2024.107375_bb0085) 2017; 120 Badertscher (10.1016/j.clay.2024.107375_bb0005) 2006; 25 Salvestrini (10.1016/j.clay.2024.107375_bb0070) 2014; 68 En-naji (10.1016/j.clay.2024.107375_bb0030) 2023; 245 González-López (10.1016/j.clay.2024.107375_bb0035) 2022; 51 Lima (10.1016/j.clay.2024.107375_bb0045) 2021; 9 Hubbe (10.1016/j.clay.2024.107375_bb0040) 2022; 51 Pourret (10.1016/j.clay.2024.107375_bb0060) 2022; 838 Schwaab (10.1016/j.clay.2024.107375_bb0080) 2017; 173 Bollinger (10.1016/j.clay.2024.107375_bb0010) 2023; 210 Chu (10.1016/j.clay.2024.107375_bb0025) 2021; 60 Canzano (10.1016/j.clay.2024.107375_bb0020) 2012; 30 Salvestrini (10.1016/j.clay.2024.107375_bb0065) 2022; 373 Wang (10.1016/j.clay.2024.107375_bb0090) 2019; 53 Mouni (10.1016/j.clay.2024.107375_bb0050) 2018; 153 Bolster (10.1016/j.clay.2024.107375_bb0015) 2007; 72 Salvestrini (10.1016/j.clay.2024.107375_bb0075) 2022; 352 |
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| Title | Discussion on “Design of acid-geopolymers based on clays by-products for methylene blue removal from wastewater” [Applied Clay Science 245 (2023) 107126] |
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