Advances in supercritical water gasification of lignocellulosic biomass for hydrogen production

Supercritical water gasification (SCWG) with biomass is a combined thermal decomposition and hydrolysis process that converts biomass feedstock into hydrogen rich syngas. Renewable biomass as feedstock provides value for the sustainable development of this technology. This review discusses the relat...

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Published inJournal of analytical and applied pyrolysis Vol. 170; p. 105934
Main Authors Wang, Qing, Zhang, Xu, Cui, Da, Bai, Jingru, Wang, Zhichao, Xu, Faxing, Wang, Zhenye
Format Journal Article
LanguageEnglish
Published Elsevier B.V 01.03.2023
Subjects
Catalysts
Hydrogen
Hydrothermal method
Lignocellulosic biomass
Supercritical water gasification
Hydrothermal method
Catalysts
Supercritical water gasification
Hydrogen
Lignocellulosic biomass
Online AccessGet full text
ISSN0165-2370
1873-250X
DOI10.1016/j.jaap.2023.105934

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Abstract Supercritical water gasification (SCWG) with biomass is a combined thermal decomposition and hydrolysis process that converts biomass feedstock into hydrogen rich syngas. Renewable biomass as feedstock provides value for the sustainable development of this technology. This review discusses the relationship between cellulose, hemicellulose, lignin and hydrogen production; considers the effects of reaction temperature, pressure, reactant concentration and reaction residence time; and explores the advantages and drawbacks of different types of catalysts for enhanced SCWG hydrogen production process. The results show that temperature and catalyst have the greatest impact on SCWG. The other operating conditions are biomass type > pressure > reactant concentration > reaction residence time. However, the SCWG mechanism of real lignocellulosic biomass remains to be studied. The interaction relationship of three components is also unclear. In addition, the development of catalysts with high stability and performance is the top priority in the development of this technology. [Display omitted] •Biomass with high cellulose content is easier to gasify and produce hydrogen.•Temperature and catalyst have the greatest impact on SCWG.•Enhancing gasification at high concentration can improve the competitiveness of SCWG.•The development of stable and recyclable catalysts will be a major direction.•The SCWG of real biomass and interactions of three components remain to be studied.
AbstractList Supercritical water gasification (SCWG) with biomass is a combined thermal decomposition and hydrolysis process that converts biomass feedstock into hydrogen rich syngas. Renewable biomass as feedstock provides value for the sustainable development of this technology. This review discusses the relationship between cellulose, hemicellulose, lignin and hydrogen production; considers the effects of reaction temperature, pressure, reactant concentration and reaction residence time; and explores the advantages and drawbacks of different types of catalysts for enhanced SCWG hydrogen production process. The results show that temperature and catalyst have the greatest impact on SCWG. The other operating conditions are biomass type > pressure > reactant concentration > reaction residence time. However, the SCWG mechanism of real lignocellulosic biomass remains to be studied. The interaction relationship of three components is also unclear. In addition, the development of catalysts with high stability and performance is the top priority in the development of this technology. [Display omitted] •Biomass with high cellulose content is easier to gasify and produce hydrogen.•Temperature and catalyst have the greatest impact on SCWG.•Enhancing gasification at high concentration can improve the competitiveness of SCWG.•The development of stable and recyclable catalysts will be a major direction.•The SCWG of real biomass and interactions of three components remain to be studied.
ArticleNumber 105934
Author Bai, Jingru
Xu, Faxing
Zhang, Xu
Wang, Zhichao
Cui, Da
Wang, Zhenye
Wang, Qing
Author_xml – sequence: 1
  givenname: Qing
  surname: Wang
  fullname: Wang, Qing
  email: rlx888@126.com
  organization: Engineering Research Centre of Oil Shale Comprehensive Utilization, Ministry of Education, Northeast Electric Power University, Jilin City, Jilin 132012, PR China
– sequence: 2
  givenname: Xu
  surname: Zhang
  fullname: Zhang, Xu
  organization: Engineering Research Centre of Oil Shale Comprehensive Utilization, Ministry of Education, Northeast Electric Power University, Jilin City, Jilin 132012, PR China
– sequence: 3
  givenname: Da
  surname: Cui
  fullname: Cui, Da
  email: jlcuida@163.com
  organization: Engineering Research Centre of Oil Shale Comprehensive Utilization, Ministry of Education, Northeast Electric Power University, Jilin City, Jilin 132012, PR China
– sequence: 4
  givenname: Jingru
  surname: Bai
  fullname: Bai, Jingru
  organization: Engineering Research Centre of Oil Shale Comprehensive Utilization, Ministry of Education, Northeast Electric Power University, Jilin City, Jilin 132012, PR China
– sequence: 5
  givenname: Zhichao
  surname: Wang
  fullname: Wang, Zhichao
  organization: Engineering Research Centre of Oil Shale Comprehensive Utilization, Ministry of Education, Northeast Electric Power University, Jilin City, Jilin 132012, PR China
– sequence: 6
  givenname: Faxing
  surname: Xu
  fullname: Xu, Faxing
  organization: Jilin Feite Environmental Protection Co. Ltd, Jilin Key Laboratory of Subcritical Hydrolysis Technology, Jilin 132200, PR China
– sequence: 7
  givenname: Zhenye
  surname: Wang
  fullname: Wang, Zhenye
  organization: Jilin Feite Environmental Protection Co. Ltd, Jilin Key Laboratory of Subcritical Hydrolysis Technology, Jilin 132200, PR China
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Catalysts
Supercritical water gasification
Hydrogen
Lignocellulosic biomass
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Snippet Supercritical water gasification (SCWG) with biomass is a combined thermal decomposition and hydrolysis process that converts biomass feedstock into hydrogen...
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SubjectTerms Catalysts
Hydrogen
Hydrothermal method
Lignocellulosic biomass
Supercritical water gasification
Title Advances in supercritical water gasification of lignocellulosic biomass for hydrogen production
URI https://dx.doi.org/10.1016/j.jaap.2023.105934
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