Tuning the magnetic and magnetoelectric response in Bi1-xYxFe0.7Mn0.3O3 multiferroics
•Yttrium substitution improves grain growth.•Optimum sintering temperature for this compound is 825 °C.•Maximum magnetoelectric coefficient is observed for x = 0.10 compound. Magnetoelectric (ME) coupling in multiferroic materials plays an important role in designing multifunctional devices because...
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| Published in | Journal of magnetism and magnetic materials Vol. 581; p. 170988 |
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| Main Authors | , , |
| Format | Journal Article |
| Language | English |
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Elsevier B.V
01.09.2023
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| Abstract | •Yttrium substitution improves grain growth.•Optimum sintering temperature for this compound is 825 °C.•Maximum magnetoelectric coefficient is observed for x = 0.10 compound.
Magnetoelectric (ME) coupling in multiferroic materials plays an important role in designing multifunctional devices because of their potential to tune polarization via a magnetic field or magnetism via an electric field. However, the single-phase ME materials have not been successfully explored in practical devices due to their low ME coupling coefficient. Here, we optimized the magnetic and magnetoelectric response of single-phase Bi1-xYxFe0.7Mn0.3O3 compounds by controlling the Y substitution and sintering temperature. Single-phase Bi1-xYxFe0.7Mn0.3O3 (where x varies from 0 to 0.20 in the step of 0.05) compounds were prepared by a standard solid-state reaction technique. The optimum sintering temperature and yttrium substitution were found to be 825 °C and x = 0.10, respectively, in which the sample shows the optimum microstructural, magnetic, and ME properties at room temperature. The optimized Bi0.9Y0.1Fe0.7Mn0.3O3 compound shows uniform growth of grains with less porosity, maximum remanent magnetization (∼0.012 emu/g), and enhanced ME coupling coefficient (35 mV/Oe.cm.). The ME coupling coefficient obtained from the optimized sample is six times higher than that of the pristine sample. This work provides a potential route for improving the ME coupling coefficient in BiFeO3-based multiferroic materials for practical applications. |
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| AbstractList | •Yttrium substitution improves grain growth.•Optimum sintering temperature for this compound is 825 °C.•Maximum magnetoelectric coefficient is observed for x = 0.10 compound.
Magnetoelectric (ME) coupling in multiferroic materials plays an important role in designing multifunctional devices because of their potential to tune polarization via a magnetic field or magnetism via an electric field. However, the single-phase ME materials have not been successfully explored in practical devices due to their low ME coupling coefficient. Here, we optimized the magnetic and magnetoelectric response of single-phase Bi1-xYxFe0.7Mn0.3O3 compounds by controlling the Y substitution and sintering temperature. Single-phase Bi1-xYxFe0.7Mn0.3O3 (where x varies from 0 to 0.20 in the step of 0.05) compounds were prepared by a standard solid-state reaction technique. The optimum sintering temperature and yttrium substitution were found to be 825 °C and x = 0.10, respectively, in which the sample shows the optimum microstructural, magnetic, and ME properties at room temperature. The optimized Bi0.9Y0.1Fe0.7Mn0.3O3 compound shows uniform growth of grains with less porosity, maximum remanent magnetization (∼0.012 emu/g), and enhanced ME coupling coefficient (35 mV/Oe.cm.). The ME coupling coefficient obtained from the optimized sample is six times higher than that of the pristine sample. This work provides a potential route for improving the ME coupling coefficient in BiFeO3-based multiferroic materials for practical applications. |
| ArticleNumber | 170988 |
| Author | Azizar Rahman, M. Kumar Saha, Sonet Akther Hossain, A.K.M. |
| Author_xml | – sequence: 1 givenname: Sonet surname: Kumar Saha fullname: Kumar Saha, Sonet organization: Department of Physics, Bangladesh University of Engineering and Technology, Dhaka 1000, Bangladesh – sequence: 2 givenname: M. surname: Azizar Rahman fullname: Azizar Rahman, M. organization: Department of Physics, Bangladesh University of Engineering and Technology, Dhaka 1000, Bangladesh – sequence: 3 givenname: A.K.M. surname: Akther Hossain fullname: Akther Hossain, A.K.M. email: akmhossain@phy.buet.ac.bd organization: Department of Physics, Bangladesh University of Engineering and Technology, Dhaka 1000, Bangladesh |
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| Title | Tuning the magnetic and magnetoelectric response in Bi1-xYxFe0.7Mn0.3O3 multiferroics |
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