Multi-layered nanostructure Bi2Se3 grown by chemical vapor deposition in selenium-rich atmosphere
•The multi-layered nanostructured Bi2Se3 were prepared by CVD using the high purity Se and Bi2Se3 powder as source materials to decrease the Se vacancies in the products.•The wide nanoribbons grown along the [1 1 2¯ 0] direction were prepared, and the growth mechanism along the different directions...
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| Published in | Applied surface science Vol. 317; pp. 257 - 261 |
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| Main Authors | , , , , |
| Format | Journal Article |
| Language | English |
| Published |
Amsterdam
Elsevier B.V
30.10.2014
Elsevier |
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| Abstract | •The multi-layered nanostructured Bi2Se3 were prepared by CVD using the high purity Se and Bi2Se3 powder as source materials to decrease the Se vacancies in the products.•The wide nanoribbons grown along the [1 1 2¯ 0] direction were prepared, and the growth mechanism along the different directions was analyzed.•The low-temperature growth mechanism of the multi-layered Bi2Se3 nanostructure was analyzed by the Raman spectra with different depths.
High quality multi-layered nanostructured bismuth selenide (Bi2Se3) with an asymmetric, elongated hexagonal morphology were obtained in a selenium-rich atmosphere by chemical vapor deposition (CVD) using high purity Se and Bi2Se3 powder as source materials. The measurement results reveal that Au particles only serve as the initial stage nucleation of the Bi2Se3 nanostructures at a low temperature. The Se powder in the source materials is helpful to ensure the stoichiometry and decrease the selenium vacancies, and causes the wide Bi2Se3 nanoribbons to grow along the lateral direction. |
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| AbstractList | •The multi-layered nanostructured Bi2Se3 were prepared by CVD using the high purity Se and Bi2Se3 powder as source materials to decrease the Se vacancies in the products.•The wide nanoribbons grown along the [1 1 2¯ 0] direction were prepared, and the growth mechanism along the different directions was analyzed.•The low-temperature growth mechanism of the multi-layered Bi2Se3 nanostructure was analyzed by the Raman spectra with different depths.
High quality multi-layered nanostructured bismuth selenide (Bi2Se3) with an asymmetric, elongated hexagonal morphology were obtained in a selenium-rich atmosphere by chemical vapor deposition (CVD) using high purity Se and Bi2Se3 powder as source materials. The measurement results reveal that Au particles only serve as the initial stage nucleation of the Bi2Se3 nanostructures at a low temperature. The Se powder in the source materials is helpful to ensure the stoichiometry and decrease the selenium vacancies, and causes the wide Bi2Se3 nanoribbons to grow along the lateral direction. High quality multi-layered nanostructured bismuth selenide (Bi2Se3) with an asymmetric, elongated hexagonal morphology were obtained in a selenium-rich atmosphere by chemical vapor deposition (CVD) using high purity Se and Bi2Se3 powder as source materials. The measurement results reveal that Au particles only serve as the initial stage nucleation of the Bi2Se3 nanostructures at a low temperature. The Se powder in the source materials is helpful to ensure the stoichiometry and decrease the selenium vacancies, and causes the wide Bi2Se3 nanoribbons to grow along the lateral direction. |
| Author | Liu, Fu Yan Bi, Dong Man, Bao Yuan Xu, Xue You Liu, Mei |
| Author_xml | – sequence: 1 givenname: Mei surname: Liu fullname: Liu, Mei email: liumei@sdnu.edu.cn organization: College of Physics and Electronics, Shandong Normal University, Jinan 250014, PR China – sequence: 2 givenname: Fu Yan surname: Liu fullname: Liu, Fu Yan organization: College of Physics and Electronics, Shandong Normal University, Jinan 250014, PR China – sequence: 3 givenname: Bao Yuan surname: Man fullname: Man, Bao Yuan organization: College of Physics and Electronics, Shandong Normal University, Jinan 250014, PR China – sequence: 4 givenname: Dong surname: Bi fullname: Bi, Dong organization: College of Physics and Electronics, Shandong Normal University, Jinan 250014, PR China – sequence: 5 givenname: Xue You surname: Xu fullname: Xu, Xue You organization: Information Research Institute, Shandong Academy of Sciences, Jinan 250014, PR China |
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| Keywords | Topological insulator Multi-layered nanostructure Bismuth selenide Chemical vapor deposition CVD Bismuth selenides Multilayers Inorganic compounds Binary compounds Nanostructures Selenium Film growth |
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| Snippet | •The multi-layered nanostructured Bi2Se3 were prepared by CVD using the high purity Se and Bi2Se3 powder as source materials to decrease the Se vacancies in... High quality multi-layered nanostructured bismuth selenide (Bi2Se3) with an asymmetric, elongated hexagonal morphology were obtained in a selenium-rich... |
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| SubjectTerms | Asymmetry Atmospheres Bismuth Bismuth selenide Chemical vapor deposition Condensed matter: electronic structure, electrical, magnetic, and optical properties Condensed matter: structure, mechanical and thermal properties Cross-disciplinary physics: materials science; rheology Elongation Exact sciences and technology Multi-layered nanostructure Nanostructure Nucleation Physics Selenides Topological insulator |
| Title | Multi-layered nanostructure Bi2Se3 grown by chemical vapor deposition in selenium-rich atmosphere |
| URI | https://dx.doi.org/10.1016/j.apsusc.2014.08.103 https://search.proquest.com/docview/1660040052 |
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