Iron-based metal–organic frameworks and derivatives for electrochemical energy storage and conversion

•Fe-MOF nanomaterials are efficient electrocatalysts for energy storage and conversion.•Recent advances in synthesis strategies and applications of Fe-MOFs were highlighted.•Overview of MOF materials, structural diversity and design of Fe-MOF were highlighted.•DFT calculations have prospect for deta...

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Published inCoordination chemistry reviews Vol. 517; p. 215959
Main Authors Adegoke, Kayode Adesina, Oyebamiji, Abel Kolawole, Adeola, Adedapo O., Olabintan, Abdullahi Biodun, Oyedotun, Kabir O., Mamba, Bhekie B., Bello, Olugbenga Solomon
Format Journal Article
LanguageEnglish
Published Elsevier B.V 15.10.2024
Subjects
Electrocatalysts
Energy conversion
Energy storage
Iron-based metal–organic frameworks
Iron-based metal–organic frameworks
Electrocatalysts
Energy conversion
Energy storage
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Abstract •Fe-MOF nanomaterials are efficient electrocatalysts for energy storage and conversion.•Recent advances in synthesis strategies and applications of Fe-MOFs were highlighted.•Overview of MOF materials, structural diversity and design of Fe-MOF were highlighted.•DFT calculations have prospect for detail understanding and mechanistic information of these materials.•Challenges and the corresponding promising strategies for improving the efficiency of Fe-MOF materials were presented. Renewable energy remainsa prominent research hotspotbecause of its potential to reduce the globalreliance on fossil fuels, which isexperiencing a significant decline. Additionally, it has become highly importantto address the pressing issue of greenhouse gas emissions in order to meet the rising demandsin population growth,industrial activities, increasingglobal climate change, and energy consumption. Iron-based metal–organic frameworks (Fe-MOFs) are currently progressive intelligent materials with multipurpose and adjustable properties for clean energy applications due to their arrays of intrinsic physicochemical and structural characteristics. Despite increasing growth designs and fabrication of Fe-MOFs and their derived materials for a wide range of electrocatalytic energy applications, there is currently no review that demonstrates these recent developments of the same for energy storage and conversion systems, thereby creating knowledge gaps in this field. This study presents recent developments in electrocatalytic applications of Fe-MOF nanomaterials for energy storage (covering batteries and supercapacitors), oxygen and hydrogen productions, alcohol oxidation, nitrogen reduction reaction (NRR), CO2 reduction reaction (CO2RR) under different categories of Fe-MOF nanomaterials involving the pristine MOF, Fe-MOF-based electrocatalyst materials, MOF-derived electrocatalyst materials, and Fe-MOF composite materials. Brief fundamental concepts covering overview of MOF materials, structural diversity and design of Fe-MOF-based constituents were highlighted before the new development in the field.This work also demonstrates the amazing advantages that MOF materials have over conventional electrocatalysts, as well as the superiority of Fe-MOF-materials over their pristine equivalents. The paucity of computational and new technological information in this subject inspired the need to evaluate the prospect of density functional theory (DFT) calculations for a detailed understanding and mechanistic study of these materials for future advancements. Lastly, we discussed some challenges and the corresponding promising strategies for improving the efficiency of Fe-MOF materials to achieve viable industrial feasibility for energy storage and conversion applications. The review serves as a wake-up call to the scientific community on the need to design and fabricate new Fe-MOFs for lasting solutions to the shortage of clean energy.
AbstractList •Fe-MOF nanomaterials are efficient electrocatalysts for energy storage and conversion.•Recent advances in synthesis strategies and applications of Fe-MOFs were highlighted.•Overview of MOF materials, structural diversity and design of Fe-MOF were highlighted.•DFT calculations have prospect for detail understanding and mechanistic information of these materials.•Challenges and the corresponding promising strategies for improving the efficiency of Fe-MOF materials were presented. Renewable energy remainsa prominent research hotspotbecause of its potential to reduce the globalreliance on fossil fuels, which isexperiencing a significant decline. Additionally, it has become highly importantto address the pressing issue of greenhouse gas emissions in order to meet the rising demandsin population growth,industrial activities, increasingglobal climate change, and energy consumption. Iron-based metal–organic frameworks (Fe-MOFs) are currently progressive intelligent materials with multipurpose and adjustable properties for clean energy applications due to their arrays of intrinsic physicochemical and structural characteristics. Despite increasing growth designs and fabrication of Fe-MOFs and their derived materials for a wide range of electrocatalytic energy applications, there is currently no review that demonstrates these recent developments of the same for energy storage and conversion systems, thereby creating knowledge gaps in this field. This study presents recent developments in electrocatalytic applications of Fe-MOF nanomaterials for energy storage (covering batteries and supercapacitors), oxygen and hydrogen productions, alcohol oxidation, nitrogen reduction reaction (NRR), CO2 reduction reaction (CO2RR) under different categories of Fe-MOF nanomaterials involving the pristine MOF, Fe-MOF-based electrocatalyst materials, MOF-derived electrocatalyst materials, and Fe-MOF composite materials. Brief fundamental concepts covering overview of MOF materials, structural diversity and design of Fe-MOF-based constituents were highlighted before the new development in the field.This work also demonstrates the amazing advantages that MOF materials have over conventional electrocatalysts, as well as the superiority of Fe-MOF-materials over their pristine equivalents. The paucity of computational and new technological information in this subject inspired the need to evaluate the prospect of density functional theory (DFT) calculations for a detailed understanding and mechanistic study of these materials for future advancements. Lastly, we discussed some challenges and the corresponding promising strategies for improving the efficiency of Fe-MOF materials to achieve viable industrial feasibility for energy storage and conversion applications. The review serves as a wake-up call to the scientific community on the need to design and fabricate new Fe-MOFs for lasting solutions to the shortage of clean energy.
ArticleNumber 215959
Author Olabintan, Abdullahi Biodun
Oyebamiji, Abel Kolawole
Adeola, Adedapo O.
Adegoke, Kayode Adesina
Oyedotun, Kabir O.
Bello, Olugbenga Solomon
Mamba, Bhekie B.
Author_xml – sequence: 1
  givenname: Kayode Adesina
  surname: Adegoke
  fullname: Adegoke, Kayode Adesina
  email: kwharyourday@gmail.com
  organization: Department of Industrial Chemistry, First Technical University, Ibadan, Nigeria
– sequence: 2
  givenname: Abel Kolawole
  surname: Oyebamiji
  fullname: Oyebamiji, Abel Kolawole
  email: abel.oyebamiji@bowen.edu.ng
  organization: Department of Chemistry and Industrial Chemistry, Bowen University, Iwo, Osun State, Nigeria
– sequence: 3
  givenname: Adedapo O.
  surname: Adeola
  fullname: Adeola, Adedapo O.
  email: adedapo.adeola@aaua.edu.ng
  organization: Department of Chemical Sciences, Adekunle Ajasin University, Akungba-Akoko, Ondo State, Nigeria
– sequence: 4
  givenname: Abdullahi Biodun
  surname: Olabintan
  fullname: Olabintan, Abdullahi Biodun
  email: deeunikchm@yahoo.com
  organization: Chemistry Department, King Fahd University of Petroleum & Minerals, Dhahran 31261, Saudi Arabia
– sequence: 5
  givenname: Kabir O.
  surname: Oyedotun
  fullname: Oyedotun, Kabir O.
  email: oyedoko@unisa.ac.za
  organization: College of Science, Engineering and Technology, University of South Africa, Florida Campus, Johannesburg 1710, South Africa
– sequence: 6
  givenname: Bhekie B.
  surname: Mamba
  fullname: Mamba, Bhekie B.
  email: mambabb@unisa.ac.za
  organization: College of Science, Engineering and Technology, University of South Africa, Florida Campus, Johannesburg 1710, South Africa
– sequence: 7
  givenname: Olugbenga Solomon
  surname: Bello
  fullname: Bello, Olugbenga Solomon
  email: osbello@lautech.edu.ng
  organization: Department of Pure and Applied Chemistry, Ladoke Akintola University of Technology, P.M.B. 4000, Ogbomoso, Nigeria
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Snippet •Fe-MOF nanomaterials are efficient electrocatalysts for energy storage and conversion.•Recent advances in synthesis strategies and applications of Fe-MOFs...
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SubjectTerms Electrocatalysts
Energy conversion
Energy storage
Iron-based metal–organic frameworks
Title Iron-based metal–organic frameworks and derivatives for electrochemical energy storage and conversion
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