Recent advances on heterojunction-based photocatalysts for the degradation of persistent organic pollutants

[Display omitted] •Heterojunctions are emerging as prospective candidates for the degradation of POPs.•The basic principles and the fabrication strategies were systematically discussed.•Recent heterojunction photodegradation of POPs and the mechanisms were appraised.•Challenges and perspectives faci...

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Published inChemical engineering journal (Lausanne, Switzerland : 1996) Vol. 426; p. 130617
Main Authors Xie, Linxuan, Du, Ting, Wang, Jing, Ma, Yiyue, Ni, Yongsheng, Liu, Zhaoli, Zhang, Liang, Yang, Chengyuan, Wang, Jianlong
Format Journal Article
LanguageEnglish
Published Elsevier B.V 15.12.2021
Subjects
Heterojunction
Photocatalyst
Photodegradation
POPs
Photodegradation
Photocatalyst
POPs
Heterojunction
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Abstract [Display omitted] •Heterojunctions are emerging as prospective candidates for the degradation of POPs.•The basic principles and the fabrication strategies were systematically discussed.•Recent heterojunction photodegradation of POPs and the mechanisms were appraised.•Challenges and perspectives facing heterojunction were insightfully elucidated. Photocatalysis has attracted a broad range of attention because of its ability of efficient solar energy utilization for environmental governance. Hence, abundant photocatalysts have been investigated continuously to meet the requirement of energy-supply issues. However, engineering photocatalysts with strong visible light-harvesting ability, efficient charge separation, and superior stability is imminently desired due to the low efficiency of photocatalytic reactions with an individual photocatalyst. Particularly the fabrication of heterostructured photocatalysts have conquered the aforementioned bottlenecks and displayed great potential in the field of contaminants degradation. Herein, we summarized the recent significant progress on the design of different heterostructured photocatalysts and their wide applications in persistent organic pollutants (POPs) degradation is highlighted. We firstly introduce the representative synthetic tactics, the charge transfer mechanism, and the categories. Thereafter we outline state-of-the-art heterostructured photocatalysts for the degradation of different types of POPs, in which the improvement of primary focus on the reason why the photocatalytic activity was high. Additionally, we proposed the ongoing challenges and perspectives of heterojunction photocatalytic systems.
AbstractList [Display omitted] •Heterojunctions are emerging as prospective candidates for the degradation of POPs.•The basic principles and the fabrication strategies were systematically discussed.•Recent heterojunction photodegradation of POPs and the mechanisms were appraised.•Challenges and perspectives facing heterojunction were insightfully elucidated. Photocatalysis has attracted a broad range of attention because of its ability of efficient solar energy utilization for environmental governance. Hence, abundant photocatalysts have been investigated continuously to meet the requirement of energy-supply issues. However, engineering photocatalysts with strong visible light-harvesting ability, efficient charge separation, and superior stability is imminently desired due to the low efficiency of photocatalytic reactions with an individual photocatalyst. Particularly the fabrication of heterostructured photocatalysts have conquered the aforementioned bottlenecks and displayed great potential in the field of contaminants degradation. Herein, we summarized the recent significant progress on the design of different heterostructured photocatalysts and their wide applications in persistent organic pollutants (POPs) degradation is highlighted. We firstly introduce the representative synthetic tactics, the charge transfer mechanism, and the categories. Thereafter we outline state-of-the-art heterostructured photocatalysts for the degradation of different types of POPs, in which the improvement of primary focus on the reason why the photocatalytic activity was high. Additionally, we proposed the ongoing challenges and perspectives of heterojunction photocatalytic systems.
ArticleNumber 130617
Author Ni, Yongsheng
Zhang, Liang
Liu, Zhaoli
Wang, Jianlong
Du, Ting
Yang, Chengyuan
Wang, Jing
Ma, Yiyue
Xie, Linxuan
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  givenname: Yongsheng
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  givenname: Zhaoli
  surname: Liu
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  givenname: Liang
  orcidid: 0000-0003-0320-9101
  surname: Zhang
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  email: wanglong79@nwsuaf.edu.cn
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Snippet [Display omitted] •Heterojunctions are emerging as prospective candidates for the degradation of POPs.•The basic principles and the fabrication strategies were...
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SubjectTerms Heterojunction
Photocatalyst
Photodegradation
POPs
Title Recent advances on heterojunction-based photocatalysts for the degradation of persistent organic pollutants
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