Multivalent metal catalysts in Fenton/Fenton-like oxidation system: A critical review

[Display omitted] •Multivalent metal catalysts in Fenton/Fenton-like oxidation system were reviewed.•Conversion of multivalent metal valence initiated the production of ROS.•Affecting factors of valence conversion of multivalent metal were summered.•Strategies for accelerating the recycle of valence...

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Published inChemical engineering journal (Lausanne, Switzerland : 1996) Vol. 466; p. 143147
Main Authors Liu, Yong, Wang, Jianlong
Format Journal Article
LanguageEnglish
Published Elsevier B.V 15.06.2023
Subjects
Advanced oxidation processes
Catalyst
Fenton oxidation
Multivalent metal
Reactive oxygen species
Advanced oxidation processes
Reactive oxygen species
Multivalent metal
Catalyst
Fenton oxidation
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Abstract [Display omitted] •Multivalent metal catalysts in Fenton/Fenton-like oxidation system were reviewed.•Conversion of multivalent metal valence initiated the production of ROS.•Affecting factors of valence conversion of multivalent metal were summered.•Strategies for accelerating the recycle of valence states were summered.•Formation and contribution to decontamination of high-valent metal were discussed. The Fenton/Fenton-like reaction is an advanced oxidation process, which is widely recognized for its efficient removal of recalcitrant organic contaminants. In Fenton/Fenton-like oxidation systems, multivalent metals are important catalysts, such as Fe, Cu, Co, Mn, Ce, Ag, Cr, Ru, W, Mo, V, Ti, etc., which can activate H2O2 to produce reactive oxygen species (ROS) by low-valent metal (Mn+) with reduction properties and high-valent metal (M(n+z)+) with oxidation properties due to the dual roles of H2O2 as reductant and oxidant. Moreover, Fenton/Fenton-like oxidation is a radical reaction process, in which the redox reaction between multivalent metals and radicals may occur. Therefore, the conversion and recycle of valence state of multivalent metals are crucial in the production of ROS and the degradation of organic contaminants. In this review, the recent advances in the conversion and recycle valence states of multivalent metals, including Fe3+/Fe2+, Cu2+/Cu+, Co3+/Co2+, Mn4+/Mn2+, Ce4+/Ce3+, Ru3+/Ru2+, Cr6+/Cr3+, Ti4+/Ti3+, Mo6+/Mo4+ and the like, were systematically reviewed. Firstly, the conversion and influencing factors of valence states of multivalent metals in Fenton processes were introduced; Secondly, the strategies for regenerating low-valent metals were summarized; Thirdly, the formation, determination methods and roles of high-valent metals in contaminant degradation were analyzed and discussed; Finally, the concluding remarks and future perspectives were proposed. This review could provide valuable information for the development of new catalysts of multivalent metals, deepen the understanding of the mechanisms of Fenton/Fenton-like processes and provide a reference for expanding the application of the multivalent metals catalytic Fenton/Fenton-like process in water and wastewater treatment.
AbstractList [Display omitted] •Multivalent metal catalysts in Fenton/Fenton-like oxidation system were reviewed.•Conversion of multivalent metal valence initiated the production of ROS.•Affecting factors of valence conversion of multivalent metal were summered.•Strategies for accelerating the recycle of valence states were summered.•Formation and contribution to decontamination of high-valent metal were discussed. The Fenton/Fenton-like reaction is an advanced oxidation process, which is widely recognized for its efficient removal of recalcitrant organic contaminants. In Fenton/Fenton-like oxidation systems, multivalent metals are important catalysts, such as Fe, Cu, Co, Mn, Ce, Ag, Cr, Ru, W, Mo, V, Ti, etc., which can activate H2O2 to produce reactive oxygen species (ROS) by low-valent metal (Mn+) with reduction properties and high-valent metal (M(n+z)+) with oxidation properties due to the dual roles of H2O2 as reductant and oxidant. Moreover, Fenton/Fenton-like oxidation is a radical reaction process, in which the redox reaction between multivalent metals and radicals may occur. Therefore, the conversion and recycle of valence state of multivalent metals are crucial in the production of ROS and the degradation of organic contaminants. In this review, the recent advances in the conversion and recycle valence states of multivalent metals, including Fe3+/Fe2+, Cu2+/Cu+, Co3+/Co2+, Mn4+/Mn2+, Ce4+/Ce3+, Ru3+/Ru2+, Cr6+/Cr3+, Ti4+/Ti3+, Mo6+/Mo4+ and the like, were systematically reviewed. Firstly, the conversion and influencing factors of valence states of multivalent metals in Fenton processes were introduced; Secondly, the strategies for regenerating low-valent metals were summarized; Thirdly, the formation, determination methods and roles of high-valent metals in contaminant degradation were analyzed and discussed; Finally, the concluding remarks and future perspectives were proposed. This review could provide valuable information for the development of new catalysts of multivalent metals, deepen the understanding of the mechanisms of Fenton/Fenton-like processes and provide a reference for expanding the application of the multivalent metals catalytic Fenton/Fenton-like process in water and wastewater treatment.
ArticleNumber 143147
Author Wang, Jianlong
Liu, Yong
Author_xml – sequence: 1
  givenname: Yong
  surname: Liu
  fullname: Liu, Yong
  organization: College of Chemistry and Materials Science, Sichuan Normal University, Chengdu 610066, China
– sequence: 2
  givenname: Jianlong
  orcidid: 0000-0001-9572-851X
  surname: Wang
  fullname: Wang, Jianlong
  email: wangjl@tsinghua.edu.cn
  organization: Laboratory of Environmental Technology, INET, Tsinghua University, Beijing 100084, China
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Snippet [Display omitted] •Multivalent metal catalysts in Fenton/Fenton-like oxidation system were reviewed.•Conversion of multivalent metal valence initiated the...
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StartPage 143147
SubjectTerms Advanced oxidation processes
Catalyst
Fenton oxidation
Multivalent metal
Reactive oxygen species
Title Multivalent metal catalysts in Fenton/Fenton-like oxidation system: A critical review
URI https://dx.doi.org/10.1016/j.cej.2023.143147
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