Self-assembled ZnO-carbon dots anode materials for high performance nickel-zinc alkaline batteries
After incorporation of a few Carbon Dots (CDs), ZnO anodes process thin carbon shells, refined microstructures and special univalent zinc sites, which result in better reactivity, higher corrosion resistance, more effective electron paths to enhance electrochemical performance in high capacity, exce...
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| Published in | Chemical engineering journal (Lausanne, Switzerland : 1996) Vol. 425; p. 130660 |
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| Main Authors | , , , , , , , , , , |
| Format | Journal Article |
| Language | English |
| Published |
Elsevier B.V
01.12.2021
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| Subjects | |
| Online Access | Get full text |
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| Abstract | After incorporation of a few Carbon Dots (CDs), ZnO anodes process thin carbon shells, refined microstructures and special univalent zinc sites, which result in better reactivity, higher corrosion resistance, more effective electron paths to enhance electrochemical performance in high capacity, excellent rate capability and long cycling stability in the Ni-Zn alkaline battery.
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•1. CDs efficiently control morphology of ZnO for sufficient electrochemical reactions.•2. With the assistance of CDs, ZnO will process conformal carbon shells with few layers.•3. Univalent zinc sites constructed by CDs play a key role during charging process.
The development of high-performance nickel-zinc (Ni-Zn) alkaline batteries is mainly plagued by short life span and poor rate performance of ZnO anode materials. To improve the cycling stability and rate capability of Ni-Zn batteries, carbon dots (CDs) are employed to construct clustered ZnO-CDs nanocomposites, coating ZnO with protective shells of carbon layers and providing electron paths to enhance conductivity of the nanocomposites. Univalent zinc species are found at the interfaces between CDs derivatives and ZnO, which are embedded in the nanoclusters and protected well by carbon coating. Theoretical calculations show univalent zinc species change the electronic structures of ZnO surface, so as to accelerate the charging process of ZnO anode materials. Such ZnO-CDs derived nanocomposites exhibit excellent rate capability (95.3%, 84.7% and 75.0% of capacity retention rate at 2, 5 and 10 A g−1, respectively) and outstanding cycling stability with 92.0% of capacity retention rate after 5000 cycles, which is far better than ZnO based anodes without the protection of CDs (39.1% retention rate from 1 to 10 A g−1 and 71.6% of capacity retention rate after 500 cycles). |
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| AbstractList | After incorporation of a few Carbon Dots (CDs), ZnO anodes process thin carbon shells, refined microstructures and special univalent zinc sites, which result in better reactivity, higher corrosion resistance, more effective electron paths to enhance electrochemical performance in high capacity, excellent rate capability and long cycling stability in the Ni-Zn alkaline battery.
[Display omitted]
•1. CDs efficiently control morphology of ZnO for sufficient electrochemical reactions.•2. With the assistance of CDs, ZnO will process conformal carbon shells with few layers.•3. Univalent zinc sites constructed by CDs play a key role during charging process.
The development of high-performance nickel-zinc (Ni-Zn) alkaline batteries is mainly plagued by short life span and poor rate performance of ZnO anode materials. To improve the cycling stability and rate capability of Ni-Zn batteries, carbon dots (CDs) are employed to construct clustered ZnO-CDs nanocomposites, coating ZnO with protective shells of carbon layers and providing electron paths to enhance conductivity of the nanocomposites. Univalent zinc species are found at the interfaces between CDs derivatives and ZnO, which are embedded in the nanoclusters and protected well by carbon coating. Theoretical calculations show univalent zinc species change the electronic structures of ZnO surface, so as to accelerate the charging process of ZnO anode materials. Such ZnO-CDs derived nanocomposites exhibit excellent rate capability (95.3%, 84.7% and 75.0% of capacity retention rate at 2, 5 and 10 A g−1, respectively) and outstanding cycling stability with 92.0% of capacity retention rate after 5000 cycles, which is far better than ZnO based anodes without the protection of CDs (39.1% retention rate from 1 to 10 A g−1 and 71.6% of capacity retention rate after 500 cycles). |
| ArticleNumber | 130660 |
| Author | Chen, Liwei Zhang, Yi-Xiao Xiong, Huan-Ming Wei, Ji-Shi Liu, Xi Niu, Xiao-Qing Zhao, Xiao Huang, Jian-Hang Zhu, Ze-Yang Wang, Yong-Gang Song, Tian-Bing |
| Author_xml | – sequence: 1 givenname: Ji-Shi surname: Wei fullname: Wei, Ji-Shi organization: Department of Chemistry, Shanghai Key Laboratory of Molecular Catalysis and Innovative Materials, Laboratory of Advanced Materials, Fudan University, Shanghai 200438, PR China – sequence: 2 givenname: Ze-Yang surname: Zhu fullname: Zhu, Ze-Yang organization: Department of Chemistry, Shanghai Key Laboratory of Molecular Catalysis and Innovative Materials, Laboratory of Advanced Materials, Fudan University, Shanghai 200438, PR China – sequence: 3 givenname: Xiao surname: Zhao fullname: Zhao, Xiao organization: Institute for Computation in Molecular and Materials Science, School of Chemical Engineering, Nanjing University of Science and Technology, Nanjing 210094, PR China – sequence: 4 givenname: Tian-Bing surname: Song fullname: Song, Tian-Bing organization: Department of Chemistry, Shanghai Key Laboratory of Molecular Catalysis and Innovative Materials, Laboratory of Advanced Materials, Fudan University, Shanghai 200438, PR China – sequence: 5 givenname: Jian-Hang surname: Huang fullname: Huang, Jian-Hang organization: Department of Chemistry, Shanghai Key Laboratory of Molecular Catalysis and Innovative Materials, Laboratory of Advanced Materials, Fudan University, Shanghai 200438, PR China – sequence: 6 givenname: Yi-Xiao surname: Zhang fullname: Zhang, Yi-Xiao organization: School of Chemistry and Chemical Engineering, In-situ Center for Physical Science, and Frontiers Science Center for Transformative Molecules, Shanghai Jiao Tong University, Shanghai 200240, PR China – sequence: 7 givenname: Xi surname: Liu fullname: Liu, Xi organization: School of Chemistry and Chemical Engineering, In-situ Center for Physical Science, and Frontiers Science Center for Transformative Molecules, Shanghai Jiao Tong University, Shanghai 200240, PR China – sequence: 8 givenname: Liwei surname: Chen fullname: Chen, Liwei organization: School of Chemistry and Chemical Engineering, In-situ Center for Physical Science, and Frontiers Science Center for Transformative Molecules, Shanghai Jiao Tong University, Shanghai 200240, PR China – sequence: 9 givenname: Xiao-Qing surname: Niu fullname: Niu, Xiao-Qing organization: Department of Chemistry, Shanghai Key Laboratory of Molecular Catalysis and Innovative Materials, Laboratory of Advanced Materials, Fudan University, Shanghai 200438, PR China – sequence: 10 givenname: Yong-Gang surname: Wang fullname: Wang, Yong-Gang organization: Department of Chemistry, Shanghai Key Laboratory of Molecular Catalysis and Innovative Materials, Laboratory of Advanced Materials, Fudan University, Shanghai 200438, PR China – sequence: 11 givenname: Huan-Ming surname: Xiong fullname: Xiong, Huan-Ming email: hmxiong@fudan.edu.cn organization: Department of Chemistry, Shanghai Key Laboratory of Molecular Catalysis and Innovative Materials, Laboratory of Advanced Materials, Fudan University, Shanghai 200438, PR China |
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| Keywords | Carbon dots Univalent Zinc ZnO anode Surface coating Nickel-zinc alkaline battery |
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