Bimetallic metal–organic frameworks and MOF-derived composites: Recent progress on electro- and photoelectrocatalytic applications

[Display omitted] •The advantages of BMOFs and their composites are summarized and discussed.•BMOFs and their composites exhibit high electro/photoelectrocatalytic properties.•We investigated the current problems and future solutions of BMOFs.•The challenges of BMOFs for electro/photoelectrocatalyst...

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Published inCoordination chemistry reviews Vol. 451; p. 214264
Main Authors Zhou, Yingtang, Abazari, Reza, Chen, Jing, Tahir, Muhammad, Kumar, Anuj, Ikreedeegh, Riyadh Ramadhan, Rani, Ekta, Singh, Harishchandra, Kirillov, Alexander M.
Format Journal Article
LanguageEnglish
Published Elsevier B.V 15.01.2022
Subjects
Composites
Electrocatalysis
Metal-organic frameworks
Oxygen evolution reaction
Photoelectrocatalysis
Synergic effect
Electrocatalysis
Photoelectrocatalysis
Composites
Oxygen evolution reaction
Metal-organic frameworks
Synergic effect
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Abstract [Display omitted] •The advantages of BMOFs and their composites are summarized and discussed.•BMOFs and their composites exhibit high electro/photoelectrocatalytic properties.•We investigated the current problems and future solutions of BMOFs.•The challenges of BMOFs for electro/photoelectrocatalysts are summarized.•This is the first review dedicated to BMOFs for electro/photoelectrocatalysts. Owing to the growing demand in areas such as energy, environmental science, electro- and photoelectrocatalysis, different reactions such as HER (hydrogen evolution), OER (oxygen evolution), ORR (oxygen reduction), and CO2RR (CO2 reduction) represent attractive strategies to overcome the challenges in sustainable energy conversion and usage. The competition for introducing catalysts with higher performance and cost-efficiency in comparison to the previous systems based on noble metals is one of the most interesting directions in this field. By merging the advantages of inorganic and organic materials, MOFs (metal–organic frameworks) have gained an ample attention as highly versatile electro- and photoelectrocatalytic platforms. This is governed by the intricate features of MOFs including extraordinary surface area, exceptional porosity, tailorable pore size, vast structural and chemical tunability, and pre- and post-synthesis structural modifiability. In contrast to monometallic compounds, bimetallic MOFs (BMOFs) and their composites offer many advantages, including improved electrical conductivity, extended active sites, high charge capacity, and adjustable electrochemical activity. Metal-organic frameworks can also be combined with other electrochemically active materials, resulting in advanced composites with large specific area, increased electrical conductivity, and superiour dispersion. Besides, some BMOFs show an enhanced electrocatalytic activity under light irradiation, thus permitting their application as photoelectrocatalysts. The present review summarizes the state-of-the-art on bimetallic MOFs and derived composites for the main current types of electro- and photoelectrocatalytic applications. The study also aims to highlight the challenges and opportunities in this area, with a focus on future perspectives of such multimetallic compounds and materials, with a particular emphasis in the field of energy and electrophotocatalysis.
AbstractList [Display omitted] •The advantages of BMOFs and their composites are summarized and discussed.•BMOFs and their composites exhibit high electro/photoelectrocatalytic properties.•We investigated the current problems and future solutions of BMOFs.•The challenges of BMOFs for electro/photoelectrocatalysts are summarized.•This is the first review dedicated to BMOFs for electro/photoelectrocatalysts. Owing to the growing demand in areas such as energy, environmental science, electro- and photoelectrocatalysis, different reactions such as HER (hydrogen evolution), OER (oxygen evolution), ORR (oxygen reduction), and CO2RR (CO2 reduction) represent attractive strategies to overcome the challenges in sustainable energy conversion and usage. The competition for introducing catalysts with higher performance and cost-efficiency in comparison to the previous systems based on noble metals is one of the most interesting directions in this field. By merging the advantages of inorganic and organic materials, MOFs (metal–organic frameworks) have gained an ample attention as highly versatile electro- and photoelectrocatalytic platforms. This is governed by the intricate features of MOFs including extraordinary surface area, exceptional porosity, tailorable pore size, vast structural and chemical tunability, and pre- and post-synthesis structural modifiability. In contrast to monometallic compounds, bimetallic MOFs (BMOFs) and their composites offer many advantages, including improved electrical conductivity, extended active sites, high charge capacity, and adjustable electrochemical activity. Metal-organic frameworks can also be combined with other electrochemically active materials, resulting in advanced composites with large specific area, increased electrical conductivity, and superiour dispersion. Besides, some BMOFs show an enhanced electrocatalytic activity under light irradiation, thus permitting their application as photoelectrocatalysts. The present review summarizes the state-of-the-art on bimetallic MOFs and derived composites for the main current types of electro- and photoelectrocatalytic applications. The study also aims to highlight the challenges and opportunities in this area, with a focus on future perspectives of such multimetallic compounds and materials, with a particular emphasis in the field of energy and electrophotocatalysis.
ArticleNumber 214264
Author Abazari, Reza
Ikreedeegh, Riyadh Ramadhan
Tahir, Muhammad
Singh, Harishchandra
Kirillov, Alexander M.
Rani, Ekta
Zhou, Yingtang
Kumar, Anuj
Chen, Jing
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  givenname: Yingtang
  orcidid: 0000-0002-8678-295X
  surname: Zhou
  fullname: Zhou, Yingtang
  email: zhouyingtang@zjou.edu.cn
  organization: National Engineering Research Center for Marine Aquaculture, Marine Science and Technology College, Zhejiang Ocean University, Zhoushan, Zhejiang Province 316004, China
– sequence: 2
  givenname: Reza
  surname: Abazari
  fullname: Abazari, Reza
  email: reza.abazari@modares.ac.ir
  organization: National Engineering Research Center for Marine Aquaculture, Marine Science and Technology College, Zhejiang Ocean University, Zhoushan, Zhejiang Province 316004, China
– sequence: 3
  givenname: Jing
  surname: Chen
  fullname: Chen, Jing
  organization: National Engineering Research Center for Marine Aquaculture, Marine Science and Technology College, Zhejiang Ocean University, Zhoushan, Zhejiang Province 316004, China
– sequence: 4
  givenname: Muhammad
  orcidid: 0000-0002-2937-5645
  surname: Tahir
  fullname: Tahir, Muhammad
  email: muhammad.tahir@uaeu.ac.ae
  organization: Chemical Reaction Engineering Group (CREG), School of Chemical and Energy Engineering, Universiti Teknologi Malaysia, Johor Bahru 81310, Johor, Malaysia
– sequence: 5
  givenname: Anuj
  surname: Kumar
  fullname: Kumar, Anuj
  email: anuj.kumar@gla.ac.in
  organization: Department of Chemistry, Institute of Humanities and Applied Science, GLA University, Mathura 281406, India
– sequence: 6
  givenname: Riyadh Ramadhan
  surname: Ikreedeegh
  fullname: Ikreedeegh, Riyadh Ramadhan
  organization: Chemical Reaction Engineering Group (CREG), School of Chemical and Energy Engineering, Universiti Teknologi Malaysia, Johor Bahru 81310, Johor, Malaysia
– sequence: 7
  givenname: Ekta
  orcidid: 0000-0002-6933-9892
  surname: Rani
  fullname: Rani, Ekta
  email: Ekta.Rani@oulu.fi
  organization: Nano and Molecular Systems Research Unit, University of Oulu, FIN-90014, Finland
– sequence: 8
  givenname: Harishchandra
  orcidid: 0000-0001-7754-5648
  surname: Singh
  fullname: Singh, Harishchandra
  organization: Nano and Molecular Systems Research Unit, University of Oulu, FIN-90014, Finland
– sequence: 9
  givenname: Alexander M.
  surname: Kirillov
  fullname: Kirillov, Alexander M.
  email: kirillov@tecnico.ulisboa.pt
  organization: Centro de Química Estrutural and Departamento de Engenharia Química, Instituto Superior Técnico, Universidade de Lisboa, Av. Rovisco Pais, 1049-001 Lisbon, Portugal
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Snippet [Display omitted] •The advantages of BMOFs and their composites are summarized and discussed.•BMOFs and their composites exhibit high...
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SubjectTerms Composites
Electrocatalysis
Metal-organic frameworks
Oxygen evolution reaction
Photoelectrocatalysis
Synergic effect
Title Bimetallic metal–organic frameworks and MOF-derived composites: Recent progress on electro- and photoelectrocatalytic applications
URI https://dx.doi.org/10.1016/j.ccr.2021.214264
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