High-performance monoclinic WO3 nanospheres with the novel NH4+ diffusion behaviors for aqueous ammonium-ion batteries
[Display omitted] •The facile and controllable synthesis for monoclinic WO3 nanospheres.•The novel three-dimensional equilibrium diffusion behaviors for monoclinic WO3.•The continuous geometric evolutions of hydrogen bonds for monoclinic WO3.•WO3 revealed fast kinetics and durable stability for aque...
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| Published in | Chemical engineering journal (Lausanne, Switzerland : 1996) Vol. 458; p. 141381 |
|---|---|
| Main Authors | , , , , , |
| Format | Journal Article |
| Language | English |
| Published |
Elsevier B.V
15.02.2023
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| Subjects | |
| Online Access | Get full text |
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| Abstract | [Display omitted]
•The facile and controllable synthesis for monoclinic WO3 nanospheres.•The novel three-dimensional equilibrium diffusion behaviors for monoclinic WO3.•The continuous geometric evolutions of hydrogen bonds for monoclinic WO3.•WO3 revealed fast kinetics and durable stability for aqueous ammonium-ion batteries.
Aqueous ammonium-ion batteries (AAIBs) have attracted tremendous attentions due to their plentiful resources, inherent security and environmental friendliness. From the first-principles calculations and ex-situ measurements, monoclinic WO3 revealed the three-dimensional equilibrium diffusion behaviors during the electrochemical processes, and the novel evolution processes of reversible building/breaking between geometric hydrogen bonds and traditional linear hydrogen bonds. Specifically, monoclinic WO3 delivered a high specific capacity of 150.6 mAh g-1 at the current density of 0.1 A g-1, and exhibited excellent rate capability of 48 mAh g-1 at the current density of 5.0 A g-1 and outstanding cycling stability of 86.6 % capacity retention after 500 cycles. Furthermore, the ammonium-ion full batteries based on the monoclinic WO3 anode and γ-MnO2 cathode achieved a perfect energy density of 64.9 Wh kg-1 and an extreme ultra-long lifespan with 95.4 % capacity retention after 5000 cycles at the current density of 3.0 A g-1. Thus, the novel insights on NH4+ diffusion behaviors and the evolution mechanisms of hydrogen bonds could promote the development of the practical applications for monoclinic WO3 in aqueous ammonium-ion batteries. |
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| AbstractList | [Display omitted]
•The facile and controllable synthesis for monoclinic WO3 nanospheres.•The novel three-dimensional equilibrium diffusion behaviors for monoclinic WO3.•The continuous geometric evolutions of hydrogen bonds for monoclinic WO3.•WO3 revealed fast kinetics and durable stability for aqueous ammonium-ion batteries.
Aqueous ammonium-ion batteries (AAIBs) have attracted tremendous attentions due to their plentiful resources, inherent security and environmental friendliness. From the first-principles calculations and ex-situ measurements, monoclinic WO3 revealed the three-dimensional equilibrium diffusion behaviors during the electrochemical processes, and the novel evolution processes of reversible building/breaking between geometric hydrogen bonds and traditional linear hydrogen bonds. Specifically, monoclinic WO3 delivered a high specific capacity of 150.6 mAh g-1 at the current density of 0.1 A g-1, and exhibited excellent rate capability of 48 mAh g-1 at the current density of 5.0 A g-1 and outstanding cycling stability of 86.6 % capacity retention after 500 cycles. Furthermore, the ammonium-ion full batteries based on the monoclinic WO3 anode and γ-MnO2 cathode achieved a perfect energy density of 64.9 Wh kg-1 and an extreme ultra-long lifespan with 95.4 % capacity retention after 5000 cycles at the current density of 3.0 A g-1. Thus, the novel insights on NH4+ diffusion behaviors and the evolution mechanisms of hydrogen bonds could promote the development of the practical applications for monoclinic WO3 in aqueous ammonium-ion batteries. |
| ArticleNumber | 141381 |
| Author | Luo, Jinhua Wen, Xiaoyu Zhang, Changfan Chen, Han Xiang, Kaixiong Zhou, Wei |
| Author_xml | – sequence: 1 givenname: Xiaoyu surname: Wen fullname: Wen, Xiaoyu organization: Hunan University of Technology, Zhuzhou, Hunan 412007, PR China – sequence: 2 givenname: Jinhua surname: Luo fullname: Luo, Jinhua organization: Changsha University, Changsha 410022, PR China – sequence: 3 givenname: Kaixiong surname: Xiang fullname: Xiang, Kaixiong organization: Hunan University of Technology, Zhuzhou, Hunan 412007, PR China – sequence: 4 givenname: Wei surname: Zhou fullname: Zhou, Wei organization: Changsha University, Changsha 410022, PR China – sequence: 5 givenname: Changfan surname: Zhang fullname: Zhang, Changfan email: zhangchangfan@263.net organization: Hunan University of Technology, Zhuzhou, Hunan 412007, PR China – sequence: 6 givenname: Han surname: Chen fullname: Chen, Han email: lzdxnchh@126.com organization: Changsha University, Changsha 410022, PR China |
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•The facile and controllable synthesis for monoclinic WO3 nanospheres.•The novel three-dimensional equilibrium diffusion behaviors for... |
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| SourceType | Enrichment Source Index Database Publisher |
| StartPage | 141381 |
| SubjectTerms | Ammonium-ion battery Aqueous battery Hydrogen bonds chemistry Monoclinic WO3 Trifurcated hydrogen bond |
| Title | High-performance monoclinic WO3 nanospheres with the novel NH4+ diffusion behaviors for aqueous ammonium-ion batteries |
| URI | https://dx.doi.org/10.1016/j.cej.2023.141381 |
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