Photocatalytic degradation of tetracycline antibiotic by a novel Bi2Sn2O7/Bi2MoO6 S-scheme heterojunction: Performance, mechanism insight and toxicity assessment
[Display omitted] •0D/3D Bi2Sn2O7/Bi2MoO6 S-scheme heterojunction was constructed.•The heterojunction exhibited excellent photocatalytic performance for antibiotics.•A plausible degradation pathway for TC was proposed.•S-scheme heterojunction largely boosted charge separation and ROS production. The...
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| Published in | Chemical engineering journal (Lausanne, Switzerland : 1996) Vol. 429; p. 132519 |
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| Main Authors | , , , , , , , , , |
| Format | Journal Article |
| Language | English |
| Published |
Elsevier B.V
01.02.2022
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| Subjects | |
| Online Access | Get full text |
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| Abstract | [Display omitted]
•0D/3D Bi2Sn2O7/Bi2MoO6 S-scheme heterojunction was constructed.•The heterojunction exhibited excellent photocatalytic performance for antibiotics.•A plausible degradation pathway for TC was proposed.•S-scheme heterojunction largely boosted charge separation and ROS production.
The fabrication of step-scheme (S-scheme) heterojunction with superior redox capability has been emerging as a prospective strategy for environmental remediation. Herein, novel Bi2Sn2O7/Bi2MoO6 S-scheme heterojunctions have been fabricated via in-situ anchoring Bi2Sn2O7 nanoparticles on Bi2MoO6 microspheres. The optimized Bi2Sn2O7/Bi2MoO6 (BSO/BMO-6%) attains the highest reaction rate constant (k) in the degradation of tetracycline hydrochloride (TC, k = 0.0397 min−1), which is 3.62 folds higher than that of pristine Bi2MoO6. Such an improvement is originated from more exposed active sites, higher photo-excited charge separation efficiency, superior redox ability, and efficient production of reactive h+, •OH and •O2–. Besides, Bi2Sn2O7/Bi2MoO6 could efficiently degrade the TC antibiotic in actual water matrix. Significantly, the toxicity evaluation verifies the nontoxicity of Bi2Sn2O7/Bi2MoO6. Moreover, the degradation pathways of TC are determined and the toxicity of degradation intermediates is appraised by using HPLC-MS spectra and QSAR prediction. A possible photocatalytic mechanism over S-scheme Bi2Sn2O7/Bi2MoO6 has been elucidated based on experimental studies combined with density functional theory (DFT) calculations. This work offers new insights for the design of high-performance S-scheme heterojunctions for environmental remediation. |
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| AbstractList | [Display omitted]
•0D/3D Bi2Sn2O7/Bi2MoO6 S-scheme heterojunction was constructed.•The heterojunction exhibited excellent photocatalytic performance for antibiotics.•A plausible degradation pathway for TC was proposed.•S-scheme heterojunction largely boosted charge separation and ROS production.
The fabrication of step-scheme (S-scheme) heterojunction with superior redox capability has been emerging as a prospective strategy for environmental remediation. Herein, novel Bi2Sn2O7/Bi2MoO6 S-scheme heterojunctions have been fabricated via in-situ anchoring Bi2Sn2O7 nanoparticles on Bi2MoO6 microspheres. The optimized Bi2Sn2O7/Bi2MoO6 (BSO/BMO-6%) attains the highest reaction rate constant (k) in the degradation of tetracycline hydrochloride (TC, k = 0.0397 min−1), which is 3.62 folds higher than that of pristine Bi2MoO6. Such an improvement is originated from more exposed active sites, higher photo-excited charge separation efficiency, superior redox ability, and efficient production of reactive h+, •OH and •O2–. Besides, Bi2Sn2O7/Bi2MoO6 could efficiently degrade the TC antibiotic in actual water matrix. Significantly, the toxicity evaluation verifies the nontoxicity of Bi2Sn2O7/Bi2MoO6. Moreover, the degradation pathways of TC are determined and the toxicity of degradation intermediates is appraised by using HPLC-MS spectra and QSAR prediction. A possible photocatalytic mechanism over S-scheme Bi2Sn2O7/Bi2MoO6 has been elucidated based on experimental studies combined with density functional theory (DFT) calculations. This work offers new insights for the design of high-performance S-scheme heterojunctions for environmental remediation. |
| ArticleNumber | 132519 |
| Author | Wang, Yaning Zhao, Wei Li, Shijie Zhang, Huiqiu Wang, Chunchun Liu, Yanping Cai, Mingjie Guo, Yang Wang, Zhaohui Chen, Xiaobo |
| Author_xml | – sequence: 1 givenname: Shijie surname: Li fullname: Li, Shijie organization: Institute of Innovation & Application, Key Laboratory of Health Risk Factors for Seafood of Zhejiang Province, National Engineering Research Center for Marine Aquaculture, Zhejiang Ocean University, Zhoushan, Zhejiang Province, 316022, China – sequence: 2 givenname: Chunchun surname: Wang fullname: Wang, Chunchun organization: Institute of Innovation & Application, Key Laboratory of Health Risk Factors for Seafood of Zhejiang Province, National Engineering Research Center for Marine Aquaculture, Zhejiang Ocean University, Zhoushan, Zhejiang Province, 316022, China – sequence: 3 givenname: Yanping surname: Liu fullname: Liu, Yanping organization: Institute of Innovation & Application, Key Laboratory of Health Risk Factors for Seafood of Zhejiang Province, National Engineering Research Center for Marine Aquaculture, Zhejiang Ocean University, Zhoushan, Zhejiang Province, 316022, China – sequence: 4 givenname: Mingjie surname: Cai fullname: Cai, Mingjie organization: Institute of Innovation & Application, Key Laboratory of Health Risk Factors for Seafood of Zhejiang Province, National Engineering Research Center for Marine Aquaculture, Zhejiang Ocean University, Zhoushan, Zhejiang Province, 316022, China – sequence: 5 givenname: Yaning surname: Wang fullname: Wang, Yaning organization: Institute of Innovation & Application, Key Laboratory of Health Risk Factors for Seafood of Zhejiang Province, National Engineering Research Center for Marine Aquaculture, Zhejiang Ocean University, Zhoushan, Zhejiang Province, 316022, China – sequence: 6 givenname: Huiqiu surname: Zhang fullname: Zhang, Huiqiu organization: Institute of Innovation & Application, Key Laboratory of Health Risk Factors for Seafood of Zhejiang Province, National Engineering Research Center for Marine Aquaculture, Zhejiang Ocean University, Zhoushan, Zhejiang Province, 316022, China – sequence: 7 givenname: Yang surname: Guo fullname: Guo, Yang organization: State Key Laboratory of Pollution Control and Resource Reuse, School of the Environment, Nanjing University, Nanjing 210023, PR China – sequence: 8 givenname: Wei surname: Zhao fullname: Zhao, Wei email: lmjzhaowei@foxmail.com organization: School of Materials Engineering, Changshu Institute of Technology, Changshu, China – sequence: 9 givenname: Zhaohui surname: Wang fullname: Wang, Zhaohui email: zhwang@des.ecnu.edu.cn organization: Shanghai Key Lab for Urban Ecological Processes and Eco-Restoration, School of Ecological and Environmental Sciences, East China Normal University, Shanghai 200241, China – sequence: 10 givenname: Xiaobo surname: Chen fullname: Chen, Xiaobo email: chenxiaobo@umkc.edu organization: Department of Chemistry, University of Missouri – Kansas City, MO 64110, USA |
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•0D/3D Bi2Sn2O7/Bi2MoO6 S-scheme heterojunction was constructed.•The heterojunction exhibited excellent photocatalytic performance for... |
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| SubjectTerms | Antibiotic degradation Bi2Sn2O7/Bi2MoO6 S-scheme heterojunction Toxicity assessment Visible-light photocatalysis |
| Title | Photocatalytic degradation of tetracycline antibiotic by a novel Bi2Sn2O7/Bi2MoO6 S-scheme heterojunction: Performance, mechanism insight and toxicity assessment |
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