Metal-based catalysts for persulfate and peroxymonosulfate activation in heterogeneous ways: A review

[Display omitted] •Heterogeneous metal-catalysts for oxidants activation were presented.•The activation mechanisms involved in catalysts/oxidants system were elucidated.•The prospects and strategies for the sustainable application were proposed. A growing number of emerging organic contaminants asso...

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Published inChemical engineering journal (Lausanne, Switzerland : 1996) Vol. 429; p. 132323
Main Authors Zheng, Xiaoxian, Niu, Xiaojun, Zhang, Dongqing, Lv, Mengyu, Ye, Xingyao, Ma, Jinling, Lin, Zhang, Fu, Mingli
Format Journal Article
LanguageEnglish
Published Elsevier B.V 01.02.2022
Subjects
Heterogeneous
Metal-based catalysts
Peroxymonosulfate
Persulfate
Sulfate radical-based advanced oxidation processes
Metal-based catalysts
Heterogeneous
Sulfate radical-based advanced oxidation processes
Peroxymonosulfate
Persulfate
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Abstract [Display omitted] •Heterogeneous metal-catalysts for oxidants activation were presented.•The activation mechanisms involved in catalysts/oxidants system were elucidated.•The prospects and strategies for the sustainable application were proposed. A growing number of emerging organic contaminants associated with the potential risks for ecosystem and human health are frequently detected in environment. Sulfate radical-based advanced oxidation processes have attracted increasing attention during the past decades, owing to their high reactivity and oxidation capability of a wide range of toxic and non-biodegradable organic compounds. Metal-based materials have been proven to be effective heterogeneous catalysts for activating persulfate to degrade many refractory organic pollutants. This article reviews the up-to-date research progresses on various heterogeneous metal-based catalysts for persulfate (PS) and peroxymonosulfate (PMS) activation, including single metal and mixed metal catalysts. The activation mechanisms of these catalysts and their fundamental behaviors in PS/PMS activation are emphatically elucidated, in which contaminants can be eliminated through radical and/or non-radical reaction pathways. In addition, an in-depth discussion about metal composite namely metal spinel, metallic glasses and other metal hybrids in PS or PMS systems for organic degradation and possible environmental applications are presented. Finally, the perspectives on the metal-based PS/PMS activation method and their remediation potential for recalcitrant compounds in practical application are also proposed.
AbstractList [Display omitted] •Heterogeneous metal-catalysts for oxidants activation were presented.•The activation mechanisms involved in catalysts/oxidants system were elucidated.•The prospects and strategies for the sustainable application were proposed. A growing number of emerging organic contaminants associated with the potential risks for ecosystem and human health are frequently detected in environment. Sulfate radical-based advanced oxidation processes have attracted increasing attention during the past decades, owing to their high reactivity and oxidation capability of a wide range of toxic and non-biodegradable organic compounds. Metal-based materials have been proven to be effective heterogeneous catalysts for activating persulfate to degrade many refractory organic pollutants. This article reviews the up-to-date research progresses on various heterogeneous metal-based catalysts for persulfate (PS) and peroxymonosulfate (PMS) activation, including single metal and mixed metal catalysts. The activation mechanisms of these catalysts and their fundamental behaviors in PS/PMS activation are emphatically elucidated, in which contaminants can be eliminated through radical and/or non-radical reaction pathways. In addition, an in-depth discussion about metal composite namely metal spinel, metallic glasses and other metal hybrids in PS or PMS systems for organic degradation and possible environmental applications are presented. Finally, the perspectives on the metal-based PS/PMS activation method and their remediation potential for recalcitrant compounds in practical application are also proposed.
ArticleNumber 132323
Author Lv, Mengyu
Fu, Mingli
Zheng, Xiaoxian
Niu, Xiaojun
Lin, Zhang
Zhang, Dongqing
Ye, Xingyao
Ma, Jinling
Author_xml – sequence: 1
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  surname: Zheng
  fullname: Zheng, Xiaoxian
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– sequence: 2
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  surname: Niu
  fullname: Niu, Xiaojun
  email: xjniu@scut.edu.cn, scutenv@outlook.com
  organization: School of Environment and Energy, South China University of Technology, Guangzhou 510006, PR China
– sequence: 3
  givenname: Dongqing
  surname: Zhang
  fullname: Zhang, Dongqing
  email: dqzhang3377@outlook.com
  organization: College of Environmental Science and Engineering, Guangdong University of Petrochemical Technology, Maoming 525000, PR China
– sequence: 4
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  fullname: Lv, Mengyu
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  fullname: Ma, Jinling
  organization: School of Environment and Energy, South China University of Technology, Guangzhou 510006, PR China
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  organization: School of Environment and Energy, South China University of Technology, Guangzhou 510006, PR China
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  givenname: Mingli
  surname: Fu
  fullname: Fu, Mingli
  organization: School of Environment and Energy, South China University of Technology, Guangzhou 510006, PR China
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Snippet [Display omitted] •Heterogeneous metal-catalysts for oxidants activation were presented.•The activation mechanisms involved in catalysts/oxidants system were...
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StartPage 132323
SubjectTerms Heterogeneous
Metal-based catalysts
Peroxymonosulfate
Persulfate
Sulfate radical-based advanced oxidation processes
Title Metal-based catalysts for persulfate and peroxymonosulfate activation in heterogeneous ways: A review
URI https://dx.doi.org/10.1016/j.cej.2021.132323
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