Transparent hierarchical columnar nanocomposites
[Display omitted] •Columnar nanocomposites mimicking the transparent teeth of deep-sea dragonfish.•Highly transparent, ultralow haze, and birefringent.•Enamel-like modulus, hardness, and indentation fracture toughness.•Functional synergy by hierarchical design. The expertise of living organisms to c...
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Published in | Chemical engineering journal (Lausanne, Switzerland : 1996) Vol. 466; p. 143167 |
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Main Authors | , , , , , , , |
Format | Journal Article |
Language | English |
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Elsevier B.V
15.06.2023
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Abstract | [Display omitted]
•Columnar nanocomposites mimicking the transparent teeth of deep-sea dragonfish.•Highly transparent, ultralow haze, and birefringent.•Enamel-like modulus, hardness, and indentation fracture toughness.•Functional synergy by hierarchical design.
The expertise of living organisms to combine a desirable set of mechanical and optical properties in biological tissues originates from genetically controlled formation of hierarchical architecture. By mimicking the enamel prisms consisting of nanorod clusters, we integrate high transparency and ultralow haze with enamel-like hardness, modulus, and indentation fracture toughness in hierarchical columnar nanocomposites. The aligned bundled nanorods from a seeded growth on top of single nanorods are the key building unit for combining all these properties, achieving a transmittance as high as 90% in the visible and ultralow haze of less than 1%, when the refractive index of fluorapatite matches with epoxy resin with appropriate crosslinkers. The highly transparent columnar nanocomposites are also optically anisotropic showing apparent birefringence. Compared with single nanorods, bundled nanorods as inorganic motif enable similar modulus but a 40% higher indentation fracture toughness owing to the additional stress passivation mechanism at the intra-rod interface, despite of higher inorganic contents. Better energy dissipation ability under dynamic conditions is achieved for hierarchical columnar nanocomposites because of more effective plastic energy dissipation pathway. The functional synergies achieved in this study using hierarchical design underly a general biomimetic principle for creating high-performance multifunctional materials. |
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AbstractList | [Display omitted]
•Columnar nanocomposites mimicking the transparent teeth of deep-sea dragonfish.•Highly transparent, ultralow haze, and birefringent.•Enamel-like modulus, hardness, and indentation fracture toughness.•Functional synergy by hierarchical design.
The expertise of living organisms to combine a desirable set of mechanical and optical properties in biological tissues originates from genetically controlled formation of hierarchical architecture. By mimicking the enamel prisms consisting of nanorod clusters, we integrate high transparency and ultralow haze with enamel-like hardness, modulus, and indentation fracture toughness in hierarchical columnar nanocomposites. The aligned bundled nanorods from a seeded growth on top of single nanorods are the key building unit for combining all these properties, achieving a transmittance as high as 90% in the visible and ultralow haze of less than 1%, when the refractive index of fluorapatite matches with epoxy resin with appropriate crosslinkers. The highly transparent columnar nanocomposites are also optically anisotropic showing apparent birefringence. Compared with single nanorods, bundled nanorods as inorganic motif enable similar modulus but a 40% higher indentation fracture toughness owing to the additional stress passivation mechanism at the intra-rod interface, despite of higher inorganic contents. Better energy dissipation ability under dynamic conditions is achieved for hierarchical columnar nanocomposites because of more effective plastic energy dissipation pathway. The functional synergies achieved in this study using hierarchical design underly a general biomimetic principle for creating high-performance multifunctional materials. |
ArticleNumber | 143167 |
Author | Tang, Jinyu Jiang, Zhonghao Sun, Weiming Hou, Ying Qi, Xiaodong Feng, Shouhua Yang, Ming Han, Shuangxia |
Author_xml | – sequence: 1 givenname: Shuangxia surname: Han fullname: Han, Shuangxia organization: State Key Laboratory of Inorganic Synthesis and Preparative Chemistry, Jilin University, Changchun 130012, China – sequence: 2 givenname: Jinyu surname: Tang fullname: Tang, Jinyu organization: State Key Laboratory of Inorganic Synthesis and Preparative Chemistry, Jilin University, Changchun 130012, China – sequence: 3 givenname: Xiaodong orcidid: 0000-0002-6886-6623 surname: Qi fullname: Qi, Xiaodong organization: State Key Laboratory of Inorganic Synthesis and Preparative Chemistry, Jilin University, Changchun 130012, China – sequence: 4 givenname: Weiming surname: Sun fullname: Sun, Weiming organization: Key Laboratory of Automobile Materials, College of Materials Science and Engineering, Jilin University, Changchun 130025, China – sequence: 5 givenname: Zhonghao surname: Jiang fullname: Jiang, Zhonghao organization: Key Laboratory of Automobile Materials, College of Materials Science and Engineering, Jilin University, Changchun 130025, China – sequence: 6 givenname: Ying surname: Hou fullname: Hou, Ying organization: State Key Laboratory of Inorganic Synthesis and Preparative Chemistry, Jilin University, Changchun 130012, China – sequence: 7 givenname: Ming orcidid: 0000-0001-8844-069X surname: Yang fullname: Yang, Ming email: mingyang@jlu.edu.cn organization: State Key Laboratory of Inorganic Synthesis and Preparative Chemistry, Jilin University, Changchun 130012, China – sequence: 8 givenname: Shouhua surname: Feng fullname: Feng, Shouhua organization: State Key Laboratory of Inorganic Synthesis and Preparative Chemistry, Jilin University, Changchun 130012, China |
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Keywords | Transparent materials Mechanical properties Biomimetic materials Nanocomposites Hierarchical architecture |
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•Columnar nanocomposites mimicking the transparent teeth of deep-sea dragonfish.•Highly transparent, ultralow haze, and... |
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SubjectTerms | Biomimetic materials Hierarchical architecture Mechanical properties Nanocomposites Transparent materials |
Title | Transparent hierarchical columnar nanocomposites |
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