Lattice distortion induced Ce-doped NiFe-LDH for efficient oxygen evolution
[Display omitted] •Inducing lattice distortion in NiFe-LDH nanosheets by Ce-doping towards accelerating electrocatalytic oxygen evolution reaction.•The optimal NiFeCe-LDH@CP only requires 267 mV to deliver 100 mA cm−2, which is 41 mV lower than pure NiFe-LDH@CP.•NiFeCe-LDH@CP have retained their str...
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| Published in | Chemical engineering journal (Lausanne, Switzerland : 1996) Vol. 464; p. 142669 |
|---|---|
| Main Authors | , , , , , , |
| Format | Journal Article |
| Language | English |
| Published |
Elsevier B.V
15.05.2023
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| Subjects | |
| Online Access | Get full text |
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| Abstract | [Display omitted]
•Inducing lattice distortion in NiFe-LDH nanosheets by Ce-doping towards accelerating electrocatalytic oxygen evolution reaction.•The optimal NiFeCe-LDH@CP only requires 267 mV to deliver 100 mA cm−2, which is 41 mV lower than pure NiFe-LDH@CP.•NiFeCe-LDH@CP have retained their structural property after 70 h stability.•DFT calculations reveal that lattice distortion could optimize the electronic structure of the Ni element in active sites and lower the energy barrier, thus accelerating the OER.
Nickel-iron layered double hydroxide (NiFe-LDH) is a promising active electrocatalyst for oxygen evolution reaction (OER). However, the development of NiFe-LDH is limited by poor electrical conductivity and inferior cycling stability. Herein, we present a structural perturbation and distinct distorted lattice strategy via Ce doping in NiFe-LDH on carbon paper (CP) (NiFeCe-LDH@CP) to boost its OER performance. Lattice distortion results in a large accessible surface area and induces more Ovac, accelerating the OER by modifying the intrinsic electronic structure and optimizing the adsorption energy of intermediates. As a result, the optimized NiFeCe-LDH@CP possesses excellent stability over 70 h and can deliver the current density of 100 mA/cm2 with the overpotentials of only 267 mV, which is 41 mV lower than pure NiFe-LDH@CP. Theoretical calculations indicate that the introduction of lattice distortion into NiFe-LDH could optimize the electronic structure of the Ni element in active sites and lower the energy barrier, thus leading to a significant increase in OER activity. This work figures out the effect of lattice distortion strategy on the improvement of OER performance, which opens new perspectives on the development of defect-rich OER electrocatalysts. |
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| AbstractList | [Display omitted]
•Inducing lattice distortion in NiFe-LDH nanosheets by Ce-doping towards accelerating electrocatalytic oxygen evolution reaction.•The optimal NiFeCe-LDH@CP only requires 267 mV to deliver 100 mA cm−2, which is 41 mV lower than pure NiFe-LDH@CP.•NiFeCe-LDH@CP have retained their structural property after 70 h stability.•DFT calculations reveal that lattice distortion could optimize the electronic structure of the Ni element in active sites and lower the energy barrier, thus accelerating the OER.
Nickel-iron layered double hydroxide (NiFe-LDH) is a promising active electrocatalyst for oxygen evolution reaction (OER). However, the development of NiFe-LDH is limited by poor electrical conductivity and inferior cycling stability. Herein, we present a structural perturbation and distinct distorted lattice strategy via Ce doping in NiFe-LDH on carbon paper (CP) (NiFeCe-LDH@CP) to boost its OER performance. Lattice distortion results in a large accessible surface area and induces more Ovac, accelerating the OER by modifying the intrinsic electronic structure and optimizing the adsorption energy of intermediates. As a result, the optimized NiFeCe-LDH@CP possesses excellent stability over 70 h and can deliver the current density of 100 mA/cm2 with the overpotentials of only 267 mV, which is 41 mV lower than pure NiFe-LDH@CP. Theoretical calculations indicate that the introduction of lattice distortion into NiFe-LDH could optimize the electronic structure of the Ni element in active sites and lower the energy barrier, thus leading to a significant increase in OER activity. This work figures out the effect of lattice distortion strategy on the improvement of OER performance, which opens new perspectives on the development of defect-rich OER electrocatalysts. |
| ArticleNumber | 142669 |
| Author | Wang, Yingying Li, Yao Li, Yongxiu Pan, Wanghao Li, Jing Liao, Yuanyuan He, Ruchen |
| Author_xml | – sequence: 1 givenname: Yuanyuan orcidid: 0000-0003-4640-5292 surname: Liao fullname: Liao, Yuanyuan organization: School of Chemistry and Chemical Engineering, Nanchang University, Nanchang, Jiangxi 330031, China – sequence: 2 givenname: Ruchen surname: He fullname: He, Ruchen organization: School of Chemistry and Chemical Engineering, Nanchang University, Nanchang, Jiangxi 330031, China – sequence: 3 givenname: Wanghao surname: Pan fullname: Pan, Wanghao organization: School of Chemistry and Chemical Engineering, Nanchang University, Nanchang, Jiangxi 330031, China – sequence: 4 givenname: Yao surname: Li fullname: Li, Yao organization: School of Chemistry and Chemical Engineering, Nanchang University, Nanchang, Jiangxi 330031, China – sequence: 5 givenname: Yingying surname: Wang fullname: Wang, Yingying organization: School of Chemistry and Chemical Engineering, Nanchang University, Nanchang, Jiangxi 330031, China – sequence: 6 givenname: Jing orcidid: 0000-0001-8630-8265 surname: Li fullname: Li, Jing email: lijingbuaa@163.com organization: School of Chemistry and Chemical Engineering, Nanchang University, Nanchang, Jiangxi 330031, China – sequence: 7 givenname: Yongxiu orcidid: 0000-0003-3522-3186 surname: Li fullname: Li, Yongxiu email: yxli@ncu.edu.cn organization: School of Chemistry and Chemical Engineering, Nanchang University, Nanchang, Jiangxi 330031, China |
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| Keywords | Oxygen evolution reaction Lattice distortion NiFe LDH Ce doping |
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•Inducing lattice distortion in NiFe-LDH nanosheets by Ce-doping towards accelerating electrocatalytic oxygen evolution reaction.•The optimal... |
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| SubjectTerms | Ce doping Lattice distortion NiFe LDH Oxygen evolution reaction |
| Title | Lattice distortion induced Ce-doped NiFe-LDH for efficient oxygen evolution |
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