Cathode of Co9S8/NiMn-LDH with enhanced cycle stability and anode of carbon gels for asymmetric supercapacitors
Nickel‑manganese layered double hydroxide (NiMn-LDH) is used for supercapacitors due to its high redox activity and theoretical capacity, while with the disadvantages of low conductivity and unstable structure. Here, we report a Co9S8/NiMn-LDH composite electrode material with a core-shell heterostr...
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| Published in | Journal of energy storage Vol. 72; p. 108505 |
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| Main Authors | , , , , , , , |
| Format | Journal Article |
| Language | English |
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Elsevier Ltd
25.11.2023
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| Abstract | Nickel‑manganese layered double hydroxide (NiMn-LDH) is used for supercapacitors due to its high redox activity and theoretical capacity, while with the disadvantages of low conductivity and unstable structure. Here, we report a Co9S8/NiMn-LDH composite electrode material with a core-shell heterostructure grown in situ on a carbon cloth (CC). NiMn-LDH nanosheets are uniformly and densely grown in the outer layer of Co9S8 nanorods, and this structure design makes full use of the high activity of NiMn-LDH. Meanwhile, the internal electric field formed at the heterogeneous interface is shown by density functional theory (DFT) calculations to effectively accelerate the diffusion of OH− in the electrode. The core-shell heterostructure makes it exhibit better electrochemical performance than NiMn-LDH as a positive electrode (178.7 mA h g−1 specific capacity at 1 A g−1, 80.6 % capacity retention after 5000 cycles). In addition, a carbon gels anode was prepared by the sol-gel method and subsequent carbonization steps, which has excellent performance (specific capacitance of 145.6 F g−1 at 1 A g−1). The assembled Co9S8/NiMn-LDH//C-gel asymmetric supercapacitor provides an energy density of 35.2 Wh kg−1 at 850 W kg−1. Further assembled into a quasi-solid-state flexible supercapacitor, two devices in series can light an LED lamp, showing its potential application prospects in energy storage systems.
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•Co9S8/NiMn-LDH with core-shell structure was successfully designed.•Further analysis was carried out by DFT calculations.•The electrochemical performance of carbon aerogel is better than that of activated carbon. |
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| AbstractList | Nickel‑manganese layered double hydroxide (NiMn-LDH) is used for supercapacitors due to its high redox activity and theoretical capacity, while with the disadvantages of low conductivity and unstable structure. Here, we report a Co9S8/NiMn-LDH composite electrode material with a core-shell heterostructure grown in situ on a carbon cloth (CC). NiMn-LDH nanosheets are uniformly and densely grown in the outer layer of Co9S8 nanorods, and this structure design makes full use of the high activity of NiMn-LDH. Meanwhile, the internal electric field formed at the heterogeneous interface is shown by density functional theory (DFT) calculations to effectively accelerate the diffusion of OH− in the electrode. The core-shell heterostructure makes it exhibit better electrochemical performance than NiMn-LDH as a positive electrode (178.7 mA h g−1 specific capacity at 1 A g−1, 80.6 % capacity retention after 5000 cycles). In addition, a carbon gels anode was prepared by the sol-gel method and subsequent carbonization steps, which has excellent performance (specific capacitance of 145.6 F g−1 at 1 A g−1). The assembled Co9S8/NiMn-LDH//C-gel asymmetric supercapacitor provides an energy density of 35.2 Wh kg−1 at 850 W kg−1. Further assembled into a quasi-solid-state flexible supercapacitor, two devices in series can light an LED lamp, showing its potential application prospects in energy storage systems.
[Display omitted]
•Co9S8/NiMn-LDH with core-shell structure was successfully designed.•Further analysis was carried out by DFT calculations.•The electrochemical performance of carbon aerogel is better than that of activated carbon. |
| ArticleNumber | 108505 |
| Author | Jin, Xiaoli Dai, Yatang Wang, Jiaheng Xie, Mingzhen Hu, Cunhai Zhong, Linzhi Wang, Shuai Gong, Jiaxu |
| Author_xml | – sequence: 1 givenname: Shuai surname: Wang fullname: Wang, Shuai organization: School of Materials and Chemistry, Southwest University of Science and Technology, Mianyang 621010, PR China – sequence: 2 givenname: Jiaheng surname: Wang fullname: Wang, Jiaheng organization: School of Materials and Chemistry, Southwest University of Science and Technology, Mianyang 621010, PR China – sequence: 3 givenname: Xiaoli surname: Jin fullname: Jin, Xiaoli organization: School of Materials and Chemistry, Southwest University of Science and Technology, Mianyang 621010, PR China – sequence: 4 givenname: Mingzhen surname: Xie fullname: Xie, Mingzhen organization: School of Materials and Chemistry, Southwest University of Science and Technology, Mianyang 621010, PR China – sequence: 5 givenname: Cunhai surname: Hu fullname: Hu, Cunhai organization: School of Materials and Chemistry, Southwest University of Science and Technology, Mianyang 621010, PR China – sequence: 6 givenname: Linzhi surname: Zhong fullname: Zhong, Linzhi organization: School of Materials and Chemistry, Southwest University of Science and Technology, Mianyang 621010, PR China – sequence: 7 givenname: Jiaxu surname: Gong fullname: Gong, Jiaxu email: gongjiaxu@swust.edu.cn organization: School of Materials and Chemistry, Southwest University of Science and Technology, Mianyang 621010, PR China – sequence: 8 givenname: Yatang surname: Dai fullname: Dai, Yatang email: daiyatang@swust.edu.cn organization: School of Materials and Chemistry, Southwest University of Science and Technology, Mianyang 621010, PR China |
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| Snippet | Nickel‑manganese layered double hydroxide (NiMn-LDH) is used for supercapacitors due to its high redox activity and theoretical capacity, while with the... |
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| SubjectTerms | Asymmetric supercapacitors Core-shell structure Density functional theory NiMn-LDH |
| Title | Cathode of Co9S8/NiMn-LDH with enhanced cycle stability and anode of carbon gels for asymmetric supercapacitors |
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