Metal organic framework derived NiCo layered double hydroxide anode aggregated with biomass derived reduced graphene oxide cathode: A hybrid device configuration for supercapattery applications

Metal-organic frameworks (MOFs), due to its exceptional characteristics like high specific surface area and design diversity, serve as an outstanding sacrificial template in forming layered double hydroxides (LDHs) for highly efficient electrodes in supercapattery devices. In this work, we have prep...

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Published inJournal of energy storage Vol. 73; p. 109264
Main Authors Prajapati, Megha, Ravi Kant, Chhaya, Allende, Scarlett, Jacob, Mohan V.
Format Journal Article
LanguageEnglish
Published Elsevier Ltd 20.12.2023
Subjects
Energy density
Metal-organic frameworks
Power density
Supercapattery
Power density
Supercapattery
Energy density
Metal-organic frameworks
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Abstract Metal-organic frameworks (MOFs), due to its exceptional characteristics like high specific surface area and design diversity, serve as an outstanding sacrificial template in forming layered double hydroxides (LDHs) for highly efficient electrodes in supercapattery devices. In this work, we have prepared bimetallic layered Nickel Cobalt LDH via in-situ etching of Co-ZIF, in different Nickel concentrations directly on Ni foam that enhances the interfacial contact between substrate and the material. The optimised NiCo LDH-2 sample exhibited remarkable electrochemical behaviour with fast electrolyte ion diffusion kinetics ideal for supercapattery device and delivered a high specific capacitance of 2567 Fg−1 at 1 Ag−1. Further, the supercapattery device assembled with Ni-Co LDH as anode and rGO derived from a sustainable source as cathode demonstrated an energy density of 21 Whkg−1, power density of 0.307 kWkg−1 and good cyclic stability with capacitance retention of 88.89 % along with coulombic efficiency of 90.58 % over 1500 cycles. This work proposes an effective approach for designing layered NiCo-LDH that can be further extended to the synthesis of other transition metal-derived LDH for supercapattery devices. [Display omitted] •Co-ZIF is converted into NiCo LDH using in situ etching method directly on Ni foam and used as anode in supercapattery device.•Eco-friendly approach was used to synthesize rGO from coffee grounds using microwave pyrolysis technique and used as cathode for the hybrid device.•The supercapattery device delivers high specific capacitance, energy and power density.•The results portrayed by the fabricated device offer great potential in efficient energy storage applications.
AbstractList Metal-organic frameworks (MOFs), due to its exceptional characteristics like high specific surface area and design diversity, serve as an outstanding sacrificial template in forming layered double hydroxides (LDHs) for highly efficient electrodes in supercapattery devices. In this work, we have prepared bimetallic layered Nickel Cobalt LDH via in-situ etching of Co-ZIF, in different Nickel concentrations directly on Ni foam that enhances the interfacial contact between substrate and the material. The optimised NiCo LDH-2 sample exhibited remarkable electrochemical behaviour with fast electrolyte ion diffusion kinetics ideal for supercapattery device and delivered a high specific capacitance of 2567 Fg−1 at 1 Ag−1. Further, the supercapattery device assembled with Ni-Co LDH as anode and rGO derived from a sustainable source as cathode demonstrated an energy density of 21 Whkg−1, power density of 0.307 kWkg−1 and good cyclic stability with capacitance retention of 88.89 % along with coulombic efficiency of 90.58 % over 1500 cycles. This work proposes an effective approach for designing layered NiCo-LDH that can be further extended to the synthesis of other transition metal-derived LDH for supercapattery devices. [Display omitted] •Co-ZIF is converted into NiCo LDH using in situ etching method directly on Ni foam and used as anode in supercapattery device.•Eco-friendly approach was used to synthesize rGO from coffee grounds using microwave pyrolysis technique and used as cathode for the hybrid device.•The supercapattery device delivers high specific capacitance, energy and power density.•The results portrayed by the fabricated device offer great potential in efficient energy storage applications.
ArticleNumber 109264
Author Jacob, Mohan V.
Ravi Kant, Chhaya
Prajapati, Megha
Allende, Scarlett
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CitedBy_id crossref_primary_10_1007_s11664_024_11048_2
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Snippet Metal-organic frameworks (MOFs), due to its exceptional characteristics like high specific surface area and design diversity, serve as an outstanding...
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SubjectTerms Energy density
Metal-organic frameworks
Power density
Supercapattery
Title Metal organic framework derived NiCo layered double hydroxide anode aggregated with biomass derived reduced graphene oxide cathode: A hybrid device configuration for supercapattery applications
URI https://dx.doi.org/10.1016/j.est.2023.109264
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