Cobalt nanoparticles encapsulated in iron and nitrogen co-doped urchin-like porous carbons as an efficient bifunctional oxygen reversible catalyst for Zn-air batteries
•Monodispersed cobalt nanoparticles encapsulated in Fe, N co-doped carbons.•This structure can reduce the degradation of agglomeration properties.•The catalyst exhibits a low reversible oxygen potential gap (0.67 V).•ZAB exhibit excellent energy density (802 mAh g−1) and durability.•The remarkable a...
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Published in | Chemical engineering journal (Lausanne, Switzerland : 1996) Vol. 436; p. 135191 |
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Main Authors | , , , , , , , , , , |
Format | Journal Article |
Language | English |
Published |
Elsevier B.V
15.05.2022
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Abstract | •Monodispersed cobalt nanoparticles encapsulated in Fe, N co-doped carbons.•This structure can reduce the degradation of agglomeration properties.•The catalyst exhibits a low reversible oxygen potential gap (0.67 V).•ZAB exhibit excellent energy density (802 mAh g−1) and durability.•The remarkable activities are due to the synergistic effect of Co and Fe-Nx/C.
Design of the cheap and high-efficiency catalysts for oxygen reduction reaction (ORR) and oxygen evolution reaction (OER) is imperative for rechargeable Zn-batteries (r-ZABs). Herein, the cobalt nanoparticles encapsulated in iron and nitrogen co-doped urchin-like porous carbons (Co@Fe-Nx/C) as a bifunctional electrocatalyst for ORR and OER is fabricated via a facile pyrolysis treatment. The Co@Fe-Nx/C catalyst displays a typical urchin-like morphology anchored with numerous CNTs and many monodispersed cobalt nanoparticles are encapsulated in the carbon matrices, which not only enable effective and fast electron transfer, but also can prevent Co nanoparticles from surface oxidation and agglomeration-induced activity degradation, thus improving the electrocatalytic activities and durability. The Co@Fe-Nx/C catalyst exhibits a superb ORR/OER catalytic activities with a low reversible oxygen potential gap (0.67 V), surpassing the commercial Pt/C and RuO2 catalysts (0.69 V). Liquid r-ZAB constructed with Co@Fe-Nx/C as the air cathode manifest outstanding energy density (802 mAh g−1), superb charge/discharge performance and excellent reversibility and durability compared to the precious metal couple catalysts. The remarkable bifunctional catalytic activities are due to the synergistic effect of Co nanoparticles and Fe-Nx/C substrates. |
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AbstractList | •Monodispersed cobalt nanoparticles encapsulated in Fe, N co-doped carbons.•This structure can reduce the degradation of agglomeration properties.•The catalyst exhibits a low reversible oxygen potential gap (0.67 V).•ZAB exhibit excellent energy density (802 mAh g−1) and durability.•The remarkable activities are due to the synergistic effect of Co and Fe-Nx/C.
Design of the cheap and high-efficiency catalysts for oxygen reduction reaction (ORR) and oxygen evolution reaction (OER) is imperative for rechargeable Zn-batteries (r-ZABs). Herein, the cobalt nanoparticles encapsulated in iron and nitrogen co-doped urchin-like porous carbons (Co@Fe-Nx/C) as a bifunctional electrocatalyst for ORR and OER is fabricated via a facile pyrolysis treatment. The Co@Fe-Nx/C catalyst displays a typical urchin-like morphology anchored with numerous CNTs and many monodispersed cobalt nanoparticles are encapsulated in the carbon matrices, which not only enable effective and fast electron transfer, but also can prevent Co nanoparticles from surface oxidation and agglomeration-induced activity degradation, thus improving the electrocatalytic activities and durability. The Co@Fe-Nx/C catalyst exhibits a superb ORR/OER catalytic activities with a low reversible oxygen potential gap (0.67 V), surpassing the commercial Pt/C and RuO2 catalysts (0.69 V). Liquid r-ZAB constructed with Co@Fe-Nx/C as the air cathode manifest outstanding energy density (802 mAh g−1), superb charge/discharge performance and excellent reversibility and durability compared to the precious metal couple catalysts. The remarkable bifunctional catalytic activities are due to the synergistic effect of Co nanoparticles and Fe-Nx/C substrates. |
ArticleNumber | 135191 |
Author | Zhao, Dengke Chen, Minzhe Li, Zilong Wang, Nan Li, Ligui Niu, Xiaojun Ning, Shunlian Li, Nanwen Yu, Xiaolong Zhu, Yuguang Zhou, Wei |
Author_xml | – sequence: 1 givenname: Yuguang surname: Zhu fullname: Zhu, Yuguang organization: Guangzhou Key Laboratory for Surface Chemistry of Energy Materials, New Energy Research Institute, Guangdong Provincial Key Laboratory of Atmospheric Environment and Pollution Control, College of Environment and Energy, School of Environment and Energy, South China University of Technology, Guangzhou Higher Education Mega Center, Guangzhou 510006, China – sequence: 2 givenname: Shunlian surname: Ning fullname: Ning, Shunlian organization: Guangzhou Key Laboratory for Surface Chemistry of Energy Materials, New Energy Research Institute, Guangdong Provincial Key Laboratory of Atmospheric Environment and Pollution Control, College of Environment and Energy, School of Environment and Energy, South China University of Technology, Guangzhou Higher Education Mega Center, Guangzhou 510006, China – sequence: 3 givenname: Xiaolong surname: Yu fullname: Yu, Xiaolong organization: Guangdong Provincial Key Laboratory of Petrochemical Pollution Processes and Control, School of Environmental Science and Engineering, Guangdong University of Petrochemical Technology, Maoming, Guangdong 525000, PR China – sequence: 4 givenname: Xiaojun surname: Niu fullname: Niu, Xiaojun organization: Guangzhou Key Laboratory for Surface Chemistry of Energy Materials, New Energy Research Institute, Guangdong Provincial Key Laboratory of Atmospheric Environment and Pollution Control, College of Environment and Energy, School of Environment and Energy, South China University of Technology, Guangzhou Higher Education Mega Center, Guangzhou 510006, China – sequence: 5 givenname: Minzhe surname: Chen fullname: Chen, Minzhe organization: Guangzhou Key Laboratory for Surface Chemistry of Energy Materials, New Energy Research Institute, Guangdong Provincial Key Laboratory of Atmospheric Environment and Pollution Control, College of Environment and Energy, School of Environment and Energy, South China University of Technology, Guangzhou Higher Education Mega Center, Guangzhou 510006, China – sequence: 6 givenname: Wei surname: Zhou fullname: Zhou, Wei organization: Guangzhou Key Laboratory for Surface Chemistry of Energy Materials, New Energy Research Institute, Guangdong Provincial Key Laboratory of Atmospheric Environment and Pollution Control, College of Environment and Energy, School of Environment and Energy, South China University of Technology, Guangzhou Higher Education Mega Center, Guangzhou 510006, China – sequence: 7 givenname: Dengke surname: Zhao fullname: Zhao, Dengke email: scutezhao@sina.com organization: Guangzhou Key Laboratory for Surface Chemistry of Energy Materials, New Energy Research Institute, Guangdong Provincial Key Laboratory of Atmospheric Environment and Pollution Control, College of Environment and Energy, School of Environment and Energy, South China University of Technology, Guangzhou Higher Education Mega Center, Guangzhou 510006, China – sequence: 8 givenname: Zilong surname: Li fullname: Li, Zilong organization: Siyuan laboratory, Guangzhou Key Laboratory of Vacuum Coating Technologies and New Energy Materials, Department of Physics, Jinan University, Guangzhou, Guangdong 510632, China – sequence: 9 givenname: Nan surname: Wang fullname: Wang, Nan email: nanwang@email.jnu.edu.cn organization: Siyuan laboratory, Guangzhou Key Laboratory of Vacuum Coating Technologies and New Energy Materials, Department of Physics, Jinan University, Guangzhou, Guangdong 510632, China – sequence: 10 givenname: Nanwen surname: Li fullname: Li, Nanwen organization: Key Laboratory of Coal Conversion, Institute of Coal Chemistry, Chinese Academy of Sciences, Taiyuan 030001, China – sequence: 11 givenname: Ligui surname: Li fullname: Li, Ligui email: esguili@scut.edu.cn organization: Guangzhou Key Laboratory for Surface Chemistry of Energy Materials, New Energy Research Institute, Guangdong Provincial Key Laboratory of Atmospheric Environment and Pollution Control, College of Environment and Energy, School of Environment and Energy, South China University of Technology, Guangzhou Higher Education Mega Center, Guangzhou 510006, China |
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Keywords | R-ZAB Oxygen evolution reaction ZIF-8 Urchin-like morphology Oxygen reduction reaction |
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SubjectTerms | Oxygen evolution reaction Oxygen reduction reaction R-ZAB Urchin-like morphology ZIF-8 |
Title | Cobalt nanoparticles encapsulated in iron and nitrogen co-doped urchin-like porous carbons as an efficient bifunctional oxygen reversible catalyst for Zn-air batteries |
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