Using Si, Al and Fe as Tracers for Source Apportionment of Air Pollutants in Lake Baikal Snowpack
The aim of this study was to select chemical species characterized by distinctly different proportions in natural and anthropogenic particulate matter that could be used as tracers for air pollutant sources. The end-member mixing approach, based on the observation that the chemical species in snow c...
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| Published in | Sustainability Vol. 12; no. 8; p. 3392 |
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| Main Authors | , , , |
| Format | Journal Article |
| Language | English |
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01.04.2020
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| ISSN | 2071-1050 2071-1050 |
| DOI | 10.3390/su12083392 |
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| Abstract | The aim of this study was to select chemical species characterized by distinctly different proportions in natural and anthropogenic particulate matter that could be used as tracers for air pollutant sources. The end-member mixing approach, based on the observation that the chemical species in snow closely correlated with land use are those that exhibit differences in concentrations across the different types of anthropogenic wastes, was used for source apportionment. The concentrations of Si and Fe normalized to Al were used as tracers in the mixing equations. Mixing diagrams showed that the major pollution sources (in descending order) are oil, coal, and wood combustion. The traces of several minor sources, such as aluminum production plants, pulp and paper mills, steel rust, and natural aluminosilicates, were also detected. It was found that the fingerprint of diesel engines on snow is similar to that of oil combustion; thus, future research of the role of diesel engines in air pollution will be needed. The insufficient precision of source apportionment is probably due to different combinations of pollution sources in different areas. Thus, principles for the delineation of areas affected by different source combinations should be the subject of further studies. |
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| AbstractList | The aim of this study was to select chemical species characterized by distinctly different proportions in natural and anthropogenic particulate matter that could be used as tracers for air pollutant sources. The end-member mixing approach, based on the observation that the chemical species in snow closely correlated with land use are those that exhibit differences in concentrations across the different types of anthropogenic wastes, was used for source apportionment. The concentrations of Si and Fe normalized to Al were used as tracers in the mixing equations. Mixing diagrams showed that the major pollution sources (in descending order) are oil, coal, and wood combustion. The traces of several minor sources, such as aluminum production plants, pulp and paper mills, steel rust, and natural aluminosilicates, were also detected. It was found that the fingerprint of diesel engines on snow is similar to that of oil combustion; thus, future research of the role of diesel engines in air pollution will be needed. The insufficient precision of source apportionment is probably due to different combinations of pollution sources in different areas. Thus, principles for the delineation of areas affected by different source combinations should be the subject of further studies. |
| Author | Silaev, Anton V. Semenov, Yuri M. Begunova, Larisa A. Semenov, Mikhail Yu |
| Author_xml | – sequence: 1 givenname: Mikhail Yu surname: Semenov fullname: Semenov, Mikhail Yu – sequence: 2 givenname: Anton V. surname: Silaev fullname: Silaev, Anton V. – sequence: 3 givenname: Yuri M. orcidid: 0000-0002-8900-6817 surname: Semenov fullname: Semenov, Yuri M. – sequence: 4 givenname: Larisa A. surname: Begunova fullname: Begunova, Larisa A. |
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| CitedBy_id | crossref_primary_10_1088_1755_1315_988_3_032050 crossref_primary_10_3390_su142214827 crossref_primary_10_3390_atmos11111184 crossref_primary_10_3390_su13105389 crossref_primary_10_3390_su132413584 crossref_primary_10_1016_j_scitotenv_2023_162637 crossref_primary_10_3390_su14106170 |
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