Facile fabrication of low-content surface-assembled MXene in silicone rubber foam materials with lightweight, wide-temperature mechanical flexibility, improved flame resistance and exceptional smoke suppression
Silicone rubber foam (SiRF) is a promising porous material that is widely applied in various fields. However, its intrinsic flammability nature remains a significant challenge. One of the simplest and most economical solutions is to incorporate high content flame-retardant fillers. Unfortunately, su...
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| Published in | Composites. Part A, Applied science and manufacturing Vol. 177; p. 107907 |
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| Main Authors | , , , , , , , , , , , |
| Format | Journal Article |
| Language | English |
| Published |
01.02.2024
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| Abstract | Silicone rubber foam (SiRF) is a promising porous material that is widely applied in various fields. However, its intrinsic flammability nature remains a significant challenge. One of the simplest and most economical solutions is to incorporate high content flame-retardant fillers. Unfortunately, such approach is limited by several drawbacks, including poor filler dispersion, difficulty in processing and negative effect on mechanical flexibility. Herein, we report a green and facile strategy for surface-assembling ultralow content of MXene sheets bonded onto the pore surface of SiRF via the effective foaming reaction process. The as-prepared MSiRF-0.2 composite at 0.2 wt% MXene exhibited lightweight characteristic, wide-temperature mechanical flexibility, UL94-V0 grade, limited oxygen index of >27%, and exceptional smoke suppression (reduction by 88.24%). Furthermore, flame-retardant mechanism was discussed based on the char structure observation. This study provides a novel approach for fabricating mechanically flexible and flame-retardant SiRF via in-situ reactive assembly of low content MXene sheets. |
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| AbstractList | Silicone rubber foam (SiRF) is a promising porous material that is widely applied in various fields. However, its intrinsic flammability nature remains a significant challenge. One of the simplest and most economical solutions is to incorporate high content flame-retardant fillers. Unfortunately, such approach is limited by several drawbacks, including poor filler dispersion, difficulty in processing and negative effect on mechanical flexibility. Herein, we report a green and facile strategy for surface-assembling ultralow content of MXene sheets bonded onto the pore surface of SiRF via the effective foaming reaction process. The as-prepared MSiRF-0.2 composite at 0.2 wt% MXene exhibited lightweight characteristic, wide-temperature mechanical flexibility, UL94-V0 grade, limited oxygen index of >27%, and exceptional smoke suppression (reduction by 88.24%). Furthermore, flame-retardant mechanism was discussed based on the char structure observation. This study provides a novel approach for fabricating mechanically flexible and flame-retardant SiRF via in-situ reactive assembly of low content MXene sheets. |
| ArticleNumber | 107907 |
| Author | Chen, Hai-Yang Qu, Zhang-Hao Qin, Yu-Qing Li, Jia-Yun Zhao, Li Wang, Peng-Huan Gong, Li-Xiu Tang, Long-Cheng Zhang, Guo-Dong Li, Yang Yang, Ling Gao, Jie-Feng |
| Author_xml | – sequence: 1 givenname: Hai-Yang surname: Chen fullname: Chen, Hai-Yang – sequence: 2 givenname: Yang surname: Li fullname: Li, Yang – sequence: 3 givenname: Peng-Huan surname: Wang fullname: Wang, Peng-Huan – sequence: 4 givenname: Zhang-Hao surname: Qu fullname: Qu, Zhang-Hao – sequence: 5 givenname: Yu-Qing surname: Qin fullname: Qin, Yu-Qing – sequence: 6 givenname: Ling surname: Yang fullname: Yang, Ling – sequence: 7 givenname: Jia-Yun surname: Li fullname: Li, Jia-Yun – sequence: 8 givenname: Li-Xiu surname: Gong fullname: Gong, Li-Xiu – sequence: 9 givenname: Li surname: Zhao fullname: Zhao, Li – sequence: 10 givenname: Guo-Dong surname: Zhang fullname: Zhang, Guo-Dong – sequence: 11 givenname: Jie-Feng orcidid: 0000-0002-6038-9770 surname: Gao fullname: Gao, Jie-Feng – sequence: 12 givenname: Long-Cheng orcidid: 0000-0002-2382-8850 surname: Tang fullname: Tang, Long-Cheng |
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