Optimizing Oxygen Electrode Bifunctionality with Platinum and Nickel Nanoparticle-Decorated Nitrogen-Doped Binary Metal Oxides

Developing bifunctional oxygen electrode materials with superior activity for oxygen reduction (ORR) and oxygen evolution (OER) reactions is essential for advancing regenerative fuel cell and rechargeable metal–air battery technologies. This present work deals with the synthesis and characterization...

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Published inProcesses Vol. 12; no. 3; p. 453
Main Authors Mladenović, Dušan, Aykut, Yasemin, Yurtcan, Ayşe B., Soylu, Gulin S. P., Santos, Diogo M. F., Miljanić, Šćepan, Šljukić, Biljana
Format Journal Article
LanguageEnglish
Published Basel MDPI AG 01.03.2024
Subjects
Air pollution
Atmospheric carbon dioxide
Carbon
Catalysis
Electrocatalysts
Electrode materials
Electrodes
Energy
Energy minerals
Fossil fuels
Fuel cells
Heat
Manganese oxides
Metal air batteries
Metal oxides
Nanoparticles
Nickel
Nickel oxides
Nitrogen
Oxygen
Oxygen evolution reactions
Rechargeable batteries
Regenerative fuel cells
St Louis Missouri
United States > US
Germany
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Abstract Developing bifunctional oxygen electrode materials with superior activity for oxygen reduction (ORR) and oxygen evolution (OER) reactions is essential for advancing regenerative fuel cell and rechargeable metal–air battery technologies. This present work deals with the synthesis and characterization of electrocatalysts containing Pt and Ni nanoparticles supported on nitrogen-doped mixed metal oxides (Mn2O3-NiO) and the systematic evaluation of their bifunctional ORR/OER performance in an alkaline medium. These electrocatalysts have been successfully synthesized by a simple and fast microwave method. PtNi/Mn2O3-NiO-N with a binary metal oxide-to-N ratio of 1:2 demonstrated the best performance among the studied materials regarding bifunctional electrocatalytic activity (∆E = 0.96 V) and robust stability.
AbstractList Developing bifunctional oxygen electrode materials with superior activity for oxygen reduction (ORR) and oxygen evolution (OER) reactions is essential for advancing regenerative fuel cell and rechargeable metal–air battery technologies. This present work deals with the synthesis and characterization of electrocatalysts containing Pt and Ni nanoparticles supported on nitrogen-doped mixed metal oxides (Mn2O3-NiO) and the systematic evaluation of their bifunctional ORR/OER performance in an alkaline medium. These electrocatalysts have been successfully synthesized by a simple and fast microwave method. PtNi/Mn2O3-NiO-N with a binary metal oxide-to-N ratio of 1:2 demonstrated the best performance among the studied materials regarding bifunctional electrocatalytic activity (∆E = 0.96 V) and robust stability.
Developing bifunctional oxygen electrode materials with superior activity for oxygen reduction (ORR) and oxygen evolution (OER) reactions is essential for advancing regenerative fuel cell and rechargeable metal–air battery technologies. This present work deals with the synthesis and characterization of electrocatalysts containing Pt and Ni nanoparticles supported on nitrogen-doped mixed metal oxides (Mn[sub.2]O[sub.3]-NiO) and the systematic evaluation of their bifunctional ORR/OER performance in an alkaline medium. These electrocatalysts have been successfully synthesized by a simple and fast microwave method. PtNi/Mn[sub.2]O[sub.3]-NiO-N with a binary metal oxide-to-N ratio of 1:2 demonstrated the best performance among the studied materials regarding bifunctional electrocatalytic activity (∆E = 0.96 V) and robust stability.
Audience Academic
Author Santos, Diogo M. F.
Mladenović, Dušan
Šljukić, Biljana
Miljanić, Šćepan
Soylu, Gulin S. P.
Aykut, Yasemin
Yurtcan, Ayşe B.
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Snippet Developing bifunctional oxygen electrode materials with superior activity for oxygen reduction (ORR) and oxygen evolution (OER) reactions is essential for...
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SubjectTerms Air pollution
Atmospheric carbon dioxide
Carbon
Catalysis
Electrocatalysts
Electrode materials
Electrodes
Energy
Energy minerals
Fossil fuels
Fuel cells
Heat
Manganese oxides
Metal air batteries
Metal oxides
Nanoparticles
Nickel
Nickel oxides
Nitrogen
Oxygen
Oxygen evolution reactions
Rechargeable batteries
Regenerative fuel cells
Title Optimizing Oxygen Electrode Bifunctionality with Platinum and Nickel Nanoparticle-Decorated Nitrogen-Doped Binary Metal Oxides
URI https://www.proquest.com/docview/3003387225
Volume 12
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