Surface optical phonon-assisted exciton photoluminescence spectroscopy in Q1D AlN nanostructures

Mechanisms and influence factors of surface optical (SO) phonon-mode-assisted exciton photoluminescence (PL) spectroscopy in quasi-1-dimensional (Q1D) nitride nanostructures remain a subject of debate. In this work, using momentum and energy conservation laws, a constraint relationship for the frequ...

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Published inApplied physics letters Vol. 123; no. 13
Main Authors Zhang, Li, Liang, Z. W., Liu, Q., Yang, A. L., Shi, Jun-Jie, Wang, Qi
Format Journal Article
LanguageEnglish
Published Melville American Institute of Physics 25.09.2023
Subjects
Applied physics
Excitation spectra
Excitons
Nanostructure
Nanowires
Phonons
Photoluminescence
Spectroscopy
Wavelengths
Wurtzite
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Abstract Mechanisms and influence factors of surface optical (SO) phonon-mode-assisted exciton photoluminescence (PL) spectroscopy in quasi-1-dimensional (Q1D) nitride nanostructures remain a subject of debate. In this work, using momentum and energy conservation laws, a constraint relationship for the frequency and wave number of SO phonon-mode-assisted exciton PL is established. Using the dispersion relationships of SO modes in anisotropic wurtzite nanowires, the frequency and wave number of SO-mode-assisted exciton PL emission are determined. The present theoretical scheme and numerical results not only explain a current experimental discrepancy but could also be used to predict and design exciton PL spectroscopy with SO phonon modes in Q1D nanostructures.
AbstractList Mechanisms and influence factors of surface optical (SO) phonon-mode-assisted exciton photoluminescence (PL) spectroscopy in quasi-1-dimensional (Q1D) nitride nanostructures remain a subject of debate. In this work, using momentum and energy conservation laws, a constraint relationship for the frequency and wave number of SO phonon-mode-assisted exciton PL is established. Using the dispersion relationships of SO modes in anisotropic wurtzite nanowires, the frequency and wave number of SO-mode-assisted exciton PL emission are determined. The present theoretical scheme and numerical results not only explain a current experimental discrepancy but could also be used to predict and design exciton PL spectroscopy with SO phonon modes in Q1D nanostructures.
Author Wang, Qi
Liu, Q.
Shi, Jun-Jie
Yang, A. L.
Zhang, Li
Liang, Z. W.
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Snippet Mechanisms and influence factors of surface optical (SO) phonon-mode-assisted exciton photoluminescence (PL) spectroscopy in quasi-1-dimensional (Q1D) nitride...
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SubjectTerms Applied physics
Excitation spectra
Excitons
Nanostructure
Nanowires
Phonons
Photoluminescence
Spectroscopy
Wavelengths
Wurtzite
Title Surface optical phonon-assisted exciton photoluminescence spectroscopy in Q1D AlN nanostructures
URI http://dx.doi.org/10.1063/5.0168167
https://www.proquest.com/docview/2868417354
Volume 123
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