Efficient piezo-catalytic dye degradation using piezoelectric 6H-SiC under harsh conditions
The development of novel piezoelectric catalysts against harsh conditions is indeed crucial for improving the piezo-catalytic degradation efficiency of colored organic dyes in wastewater. In this work, 6H-SiC nanoparticles (NPs) are utilized to piezo-catalytic degrade rhodamine B (RhB) and methylene...
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| Published in | Rare metals Vol. 43; no. 7; pp. 3173 - 3184 |
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| Main Authors | , , , , , , , |
| Format | Journal Article |
| Language | English |
| Published |
Beijing
Nonferrous Metals Society of China
01.07.2024
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| Subjects | |
| Online Access | Get full text |
| ISSN | 1001-0521 1867-7185 |
| DOI | 10.1007/s12598-024-02717-6 |
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| Abstract | The development of novel piezoelectric catalysts against harsh conditions is indeed crucial for improving the piezo-catalytic degradation efficiency of colored organic dyes in wastewater. In this work, 6H-SiC nanoparticles (NPs) are utilized to piezo-catalytic degrade rhodamine B (RhB) and methylene blue (MB) under ultrasonic vibration for the first time. The degradation efficiency of RhB and MB reaches 98.8% and 98.7% within 80 min. The piezoelectricity of 6H-SiC is comprehensively analyzed by the piezoresponse force microscope (PFM) and finite element method (FEM). The strong oxidizing active free radicals generated by the continuous piezoelectric polarized electric field of 6H-SiC, i.e., •O
2
−
and •OH, induce the decomposition reactions of colored organic dyes in solution. And the dyes are proven to degrade to harmless or less-harmful products gradually during the piezo-catalysis process by high-performance liquid chromatography tandem mass spectrometry (HPLC–MS). Moreover, RhB is also decomposed efficiently by 6H-SiC NPs under acidic and alkaline conditions. These results prove the feasibility of 6H-SiC for decomposing common water pollutants under harsh conditions and provide a new perspective for water purification.
Graphical abstract |
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| AbstractList | The development of novel piezoelectric catalysts against harsh conditions is indeed crucial for improving the piezo-catalytic degradation efficiency of colored organic dyes in wastewater. In this work, 6H-SiC nanoparticles (NPs) are utilized to piezo-catalytic degrade rhodamine B (RhB) and methylene blue (MB) under ultrasonic vibration for the first time. The degradation efficiency of RhB and MB reaches 98.8% and 98.7% within 80 min. The piezoelectricity of 6H-SiC is comprehensively analyzed by the piezoresponse force microscope (PFM) and finite element method (FEM). The strong oxidizing active free radicals generated by the continuous piezoelectric polarized electric field of 6H-SiC, i.e., •O
2
−
and •OH, induce the decomposition reactions of colored organic dyes in solution. And the dyes are proven to degrade to harmless or less-harmful products gradually during the piezo-catalysis process by high-performance liquid chromatography tandem mass spectrometry (HPLC–MS). Moreover, RhB is also decomposed efficiently by 6H-SiC NPs under acidic and alkaline conditions. These results prove the feasibility of 6H-SiC for decomposing common water pollutants under harsh conditions and provide a new perspective for water purification.
Graphical abstract |
| Author | Hou, Xin-Mei Yang, Tao Wang, Kang Wang, En-Hui Zhou, Lin-Lin Wang, Hai-Long Zhu, Lai-Pan Chou, Kuo-Chih |
| Author_xml | – sequence: 1 givenname: Lin-Lin surname: Zhou fullname: Zhou, Lin-Lin organization: Institute for Carbon Neutrality, University of Science and Technology Beijing – sequence: 2 givenname: Tao orcidid: 0000-0002-0043-5501 surname: Yang fullname: Yang, Tao email: yangtaoustb@ustb.edu.cn organization: Institute for Carbon Neutrality, University of Science and Technology Beijing, Institute of Steel Sustainable Technology, Liaoning Academy of Materials – sequence: 3 givenname: Kang surname: Wang fullname: Wang, Kang organization: Institute for Carbon Neutrality, University of Science and Technology Beijing – sequence: 4 givenname: Lai-Pan surname: Zhu fullname: Zhu, Lai-Pan organization: Beijing Institute of Nanoenergy and Nanosystems, Chinese Academy of Sciences – sequence: 5 givenname: En-Hui surname: Wang fullname: Wang, En-Hui organization: Institute for Carbon Neutrality, University of Science and Technology Beijing, Institute of Steel Sustainable Technology, Liaoning Academy of Materials – sequence: 6 givenname: Kuo-Chih surname: Chou fullname: Chou, Kuo-Chih organization: Institute for Carbon Neutrality, University of Science and Technology Beijing – sequence: 7 givenname: Hai-Long surname: Wang fullname: Wang, Hai-Long organization: School of Materials Science Engineering, Zhengzhou University – sequence: 8 givenname: Xin-Mei orcidid: 0000-0001-9486-478X surname: Hou fullname: Hou, Xin-Mei email: houxinmeiustb@ustb.edu.cn organization: Institute for Carbon Neutrality, University of Science and Technology Beijing, Institute of Steel Sustainable Technology, Liaoning Academy of Materials, Beijing Advanced Innovation Center for Materials Genome Engineering Beijing, University of Science and Technology |
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| Copyright | Youke Publishing Co.,Ltd 2024. Springer Nature or its licensor (e.g. a society or other partner) holds exclusive rights to this article under a publishing agreement with the author(s) or other rightsholder(s); author self-archiving of the accepted manuscript version of this article is solely governed by the terms of such publishing agreement and applicable law. |
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| Keywords | 6H-SiC Piezo-catalytic degradation Rhodamine B (RhB) Harsh conditions Methylene blue (MB) |
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| Title | Efficient piezo-catalytic dye degradation using piezoelectric 6H-SiC under harsh conditions |
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