Highly sensitive strain sensors with wide operation range from strong MXene-composited polyvinyl alcohol/sodium carboxymethylcellulose double network hydrogel
Double network (DN) conductive hydrogels have become a hotspot for wearable sensors. However, building DN hydrogel-based strain sensors with excellent mechanical strength, high sensitivity, and wide operation window still remains a challenge. This paper fabricates a high-performance strain sensor fr...
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| Published in | Advanced composites and hybrid materials Vol. 5; no. 3; pp. 1976 - 1987 |
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| Main Authors | , , , , , , , , , , , , |
| Format | Journal Article |
| Language | English |
| Published |
Cham
Springer International Publishing
01.09.2022
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| Subjects | |
| Online Access | Get full text |
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| Abstract | Double network (DN) conductive hydrogels have become a hotspot for wearable sensors. However, building DN hydrogel-based strain sensors with excellent mechanical strength, high sensitivity, and wide operation window still remains a challenge. This paper fabricates a high-performance strain sensor from MXene-composited polyvinyl alcohol/sodium carboxymethylcellulose (PVA/CMC) DN hydrogel which is further reinforced by tannic acid (TA). In this PCTM (short for PVA/CMC/TA/MXene hydrogel), PVA serves as the flexible backbone, CMC mainly functions as the rigid subnetwork skeleton in the hydrogel, and naturally occurring TA further enhances the mechanical properties of the hydrogel via tight hydrogen bonds between TA and the polymer chains of PVA and CMC. MXene is utilized to build the conductive path, and its abundant hydrophilic functional groups help to achieve a uniform distribution in the hydrogel, which is beneficial for achieving high sensitivity and wide operation window. The unique multiple synergetic networks of PCTM impart promising mechanical strength (a fracture tensile strength of 1.8 MPa at a fracture strain of 740%) and high sensitivity with a wide detection window (a gauge factor of 2.9 at a strain range of 0–700%) as well as long-term durability over 3000 continuous cycles. Moreover, the sensor also exhibits accurate response to different types of human motions. As a proof of concept, a PCTM sensor is fabricated for visual detection of the pressure, suggesting its promising potentials for stretchable electronic sensors.
Graphical abstract |
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| AbstractList | Double network (DN) conductive hydrogels have become a hotspot for wearable sensors. However, building DN hydrogel-based strain sensors with excellent mechanical strength, high sensitivity, and wide operation window still remains a challenge. This paper fabricates a high-performance strain sensor from MXene-composited polyvinyl alcohol/sodium carboxymethylcellulose (PVA/CMC) DN hydrogel which is further reinforced by tannic acid (TA). In this PCTM (short for PVA/CMC/TA/MXene hydrogel), PVA serves as the flexible backbone, CMC mainly functions as the rigid subnetwork skeleton in the hydrogel, and naturally occurring TA further enhances the mechanical properties of the hydrogel via tight hydrogen bonds between TA and the polymer chains of PVA and CMC. MXene is utilized to build the conductive path, and its abundant hydrophilic functional groups help to achieve a uniform distribution in the hydrogel, which is beneficial for achieving high sensitivity and wide operation window. The unique multiple synergetic networks of PCTM impart promising mechanical strength (a fracture tensile strength of 1.8 MPa at a fracture strain of 740%) and high sensitivity with a wide detection window (a gauge factor of 2.9 at a strain range of 0–700%) as well as long-term durability over 3000 continuous cycles. Moreover, the sensor also exhibits accurate response to different types of human motions. As a proof of concept, a PCTM sensor is fabricated for visual detection of the pressure, suggesting its promising potentials for stretchable electronic sensors.
Graphical abstract |
| Author | Huang, Mina Wei, Huige Nassan, Mohamed A. Faheim, Abeer A. Li, Ang El-Bahy, Zeinhom M. Li, Jiongru Kong, Deshuo Algadi, Hassan Cui, Dapeng Xu, Cuixia El-Bahy, Salah M. Li, Tuo |
| Author_xml | – sequence: 1 givenname: Deshuo surname: Kong fullname: Kong, Deshuo organization: Tianjin Key Laboratory of Brine Chemical Engineering and Resource Eco-Utilization, College of Chemical Engineering and Materials Science, Tianjin University of Science and Technology – sequence: 2 givenname: Zeinhom M. surname: El-Bahy fullname: El-Bahy, Zeinhom M. organization: Department of Chemistry, Faculty of Science, Al-Azhar University – sequence: 3 givenname: Hassan surname: Algadi fullname: Algadi, Hassan organization: Department of Electrical Engineering, Faculty of Engineering, Najran University – sequence: 4 givenname: Tuo surname: Li fullname: Li, Tuo organization: Tianjin Key Laboratory of Brine Chemical Engineering and Resource Eco-Utilization, College of Chemical Engineering and Materials Science, Tianjin University of Science and Technology – sequence: 5 givenname: Salah M. surname: El-Bahy fullname: El-Bahy, Salah M. organization: Department of Chemistry, Turabah University College, Taif University – sequence: 6 givenname: Mohamed A. surname: Nassan fullname: Nassan, Mohamed A. organization: Department of Clinical Laboratory Sciences, Turabah University College, Taif University – sequence: 7 givenname: Jiongru surname: Li fullname: Li, Jiongru organization: Tianjin Key Laboratory of Brine Chemical Engineering and Resource Eco-Utilization, College of Chemical Engineering and Materials Science, Tianjin University of Science and Technology – sequence: 8 givenname: Abeer A. surname: Faheim fullname: Faheim, Abeer A. organization: Department of Chemistry, Faculty of Science, Al-Azhar University – sequence: 9 givenname: Ang surname: Li fullname: Li, Ang organization: Tianjin Key Laboratory of Brine Chemical Engineering and Resource Eco-Utilization, College of Chemical Engineering and Materials Science, Tianjin University of Science and Technology – sequence: 10 givenname: Cuixia surname: Xu fullname: Xu, Cuixia organization: Analytical Development Department, Aucta Pharmaceuticals Inc – sequence: 11 givenname: Mina surname: Huang fullname: Huang, Mina organization: College of Materials Science and Engineering, Taiyuan University of Science and Technology – sequence: 12 givenname: Dapeng surname: Cui fullname: Cui, Dapeng email: dapeng@tust.edu.cn organization: College of Light Industry Science and Engineering, Tianjin University of Science and Technology – sequence: 13 givenname: Huige orcidid: 0000-0003-3977-1147 surname: Wei fullname: Wei, Huige email: huigewei@tust.edu.cn organization: Tianjin Key Laboratory of Brine Chemical Engineering and Resource Eco-Utilization, College of Chemical Engineering and Materials Science, Tianjin University of Science and Technology |
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| Keywords | Wide operation window High sensitivity Stretchable electronic sensors Double network |
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| Snippet | Double network (DN) conductive hydrogels have become a hotspot for wearable sensors. However, building DN hydrogel-based strain sensors with excellent... |
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| Title | Highly sensitive strain sensors with wide operation range from strong MXene-composited polyvinyl alcohol/sodium carboxymethylcellulose double network hydrogel |
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