Bifunctional nanoparticle–SILP catalysts (NPs@SILP) for the selective deoxygenation of biomass substrates
Ruthenium nanoparticles were immobilized onto an acidic supported ionic liquid phase (RuNPs[at]SILP) in the development of bifunctional catalysts for the selective deoxygenation of biomass substrates. RuNPs[at]SILPs possessed high catalytic activities, selectivities and recyclabilities in the hydrog...
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| Published in | Chemical science (Cambridge) Vol. 5; no. 12; pp. 4895 - 4905 |
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| Main Authors | , , , , , |
| Format | Journal Article |
| Language | English |
| Published |
01.01.2014
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| Subjects | |
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| Abstract | Ruthenium nanoparticles were immobilized onto an acidic supported ionic liquid phase (RuNPs[at]SILP) in the development of bifunctional catalysts for the selective deoxygenation of biomass substrates. RuNPs[at]SILPs possessed high catalytic activities, selectivities and recyclabilities in the hydrogenolytic deoxygenation and ring opening of C sub(8)- and C sub(9)-substrates derived from furfural or 5-hydroxymethylfurfural and acetone. Tailoring the acidity of the SILP through the ionic liquid loading provided a molecular parameter by which the catalytic activity and selectivity of the RuNPs[at]SILPs were controlled to provide a flexible catalyst system toward the formation of different classes of value-added products: cyclic ethers, primary alcohols or aliphatic ethers. |
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| AbstractList | Ruthenium nanoparticles were immobilized onto an acidic supported ionic liquid phase (RuNPs[at]SILP) in the development of bifunctional catalysts for the selective deoxygenation of biomass substrates. RuNPs[at]SILPs possessed high catalytic activities, selectivities and recyclabilities in the hydrogenolytic deoxygenation and ring opening of C sub(8)- and C sub(9)-substrates derived from furfural or 5-hydroxymethylfurfural and acetone. Tailoring the acidity of the SILP through the ionic liquid loading provided a molecular parameter by which the catalytic activity and selectivity of the RuNPs[at]SILPs were controlled to provide a flexible catalyst system toward the formation of different classes of value-added products: cyclic ethers, primary alcohols or aliphatic ethers. |
| Author | Luska, Kylie L. Leitner, Walter Adams, Alina Julis, Jennifer Stavitski, Eli Zakharov, Dmitri N. |
| Author_xml | – sequence: 1 givenname: Kylie L. surname: Luska fullname: Luska, Kylie L. – sequence: 2 givenname: Jennifer surname: Julis fullname: Julis, Jennifer – sequence: 3 givenname: Eli surname: Stavitski fullname: Stavitski, Eli – sequence: 4 givenname: Dmitri N. surname: Zakharov fullname: Zakharov, Dmitri N. – sequence: 5 givenname: Alina surname: Adams fullname: Adams, Alina – sequence: 6 givenname: Walter surname: Leitner fullname: Leitner, Walter |
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| SubjectTerms | Biomass Catalysis Catalysts Catalytic activity Deoxygenation Ethers Ionic liquids Selectivity |
| Title | Bifunctional nanoparticle–SILP catalysts (NPs@SILP) for the selective deoxygenation of biomass substrates |
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