Polymer electrolyte lithium batteries rechargeability and positive electrode degradation : an AC impedance study
The relationship between cycling performance and AC impedance measurements were used to elucidate some of the reported failure mechanisms of rechargeable lithium polymer electrolyte batteries. The rapid initial capacity decay observed within the first few cycles of the polymer electrolyte/V sub(6)O...
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| Published in | Journal of applied electrochemistry Vol. 21; no. 4; pp. 301 - 307 |
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| Main Authors | , , , , |
| Format | Journal Article |
| Language | English |
| Published |
Heidelberg
Springer
01.04.1991
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| Subjects | |
| Online Access | Get full text |
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| Abstract | The relationship between cycling performance and AC impedance measurements were used to elucidate some of the reported failure mechanisms of rechargeable lithium polymer electrolyte batteries. The rapid initial capacity decay observed within the first few cycles of the polymer electrolyte/V sub(6)O sub(13) based composite cathode is shown to be related to the properties of the composite cathode active material, while the slower capacity decay observed during subsequent cycles, under continuous cycling regimes, appears to be related to a loss of ionic and electronic contact in the composite cathode. |
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| AbstractList | The relationship between cycling performance and AC impedance measurements were used to elucidate some of the reported failure mechanisms of rechargeable lithium polymer electrolyte batteries. The rapid initial capacity decay observed within the first few cycles of the polymer electrolyte/V sub(6)O sub(13) based composite cathode is shown to be related to the properties of the composite cathode active material, while the slower capacity decay observed during subsequent cycles, under continuous cycling regimes, appears to be related to a loss of ionic and electronic contact in the composite cathode. |
| Author | KOKSBANG, R OLSEN, I. I FAUTEUX, D KNUDSEN, N TONDER, P. E |
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| Issue | 4 |
| Keywords | Cathode Electrode electrolyte interface Lithium Polymer Secondary cell Electrode material Vanadium Oxides Thin film Charge discharge cycle Electrolyte Battery Fault diagnostic Electrical impedance |
| Language | English |
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| References | R. Koksbang (CR33) 1989; 136 S. Morzilli (CR22) 1987; 32 S. Skaarup (CR8) 1988 D. H. Shen (CR15) 1989 (CR5) 1984 B. A. Boukamp (CR34) 1984; 11 F. Bonino (CR18) 1986; 18 B. V. Ratnakumar (CR27) 1989; 19 F. C. Laman (CR31) 1985; 14 J. S. Lundsgaard (CR3) 1990 M. B. Armand (CR2) 1979 M. Hiratani (CR19) 1988; 28?30 R. Koksbang (CR4) 1990; 32 C. C. Hunter (CR9) 1988; 24 B. Scrosati (CR10) 1989; 136 M. G. S. R. Thomas (CR28) 1985; 132 J. G. Thevenin (CR14) 1987; 134 B. C. H. Steele (CR26) 1983; 9/10 P. G. Bruce (CR30) 1989; 36 M. Gauthier (CR7) 1989 CR1 F. Croce (CR23) 1988; 18 G. Montesperelli (CR17) 1990; 37 M. Gauthier (CR6) 1985; 132 T. Jacobsen (CR32) 1985; 30 B. Scrosati (CR11) 1988; 20 P. G. Bruce (CR29) 1988; 33 P. W. M. Jacobs (CR20) 1989; 26 D. Fauteux (CR24) 1985; 17 R. V. Moshtev (CR16) 1984; 180 S. Panero (CR12) 1983; 130 J. Thevenin (CR13) 1985; 14 D. Fauteux (CR25) 1988; 135 P. Ravn Sorensen (CR21) 1982; 27 K. West (CR35) 1983; 28 |
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Ratnakumar – volume: 28?30 start-page: 1431 year: 1988 ident: CR19 publication-title: Solid State Ionics doi: 10.1016/0167-2738(88)90398-0 contributor: fullname: M. Hiratani – volume: 20 start-page: 219 year: 1988 ident: CR11 publication-title: Brit. Polym. J. doi: 10.1002/pi.4980200311 contributor: fullname: B. Scrosati – volume: 134 start-page: 273 year: 1987 ident: CR14 publication-title: J. Electrochem. Soc. doi: 10.1149/1.2100445 contributor: fullname: J. G. Thevenin |
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| SubjectTerms | Applied sciences Direct energy conversion and energy accumulation Electrical engineering. Electrical power engineering Electrical power engineering Electrochemical conversion: primary and secondary batteries, fuel cells Exact sciences and technology |
| Title | Polymer electrolyte lithium batteries rechargeability and positive electrode degradation : an AC impedance study |
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